Article
Chemistry, Inorganic & Nuclear
Pengxiang Pei, Pengbo DuanMu, Binbin Wang, Xuan Miao, Cheng Zhang, Weisheng Liu
Summary: The multicolor long persistent luminescence material NCGOF:Tb3+ can achieve color changes from blue to cyan and bright green by adjusting the concentration of Tb3+, with afterglow times ranging from 5.62 hours to 8.52 hours. Anticounterfeiting devices fabricated based on this material can be easily detected using a portable ultraviolet lamp and are impossible to counterfeit.
DALTON TRANSACTIONS
(2021)
Article
Chemistry, Physical
Yunhui Wu, Jiurong Li, Xiujian Zhao, Xiao Gong
Summary: In this study, nickel-doped carbon dots (Ni-CDs) with tunable fluorescence emission were successfully synthesized using a simple one-step solvothermal method. The introduction of Ni enhanced the fluorescence intensity and caused a redshift. By mixing Ni-CDs with polyvinylpyrrolidone (PVP), the self-quenching effect of solid-state fluorescence was effectively avoided. Based on this, high-performance green, yellow, and red light-emitting diodes (LEDs) were constructed, demonstrating the potential of these carbon dots for solid-state lighting applications.
Article
Engineering, Environmental
Jianhao Hua, Peng Hua, Kunhao Qin
Summary: In this study, nitrogen and fluorine co-doped carbon dots (N, F-CDs) were successfully prepared, exhibiting high fluorescence quantum yield, tunable multicolor emission, and excellent antibacterial activity. These versatile N, F-CDs were applied in biolabeling and antibacterial experiments, and the antibacterial mechanisms were studied at the molecular level. This work provides new insights for the development of highly fluorescent multicolor carbon dots and facilitates the design and application of carbon dots-based nanomaterials in biological environments.
JOURNAL OF HAZARDOUS MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Hyeong Seop Shim, Jun Myung Kim, Seonghyun Jeong, Youngwon Ju, Sung Jae Won, Jeongyun Choi, Sangwon Nam, Aniruddha Molla, Joohoon Kim, Jae Kyu Song
Summary: Three types of carbon dots with low toxicity, high stability, and high quantum yield were synthesized, showing distinct optical transitions and single chromophore-like nature. The controllability of optical transitions in carbon dots enhances their potential for various applications as alternatives to toxic element-containing quantum dots.
NANOSCALE ADVANCES
(2022)
Article
Chemistry, Multidisciplinary
Yan Li, Can Liu, Yulong An, Menglin Chen, Yunwu Zheng, Hao Tian, Rui Shi, Xiahong He, Xu Lin
Summary: Multicolor luminescent carbon dots were prepared by a solvothermal method using tannic acid and phthalaldehyde as carbon sources. The distinct optical features of these carbon dots are based on differences in the sizes of sp(2) domains, which can be governed by the structure of phthalaldehyde.
NEW JOURNAL OF CHEMISTRY
(2021)
Article
Polymer Science
Lorenzo Vallan, Anh Thy Bui, Gediminas Jonusauskas, Nathan D. McClenaghan, Emin Istif, Daniele Mantione, Eleni Pavlopoulou, Cyril Brochon, Georges Hadziioannou, Eric Cloutet
Summary: In recent years, there has been considerable interest in nonconjugated organic luminophores, which provide a new conceptual basis for alternative photoluminescence-based technologies. This study utilized the polymerization of 3,4-dihydropyran to prepare nonconjugated photoluminescent polymer nanoparticles. The remarkable feature of this material is its excitation-dependent multicoloremission, ranging from blue to yellow, which is attributed to the presence of independent, non-interacting chromophores on the polymer structure. The removal of unsaturated structures furthermore enhances the photoluminescence quantum yield (QY) of the polymer up to 0.20 (lambda(ex) = 355 nm). This work introduces a new type of nonconjugated organic luminophore with high QY and multicoloremission.
Article
Chemistry, Multidisciplinary
Longshi Rao, Qing Zhang, Bin Sun, Mingfu Wen, Jiayang Zhang, Guisheng Zhong, Ting Fu, Xiaodong Niu
Summary: Using a solvent engineering strategy, full-color emissive carbon dots (CDs) were produced with excellent photoelectric properties and stable fluorescence performance. By tuning the volume ratio of water and dimethylformamide (H2O/DMF), the emission wavelengths of the CDs changed, and they exhibited stable fluorescence performance even after undergoing heating and UV light irradiation. Bright multicolor light-emitting diodes with a high color rendering index (CRI) were obtained using these CDs.
Article
Chemistry, Multidisciplinary
Xu Wang, Huyun Sun, Yingxi Lu, Xianfeng Zhou
Summary: In this study, fluorescent non-conjugated polymeric multilayers with tunable multicolor photoluminescence were prepared using a simple layer-by-layer assembly method. These multilayers exhibited strong blue, green, and red fluorescence in the visible region and showed different sensitivities to metal ions. The LbL-assembled multilayers provide a new perspective for the preparation of fluorescent non-conjugated polymeric films, offering a simpler synthesis route and excellent photo stability and biocompatibility.
MATERIALS CHEMISTRY FRONTIERS
(2023)
Article
Chemistry, Multidisciplinary
Yan Li, Can Liu, Hao Sun, Menglin Chen, Defa Hou, Yunwu Zheng, Haijiao Xie, Bei Zhou, Xu Lin
Summary: This paper presents a method to obtain multicolor luminescent carbon dots by pyrolysis under different reaction conditions, revealing the forbidden band tuning and formation mechanism of carbon dots. Different acid-base conditions lead to different reaction paths of the precursors, forming molecular fluorophores with different conjugated structures, which eventually form carbon dots and enhance the photoluminescence of the system by inhibiting the movement of the fluorescent centers.
Review
Chemistry, Inorganic & Nuclear
Yujia Liu, Thanawat Chaiprasert, Armelle Ouali, Masafumi Unno
Summary: This review provides an overview of synthetic routes to different stereoregular CSDs and discusses their potential applications in various fields. The synthesis and functionalization methods of all-cis-T-4 are emphasized, highlighting the possible research directions of CSDs in the future.
DALTON TRANSACTIONS
(2022)
Article
Chemistry, Multidisciplinary
Bin Liu, Bo Chu, Ya-Ling Wang, Lan-Fang Hu, Shengliang Hu, Xing-Hong Zhang
Summary: This study presents a new type of carbon dioxide (CO2)-derived CPD with significant quantum yields in both solution and solid state. The synthesis of CPDs involved the polymerization of small molecules and the self-passivation of poly(hydroxyurethane) chains, allowing for solid-state fluorescence. Additionally, the synthesis process consumes a significant amount of CO2, offering a new method for fixing CO2 to functional carbon materials.
Article
Chemistry, Multidisciplinary
Yulong An, Xu Lin, Yuxi Zhou, Yan Li, Yunwu Zheng, Chunhua Wu, Kaimeng Xu, Xijuan Chai, Can Liu
Summary: Red, green, and blue carbon dots (RGB CDs) were successfully synthesized with stable optical properties and significant photoluminescence characteristics. A white fluorescent CD solution was prepared by mixing these multicolor fluorescent CDs in appropriate proportions.
Review
Chemistry, Multidisciplinary
Md Moniruzzaman, Jongsung Kim
Summary: Carbon dots (CDs) with unique and tunable multicolor photoluminescence (PL) emission have received great attention in recent years for their potential applications in the biomedical and optoelectronic fields. This review focuses on the advancement of synthesis and post-synthesis techniques for achieving tunable multicolor emission. Various synthesis strategies and post synthesis strategies have been discussed, including the selection of benzenoid precursor, acid/base treatment, optimization of reaction conditions, solvent engineering, and chemical doping. Furthermore, the need for a concise review article focusing on systematic synthesis and post synthesis strategies with PL mechanism elucidation is highlighted.
Article
Chemistry, Physical
Mattia Salomone, Michele Re Fiorentin, Giancarlo Cicero, Francesca Risplendi
Summary: The study analyzes the stability and electronic properties of an InSe monolayer with point defects, showing the presence of deep defect states within the band gap. It predicts that Ge as a substitution impurity of Se could be a promising material for single-photon emitters due to its optical properties and strongly peaked spectrum in the near-infrared.
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
(2021)
Article
Nanoscience & Nanotechnology
Panpan Zhu, Jiayu Li, Lixia Gao, Jie Xiong, Kejun Tan
Summary: Research on multiemission fluorescent carbon dots excited at one wavelength has shown great promise due to their label-free property, easy synthesis, multicolor visualization, and ability to prevent background interference. A new template strategy using fluorescent precursors has been developed for the synthesis of multiemission carbon dots (M-CDs), which show three different emissions attributed to solvent, surface defect, and precursor luminophores. The M-CDs can meet optical requirements by adjusting the amount of NaOH or solvothermal synthesis time, demonstrating better capabilities than previously reported M-CDs. Additionally, a multicolor sensor using M-CDs and rhodamine B has been successfully utilized for cell imaging, showing a color evolution from dark blue to orange based on the pH value of the medium.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Biochemical Research Methods
Fuchun Si, Zenghui Liu, Jinge Li, Huaixia Yang, Yanju Liu, Jinming Kong
Summary: An electrochemical detection strategy for exosomes was established based on DNA/ferrocene-modified single-walled carbon nanotube complex. The method showed high sensitivity and good selectivity, providing a potential platform for early diagnosis and biomedical applications.
ANALYTICAL BIOCHEMISTRY
(2023)
Review
Engineering, Biomedical
Ke Liang, Jiechao Ge, Pengfei Wang
Summary: Carbon dots (CDs) are recognized as emerging nanotheranostics for biomedical applications. The introduction of metal ion in CDs endowed metal-doped CDs (MCDs) with tunable optical properties and new intrinsic properties. This review summarizes the recent progress and discusses the challenges and potential development of photonic MCDs as emerging nanoagents for disease-related diagnostic and cancer therapy.
BIOMEDICAL MATERIALS
(2023)
Article
Nanoscience & Nanotechnology
Honglei Gao, Zhiyi Li, Zhi Pang, Yuanyuan Qin, Guanhao Liu, Teng Gao, Xiangyu Dong, Shaogang Shen, Xin Xie, Pengfei Wang, Chun-Sing Lee, Ying Wang
Summary: Novel ultrapure blue TADF emitters of TSBA-Cz and TSBA-PhCz were designed and synthesized for high-efficiency OLEDs. These emitters exhibited a pure blue emission peak, narrow FWHM, and small Delta EST, showcasing excellent TADF behavior. The TADFOLED devices using these emitters achieved ultrapure blue EL with narrow FWHM and high external quantum efficiencies.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Chemistry, Multidisciplinary
Hui Ma, Qianqian Jiang, Xinlei Ma, Ruoqi Chen, Kun Hua, Xiubin Yang, Jiechao Ge, Junhui Ji, Mianqi Xue
Summary: Lossless and efficient robotic grasping is crucial in various fields, but current sensors for grasping behavior feedback face limitations. To solve this, lightweight distance sensor-based microfibers were developed to assist robotic grasping. The microsensor exhibited high sensitivity, fast response time, high resolution, and stability. By correlating the sensor's signal with the grasp state, safe and effective grasping and release can be achieved. The lightweight and high-powered distance sensor has potential applications in intelligent fetching, medical surgery, automatic machines, and cultural relics excavation.
Article
Nanoscience & Nanotechnology
Haoran Wang, Tiejin Chen, Haohui Ren, Weimin Liu, Fuchun Nan, Jiechao Ge, Pengfei Wang
Summary: Photodynamic therapy (PDT) based on the generation of reactive oxygen species (ROS) has gained attention in tumor treatment. However, the hypoxic tumor microenvironment inhibits ROS generation and high glutathione levels neutralize ROS, reducing the effectiveness of PDT. This study constructs porphyrinic metal-organic framework PCN-224 and decorates it with gold nanoparticles (PCN-224@Au) to enhance ROS generation and deplete glutathione, amplifying damage to cancer cells. In vitro and in vivo experiments demonstrate that PCN-224@Au can serve as an oxidative stress amplifier for enhanced PDT, providing a promising solution for addressing intratumor hypoxia and high GSH levels.
ACS APPLIED BIO MATERIALS
(2023)
Article
Engineering, Biomedical
Shuaishuai Bian, Xiuli Zheng, Weimin Liu, Jihao Li, Zekun Gao, Haohui Ren, Wenjun Zhang, Chun-Sing Lee, Pengfei Wang
Summary: In this study, a highly-stable and bright aggregation induced emission (AIE) fluorophore (PTPE3 NP) was developed for dynamic fluorescence (FL) imaging of vascular dysfunction beyond the 1300 nm window during vascular-targeted photodynamic therapy (V-PDT). The PTPE3 NP showed excellent brightness and high resolution, enabling clear images of vasculature and real-time tracking of blood circulation. Furthermore, the PTPE3 NP allowed visualization of mesenteric and tumor vascular dysfunction and real-time monitoring of blood flow velocity (BFV) during V-PDT, providing a powerful approach to assess vascular responses and evaluate the efficacy of V-PDT.
Article
Engineering, Biomedical
Lin Kong, Jian Wang, Yunxiu Zhang, Ke Liang, Jian Li, Xiaokuang Xue, Tiejin Chen, Jiechao Ge, Pengfei Wang
Summary: Photodynamic therapy (PDT) is an emerging treatment method that has attracted interest due to its non-invasiveness, repeatable treatment, high spatiotemporal resolution, and few side effects. However, the short lifespan and diffusion distance of reactive oxygen species in tumor cells seriously limit the therapeutic efficacy of PDT. Therefore, the design and preparation of photosensitizers targeting specific subcellular organelles can significantly improve the efficacy of PDT.
BIOMEDICAL MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Ke Liang, Fanghao Zhao, Fuchun Nan, Jian Wang, Yunxiu Zhang, Jian Li, Xiaokuang Xue, Tiejin Chen, Lin Kong, Jiechao Ge, Pengfei Wang
Summary: In this study, a triple reactive oxygen species (ROS) generator, hyaluronic acid-modified Pt nanoparticles/carbon dots-loaded mesoporous silica (HA-PCD), was developed for photodynamic/catalytic combination therapy of hypoxic tumors. Under laser irradiation, HA-PCD generated singlet oxygen (O-1(2)) and Pt nanoparticles produced oxygen and hydroxyl radicals for enhanced therapy. The surface modification of HA facilitated tumor cell targetability. This novel nanoplatform shows great potential for synergistic photodynamic/catalytic therapy of hypoxic tumors.
MATERIALS CHEMISTRY FRONTIERS
(2023)
Article
Chemistry, Multidisciplinary
Xuewei Li, Weimin Liu, Xiuli Zheng, Meiyu Jiang, Yimin Guo, Jie Sha, Jiasheng Wu, Haohui Ren, Honglei Gao, Shuai Wang, Pengfei Wang
Summary: Two photosensitizers (CCOH and CCN) were designed and synthesized by incorporating coumarin into the curcumin structure. Compared with curcumin, CCOH and CCN generated more reactive oxygen species (ROS) through type I and II synergy upon light irradiation. Cell experiments demonstrated that CCN, with excellent LD-targeting effect, could be utilized to monitor the changes in morphology and number of LDs in tumor cells during PDT.
CHEMICAL COMMUNICATIONS
(2023)
Article
Chemistry, Multidisciplinary
Xiuli Zheng, Sheng-Nan Lei, Zekun Gao, Xiangyu Dong, Hongyan Xiao, Weimin Liu, Chen-Ho Tung, Li-Zhu Wu, Pengfei Wang, Huan Cong
Summary: Researchers report two fluorescent hydrophilic cyclophanes that can effectively bind hypocrellin B (HB), a commonly used photosensitizer for photodynamic therapy (PDT), with high binding constants in aqueous solutions. The macrocycles have extended electron-deficient cavities and can be easily synthesized through photo-induced ring expansions. The resulting supramolecular PSs show desirable stability, biocompatibility, and cellular delivery, as well as excellent PDT efficiency against cancer cells. Moreover, cell imaging results indicate different delivery effects at the cellular level for the two supramolecular PSs.
Article
Engineering, Biomedical
Shuaishuai Bian, Xiuli Zheng, Weimin Liu, Zekun Gao, Yingpeng Wan, Jihao Li, Haohui Ren, Wenjun Zhang, Chun-Sing Lee, Pengfei Wang
Summary: This study developed a pH-responsive nanoplatform for real-time monitoring of tumor vascular disruption, long-term tracking of tumor progression, and combined anti-vascular/photothermal therapy.
Article
Materials Science, Biomaterials
Yanping Wang, Xuewei Li, Weimin Liu, Jie Sha, Zhe Yu, Shuai Wang, Haohui Ren, Wenjun Zhang, Chun-Sing Lee, Pengfei Wang
Summary: This work describes the synthesis and application of a curcumin-based photosensitizer, CN, which can simultaneously target lipid droplets and the endoplasmic reticulum, enhancing the efficiency of photodynamic therapy. CN exhibits longer absorption and emission wavelengths and sensitivity to polarity, leading to excellent photodynamic effects. The phototoxicity of CN results in apoptosis by destroying the endoplasmic reticulum and ferroptosis by oxidizing polyunsaturated fatty acids in lipid droplets.
JOURNAL OF MATERIALS CHEMISTRY B
(2023)
Article
Chemistry, Multidisciplinary
Laetitia Bardet, Herve Roussel, Stefano Saroglia, Masoud Akbari, David Munoz-Rojas, Carmen Jimenez, Aurore Denneulin, Daniel Bellet
Summary: The thermal instability of silver nanowires leads to increased electrical resistance in AgNW networks. Understanding the relationship between structural and electrical properties of AgNW networks is crucial for their integration as transparent electrodes in flexible optoelectronics. In situ X-ray diffraction measurements were used to study the crystallographic evolution of Ag-specific Bragg peaks during thermal ramping, revealing differences in thermal and structural transitions between bare and SnO2-coated AgNW networks.
Article
Chemistry, Multidisciplinary
Nathalia Cancino-Fuentes, Arnau Manasanch, Joana Covelo, Alex Suarez-Perez, Enrique Fernandez, Stratis Matsoukis, Christoph Guger, Xavi Illa, Anton Guimera-Brunet, Maria V. Sanchez-Vives
Summary: This study provides a comprehensive characterization of graphene-based solution-gated field-effect transistors (gSGFETs) for brain recordings, highlighting their potential clinical applications.
Article
Chemistry, Multidisciplinary
Sikandar Aftab, Hailiang Liu, Dhanasekaran Vikraman, Sajjad Hussain, Jungwon Kang, Abdullah A. Al-Kahtani
Summary: This study examines the effects of hybrid nanoparticles made of NiO@rGO and NiO@CNT on the active layers of polymer solar cells and X-ray photodetectors. The findings show that these hybrid nanoparticles can enhance the charge carrier capacities and exciton dissociation properties of the active layers. Among the tested configurations, the NiO@CNT device demonstrates superior performance in converting sunlight into electricity, and achieves the best sensitivity for X-ray detection.
Article
Chemistry, Multidisciplinary
Hyo Jung Shin, Seung Gyu Choi, Fengrui Qu, Min-Hee Yi, Choong-Hyun Lee, Sang Ryong Kim, Hyeong-Geug Kim, Jaewon Beom, Yoonyoung Yi, Do Kyung Kim, Eun-Hye Joe, Hee-Jung Song, Yonghyun Kim, Dong Woon Kim
Summary: This study investigates the role of SOX9 in reactive astrocytes following ischemic brain damage using a PLGA nanoparticle plasmid delivery system. The results demonstrate that PLGA nanoparticles can reduce ischemia-induced neurological deficits and infarct volume, providing a potential opportunity for stroke treatment.
Article
Chemistry, Multidisciplinary
Anurag Chaudhury, Koushik Debnath, Nikhil R. Jana, Jaydeep K. Basu
Summary: The study investigates the interaction between nanoparticles and cell membranes, and identifies key parameters, including charge, crowding, and membrane fluidity, that determine the adsorbed concentration and unbinding transition of nanoparticles.
Article
Chemistry, Multidisciplinary
Sina Sadeghi, Fazel Bateni, Taekhoon Kim, Dae Yong Son, Jeffrey A. Bennett, Negin Orouji, Venkat S. Punati, Christine Stark, Teagan D. Cerra, Rami Awad, Fernando Delgado-Licona, Jinge Xu, Nikolai Mukhin, Hannah Dickerson, Kristofer G. Reyes, Milad Abolhasani
Summary: In this study, an autonomous approach for the development of lead-free metal halide perovskite nanocrystals is presented, which integrates a modular microfluidic platform with machine learning-assisted synthesis modeling. This approach enables rapid and optimized synthesis of copper-based lead-free nanocrystals.
Article
Chemistry, Multidisciplinary
Zahir Abbas, Nissar Hussain, Surender Kumar, Shaikh M. Mobin
Summary: The rational construction of free-standing and flexible electrodes for electrochemical energy storage devices is an emerging research focus. In this study, a redox-active metal-organic framework (MOF) was prepared on carbon nanofibers using an in situ approach, resulting in a flexible electrode with high redox-active behavior and unique properties such as high flexibility and lightweight. The prepared electrode showed excellent cyclic retention and rate capability in supercapacitor applications. Additionally, it could be used as a freestanding electrode in flexible devices at different bending angles.
Article
Chemistry, Multidisciplinary
Lishan Zhang, Xiaoting Zhang, Hui Ran, Ze Chen, Yicheng Ye, Jiamiao Jiang, Ziwei Hu, Miral Azechi, Fei Peng, Hao Tian, Zhili Xu, Yingfeng Tu
Summary: Photodynamic therapy (PDT) is a promising local treatment modality in cancer therapy, but its therapeutic efficacy is restricted by ineffective delivery of photosensitizers and tumor hypoxia. In this study, a phototactic Chlorella-based near-infrared (NIR) driven green affording-oxygen microrobot system was developed for enhanced PDT. The system exhibited desirable phototaxis and continuous oxygen generation, leading to the inhibition of tumor growth in mice. This study demonstrates the potential of using a light-driven green affording-oxygen microrobot to enhance photodynamic therapy.
Article
Chemistry, Multidisciplinary
Yujin Li, Jing Xu, Xinqi Luo, Futing Wang, Zhong Dong, Ke-Jing Huang, Chengjie Hu, Mengyi Hou, Ren Cai
Summary: In this study, hollow heterostructured materials were constructed using an innovative template-engaged method as cathodes for zinc-ion batteries. The materials exhibited fast Zn2+ transport channels, improved electrical conductivity, and controlled volume expansion during cycling. The designed structure allowed for an admirable reversible capacity and high coulombic efficiency.
Article
Chemistry, Multidisciplinary
Paritosh Mahato, Shashi Shekhar, Rahul Yadav, Saptarshi Mukherjee
Summary: This study comprehensively elucidates the role of the core and electrostatic surface of metal nanoclusters in catalytic reduction reactions. The electrostatic surface dramatically modulates the reactivity of metal nanoclusters.
Article
Chemistry, Multidisciplinary
Pei Liu, Mengdi Liang, Zhengwei Liu, Haiyu Long, Han Cheng, Jiahe Su, Zhongbiao Tan, Xuewen He, Min Sun, Xiangqian Li, Shuai He
Summary: This study demonstrates a simple and environmentally-friendly method for the synthesis of zinc oxide nanozymes (ZnO NZs) using wasted hop extract (WHE). The WHE-ZnO NZs exhibit exceptional peroxidase-like activity and serve as effective catalysts for the oxidation of 3,3,5,5-tetramethylbenzidine (TMB) in the presence of hydrogen peroxide (H2O2). In addition, a straightforward colorimetric technique for detecting both H2O2 and glucose was developed using the WHE-ZnO NZs as peroxidase-like catalysts.
Article
Chemistry, Multidisciplinary
Hyunkyu Oh, Young Jun Lee, Eun Ji Kim, Jinseok Park, Hee-Eun Kim, Hyunsoo Lee, Hyunjoo Lee, Bumjoon J. Kim
Summary: Mesoporous carbon particles have unique structural properties that make them suitable as support materials for catalytic applications. This study investigates the impact of channel nanostructures on the catalytic activity of porous carbon particles (PCPs) by fabricating PCPs with controlled channel exposure on the carbon surface. The results show that PCPs with highly open channel nanostructures exhibit significantly higher catalytic activity compared to those with closed channel nanostructures.
Article
Chemistry, Multidisciplinary
Yunjie Lu, Zhaohui Li, Zewei Li, Shihao Zhou, Ning Zhang, Jianming Zhang, Lu Zong
Summary: A tough, long-lasting adhesive and highly conductive nanocomposite hydrogel (PACPH) was fabricated via the synergy of interfacial entanglement and adhesion group densification. PACPH possesses excellent mechanical properties, interfacial adhesion strength, and conductivity, making it a promising material for long-term monitoring of human activities and electrocardiogram signals.
Article
Chemistry, Multidisciplinary
Zichao Wei, Audrey Vandergriff, Chung-Hao Liu, Maham Liaqat, Mu-Ping Nieh, Yu Lei, Jie He
Summary: We have developed a simple method to prepare polymer-grafted plasmonic metal nanoparticles with pH-responsive surface-enhanced Raman scattering. By using pH-responsive polymers as ligands, the aggregation of nanoparticles can be controlled, leading to enhanced SERS. The pH-responsive polymer-grafted nanoparticles show high reproducibility and sensitivity in solution, providing a novel approach for SERS without the need for sample pre-concentration.
Article
Chemistry, Multidisciplinary
Melis Ozge Alas Colak, Ahmet Gungor, Merve Buldu Akturk, Emre Erdem, Rukan Genc
Summary: This research investigates the effect of functionalizing carbon dots with hydroxyl polymers on their performance as electrode materials in a supercapacitor. The results show that the functionalized carbon dots exhibit excellent electrochemical performance and improved stability.
