Article
Green & Sustainable Science & Technology
Min Zhong, Jiawei Yan, Lei Wang, Ye Huang, Li Li, Shenghui Gao, Yafei Tian, Wenzhuo Shen, Jiali Zhang, Shouwu Guo
Summary: In this study, porous graphite modified with graphene oxide was prepared, resulting in a hierarchical porous composite material. This unique structure not only facilitates the transfer and diffusion of electrons and ions, but also provides more active sites, greatly improving the electrochemical performance. The composite material exhibits excellent reversible capacity, capacity retention, and cycling stability.
SUSTAINABLE MATERIALS AND TECHNOLOGIES
(2022)
Article
Nanoscience & Nanotechnology
Yangcheng Mo, Shuchan Li, Jie Yu
Summary: Graphene greatly improves the performance of silicon anodes, making them highly promising for high-performance lithium-ion batteries.
ACS APPLIED NANO MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Jinhui Xu, Qingyang Yin, Xinru Li, Xinyi Tan, Qian Liu, Xing Lu, Bocheng Cao, Xintong Yuan, Yuzhang Li, Li Shen, Yunfeng Lu
Summary: Novel anode materials for lithium-ion batteries were synthesized by growing spheres of graphene and carbon nanotubes around silicon particles, resulting in composites with high electrical conductivity and mechanical resiliency. These materials can withstand the high-pressure calendering process in electrode fabrication and the stress induced during charging and discharging of the electrodes.
Article
Nanoscience & Nanotechnology
Hongyan Zhou, Mengjing Jin, Bojian Zhou, Jianguo Zhao, Weihua Han
Summary: The composite material of SnO2/MoO3 at a 1:1 ratio showed exceptional electrochemical performance after 300 cycles, attributed to its unique 3D porous structure. The addition of graphene improved electrical conductivity, resulting in better electrochemical performance of SnO2/MoO3@Graphene composite material.
Article
Chemistry, Multidisciplinary
Sul Ki Park, Davor Copic, Tommy Zijian Zhao, Agnieszka Rutkowska, Bo Wen, Kate Sanders, Ruhan He, Hyun-Kyung Kim, Michael De Volder
Summary: Lithium metal is a promising anode material for lithium-ion batteries due to its high specific capacity and low potential. However, issues such as Li consumption and dendrite growth during cycling have hindered its practical application. In this study, a scalable fabrication method for 3D Cu anodes using one-step electrodeposition is reported, which shows high Coulombic efficiencies and cycling stability.
Article
Chemistry, Physical
Hongri Wan, Xinzhe Ju, Tiantian He, Teng Chen, Yingmei Zhou, Cai Zhang, Jiaomei Wang, Yan Xu, Bing Yao, Wenchang Zhuang, Xihua Du
Summary: The study successfully fabricated S-doped porous carbon from biomass waste and found it to exhibit high capacity and cycling stability in both lithium ion batteries and sodium ion batteries. The unique structure of the new material increases specific surface area and additional active sites, which is significant for enhancing battery performance.
JOURNAL OF ALLOYS AND COMPOUNDS
(2021)
Article
Chemistry, Physical
Yanqing Wang, Chunshun Yuan, Kunming Li, Dong Li, Anqi Ju
Summary: This study successfully prepared freestanding porous silicon@heteroatom-doped porous carbon fiber by designing a porous structure and adopting heteroatom doping strategy. The material exhibits excellent reversible capacity and cycling stability, indicating its potential application in advanced energy storage.
ACS APPLIED ENERGY MATERIALS
(2022)
Article
Chemistry, Physical
He Lin, Nan Lou, Dongdong Yang, Rencheng Jin, Yong Huang
Summary: The study introduced two MoSSe/graphene heterostructures which not only overcame the drawbacks of MoSSe but also integrated the advantages of individual components. Through computations, it was found that the heterostructures exhibited good structural stability, high ion conductivity, and mechanical stiffness, making them potential materials for high-performance LIBs.
JOURNAL OF ALLOYS AND COMPOUNDS
(2021)
Article
Nanoscience & Nanotechnology
Fei Qi, Qiuran Li, Wenxia Zhang, Qiang Huang, Bingyan Song, Yuanfu Chen, Jiarui He
Summary: In this study, a three-dimensional and freestanding ReS2/graphene heterostructure (3DRG) was synthesized for the first time via a one-pot hydrothermal method, which can be directly used as a freestanding and binder-free anode for lithium-ion batteries (LIBs). The 3DRG anode exhibits hierarchically sandwich-like, nanoporous, and conductive three-dimensional network constructed by two-dimensional ReS2/graphene heterostructural nanosheets. With a current density of 100 mA g-1, the 3DRG anode delivers a high reversible specific capacity of 653 mAh g-1. It also shows higher rate capability and cycling stability compared to the bare ReS2 anode.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Chemistry, Physical
Xiaofu Tang, Diping Zeng, Dongrui Chen, Wenmin Guo, Jun Fu, Lihua Zou
Summary: This study develops a rational strategy to trap porous silicon within a stable 3D framework of interconnected N-doped graphene and carbon nanotubes, forming a composite material of PSi@NG/CNT. The PSi@NG/CNT composite exhibits excellent lithium storage properties with high specific capacity, remarkable rate capability, good cycling retention, and high columbic efficiency. This work provides new insights into the rational design of electroactive materials with ultrahigh stability for silicon-based anodes in high energy density lithium-ion batteries.
JOURNAL OF ALLOYS AND COMPOUNDS
(2022)
Article
Engineering, Chemical
Mingjun Sun, Yaohui Qu, Fanyan Zeng, Yong Yang, Keng Xu, Cailei Yuan, Zhang-Hui Lu
Summary: In this study, novel S-doped carbon nanosheets were successfully prepared and utilized as anode materials for Na-ion batteries. These nanosheets exhibited high reversible capacity, high rate performance, and long-term cycling stability. The superior electrochemical properties were attributed to the synergistic effect of S doping, hierarchical pores, and the sandwich-like structure. This research not only provides a high-performance anode material for Na-ion batteries but also offers a new method for preparing S-doped carbon materials for various applications.
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
(2022)
Article
Energy & Fuels
Shengnan Lin, Tingan Zhang
Summary: With the increasing demand for battery performance due to the advancement of mobile and portable electronic devices, anode materials, as an important factor affecting the electrochemical performance of lithium ion storage, have attracted widespread attention. This study provides a creative and effective approach to synthesize four different NiCo-MOFs materials. The electrochemical studies reveal that NiCo-EDTA and NiCo-BI demonstrate slower capacity decrease and excellent cycle performance compared to NiCo-PTA and NiCo-H3BTC.
JOURNAL OF ENERGY STORAGE
(2023)
Article
Biochemistry & Molecular Biology
Chao Jin, Zigang Wang, Chang Luo, Chunling Qin, Yongyan Li, Zhifeng Wang
Summary: In this study, NiFe2O4/NiO composites with a dual-network structure were fabricated using a simple dealloying method. The material, composed of nanosheet networks and ligament-pore networks, provides sufficient space for volume expansion and promotes the rapid transfer of electrons and Li ions. As a result, the material exhibits excellent electrochemical performance, retaining 756.9 mAh g(-1) after 100 cycles at a current density of 200 mA g(-1) and retaining 641.1 mAh g(-1) after 1000 cycles at a current density of 500 mA g(-1).
INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES
(2023)
Article
Chemistry, Physical
Jing Xiao, Junwei Han, Debin Kong, Huifeng Shi, Xiaojuan Du, Ziyun Zhao, Fanqi Chen, Peng Lan, Shichao Wu, Yuefei Zhang, Quan-Hong Yang
Summary: By embedding carbon nanotubes into a graphene hydrogel, a self-adaptable carbon network is built to buffer the volume fluctuations of noncarbon nanoparticles and maintain dynamic electrical connectivity during charging and discharging. This structure enables the noncarbon anode to achieve high volumetric capacities and long cycle life.
ENERGY STORAGE MATERIALS
(2022)
Review
Chemistry, Multidisciplinary
Guanjia Zhu, Dandan Luo, Xiaoyi Chen, Jianping Yang, Haijiao Zhang
Summary: This review surveys the recent advances of emerging multiscale porous anodes for fast charging lithium-ion batteries (LIBs). It clarifies the effects of pore parameters such as porosity, tortuosity, and gradient on fast charging ability from an electrochemical kinetic perspective. The review also presents efforts to implement multiscale porous anodes at both material and electrode levels and evaluates the essential merits and limitations of several quintessential fast charging porous anodes. Additionally, it highlights the challenges and future prospects of multiscale porous fast charging anode design associated with materials and electrodes.
Article
Chemistry, Physical
Xi Qin, Jing Teng, Wenyao Guo, Lei Wang, Shuning Xiao, Qunjie Xu, Yulin Min, Jinchen Fan
Summary: This study demonstrates the improved electrocatalytic activity of NiFe LDH towards OER by applying an external magnetic field. The results show a significant reduction in overpotential and Tafel slope of NiFe LDH under a magnetic field of 200 mT. The magnetic field enhancing effect is likely derived from magnetohydrodynamic effects, charge transfer effects, and alignment of magnetic moments of NiFe LDH.
Review
Chemistry, Multidisciplinary
Chengpeng He, Xiuwen Zhao, Mengjia Huo, Wenrui Dai, Xuejian Cheng, Junhe Yang, Yingchun Miao, Shuning Xiao
Summary: This review summarizes the important role of metal-organic frameworks (MOFs) in the capture and catalytic conversion of industrial exhaust gases. The key points include surface modification, interface promotion, and structure optimization. These findings are valuable for the design and development of MOFs with excellent exhaust gas treatment performance.
Article
Chemistry, Multidisciplinary
Qing Zhang, Enlong Li, Yongshuai Wang, Changsong Gao, Congyong Wang, Lin Li, Dechao Geng, Huipeng Chen, Wei Chen, Wenping Hu
Summary: Researchers have developed an ultralow-power vertical transistor based on transition-metal carbides/nitrides (MXene) and organic single crystal, which exhibits high J(ON) and J(ON)/J(OFF) ratio under ultralow working voltage and can simulate biological synapse functions with extremely low power consumption.
ADVANCED MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Meng Wang, Jie Chen, Zhangliu Tian, Wenrui Dai, Baihua Cui, Xinhang Cui, Dong Wang, Yukun Xiao, Xu Lian, Chonglai Jiang, Haotian Yang, Yihe Wang, Zejun Sun, Yishui Ding, Yi-Yang Sun, Jia Zhang, Wei Chen
Summary: Research reveals that by adjusting the surface structure of WO3 photocathodes, the formation of Li2O2 can be controlled and the photocatalytic reaction activity can be enhanced. Additionally, the (002) facet is found to have higher oxidation ability, resulting in an ultralow polarization overpotential and high discharge capacity over the (002) facet dominated WO3 photocathode.
ENERGY & ENVIRONMENTAL SCIENCE
(2023)
Article
Multidisciplinary Sciences
Zhangliu Tian, Yumin Da, Meng Wang, Xinyu Dou, Xinhang Cui, Jie Chen, Rui Jiang, Shibo Xi, Baihua Cui, Yani Luo, Haotian Yang, Yu Long, Yukun Xiao, Wei Chen
Summary: Photoelectrochemical oxidation provides a promising strategy for glucaric acid production. In this work, selective oxidation of glucose to glucaric acid is realized on the photoanode of defective TiO2 decorated with single-atom Pt via a photoelectrochemical strategy. By optimizing oxygen vacancies, the defective TiO2 photoanode exhibits greatly improved charge separation, significantly enhanced selectivity, and yield of C-6 products.
NATURE COMMUNICATIONS
(2023)
Article
Materials Science, Multidisciplinary
Yumin Da, Zhangliu Tian, Rui Jiang, Yuan Liu, Xu Lian, Shibo Xi, Yi Shi, Yongping Wang, Haotian Lu, Baihua Cui, Jinfeng Zhang, Xiaopeng Han, Wei Chen, Wenbin Hu
Summary: This paper reports the synthesis of a PtNi-NC catalyst with high catalytic activity. Density functional theory calculations reveal that PtNi dual atoms generate a synergistic effect by modulating the local electronic structure and optimizing the charge distribution, contributing to optimized adsorption properties and enhanced electrocatalytic performance. This work provides a new avenue for the fabrication of dual-atom catalysts.
SCIENCE CHINA-MATERIALS
(2023)
Article
Chemistry, Physical
Li Peize, Lian Xu, Gou Jian, Duan Sisheng, Ding Yishui, Niu Yuxiang, Chen Wei
Summary: Realizing effective Ohmic contact to SiC is a major challenge in high-power and high-frequency SiC electronics. Here, we grew a high-work-function interfacial molybdenum trioxide (MoO3) layer on 4H-SiC(0001) and investigated its surface properties during annealing in different gas environments. The results show that the MoO3 layer tends to be reduced and the surface work function decreases accordingly, making it a promising approach for achieving effective Ohmic contact with SiC.
Article
Chemistry, Physical
Yumin Da, Rui Jiang, Zhangliu Tian, Ganwen Chen, Yukun Xiao, Jinfeng Zhang, Shibo Xi, Yida Deng, Wei Chen, Xiaopeng Han, Wenbin Hu
Summary: Alloying platinum with early transition metals is a promising approach to optimize catalyst adsorption behaviors. A strategy combining thermal shock technique with electrochemical activation is reported for the first time to prepare Pt3V alloy as a hydrogen evolution reaction catalyst. The as-prepared catalyst exhibits exceptional catalytic activity and durability, outperforming the state-of-the-art Pt/C catalyst. This work may inspire future research on Pt-based early transition metal alloy catalysts for electrocatalysis.
ADVANCED ENERGY MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Youkun Sun, Suxin Qiu, Ziwei Fang, Junhe Yang, Xueling Song, Shuning Xiao
Summary: The development of efficient photothermal desalination devices is crucial for solving the freshwater shortage problem. Extensive research has been conducted on the design and preparation of efficient photothermal materials with broad light absorption range. However, the performance of photothermal catalysts for purifying complex seawater still faces significant challenges.
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
(2023)
Review
Engineering, Manufacturing
Zhiyang Lyu, Jinlan Wang, Yunfei Chen
Summary: Four-dimensional printing allows for the transformation of 3D-printed architectures over time, which has generated excitement in various research fields. This review summarizes recent developments in 4D printing, focusing on smart materials, structural designs, stimulus designs, and new functionalities for multidisciplinary applications.
INTERNATIONAL JOURNAL OF EXTREME MANUFACTURING
(2023)
Article
Chemistry, Multidisciplinary
Xiang Chen, Xinyue Xu, Yuwen Cheng, He Liu, Dongdong Li, Yumin Da, Yongtao Li, Dongming Liu, Wei Chen
Summary: The study presents a facile strategy to enhance the oxygen evolution reaction (OER) activity of Ni-based materials through doping and interfacial modulation. Experimental and theoretical results demonstrate that this strategy can effectively tune the binding energies of OER intermediates and reduce the energy barrier, leading to significantly improved OER activity.
Article
Chemistry, Physical
Xiangrui Geng, Yishui Ding, Yuan Liu, Xiangyu Hou, Tengyu Jin, Wei Chen
Summary: Achieving effective Ohmic contact between SiC and metal electrodes remains a challenge due to the high Schottky barrier. One promising approach is to introduce a high-work-function interfacial layer. However, the interaction mechanisms between the interfacial layer and the SiC substrate have been rarely studied. In this work, layers of high-work-function MoO3 and Pt were grown on the SiC surface, and the evolutions of the system during annealing under different environments were studied. The results provide a detailed understanding of the Pt/MoO3 interface and its response to various conditions.
Article
Electrochemistry
Yuan Liu, Xu Lian, Xiaojiang Yu, Yuxiang Niu, Jinlin Yang, Yishui Ding, Wei Chen
Summary: This study investigates the interaction processes between alkali metal anodes (AMAs) and organic protective materials containing nitrogen groups. The results show that Li and Na preferentially interact with the outer nitrile groups of the protective material before interacting with the inner imine groups. Additionally, the sodiophilicity difference between the two nitrogen-containing groups is smaller compared to their lithiophilicity difference. These findings provide valuable insights for the development of more effective protective materials in the future.
BATTERIES & SUPERCAPS
(2023)
Article
Chemistry, Physical
Chen Sun, Kunfeng Zhao, Adam Boies, Shuning Xiao, Zhiguo Yi
Summary: A highly active and stable NiO nanocrystalline decorated on ZnO-CoNi solid solution catalyst is reported, which achieves 88% photocatalytic conversion of methane to CO2 and H2O under ambient conditions. The excellent performance of the catalyst originates from the high mobility of surface lattice oxygen of supported NiO nanocrystallines driven by the photogenerated electrons and internal electric field of ZnO-CoNi solid solution. Moreover, even at high methane concentrations up to 5000 ppm, the methane conversion of the catalyst remains above 37%, showing promise for methane elimination applications near large methane emission sources.
APPLIED CATALYSIS B-ENVIRONMENTAL
(2023)
Review
Chemistry, Multidisciplinary
Yumin Da, Rui Jiang, Zhangliu Tian, Xiaopeng Han, Wei Chen, Wenbin Hu
Summary: The development of cost-effective and highly efficient electrocatalysts is crucial for achieving a low-carbon footprint in the industry. Single-atom alloys (SAAs) have unique electronic structures, well-defined active sites, and maximum atom utilization, making them promising replacements for traditional noble metal catalysts. SAAs can tailor the adsorption properties of reaction species to promote electrocatalytic behaviors.
Article
Chemistry, Multidisciplinary
Laetitia Bardet, Herve Roussel, Stefano Saroglia, Masoud Akbari, David Munoz-Rojas, Carmen Jimenez, Aurore Denneulin, Daniel Bellet
Summary: The thermal instability of silver nanowires leads to increased electrical resistance in AgNW networks. Understanding the relationship between structural and electrical properties of AgNW networks is crucial for their integration as transparent electrodes in flexible optoelectronics. In situ X-ray diffraction measurements were used to study the crystallographic evolution of Ag-specific Bragg peaks during thermal ramping, revealing differences in thermal and structural transitions between bare and SnO2-coated AgNW networks.
Article
Chemistry, Multidisciplinary
Nathalia Cancino-Fuentes, Arnau Manasanch, Joana Covelo, Alex Suarez-Perez, Enrique Fernandez, Stratis Matsoukis, Christoph Guger, Xavi Illa, Anton Guimera-Brunet, Maria V. Sanchez-Vives
Summary: This study provides a comprehensive characterization of graphene-based solution-gated field-effect transistors (gSGFETs) for brain recordings, highlighting their potential clinical applications.
Article
Chemistry, Multidisciplinary
Sikandar Aftab, Hailiang Liu, Dhanasekaran Vikraman, Sajjad Hussain, Jungwon Kang, Abdullah A. Al-Kahtani
Summary: This study examines the effects of hybrid nanoparticles made of NiO@rGO and NiO@CNT on the active layers of polymer solar cells and X-ray photodetectors. The findings show that these hybrid nanoparticles can enhance the charge carrier capacities and exciton dissociation properties of the active layers. Among the tested configurations, the NiO@CNT device demonstrates superior performance in converting sunlight into electricity, and achieves the best sensitivity for X-ray detection.
Article
Chemistry, Multidisciplinary
Hyo Jung Shin, Seung Gyu Choi, Fengrui Qu, Min-Hee Yi, Choong-Hyun Lee, Sang Ryong Kim, Hyeong-Geug Kim, Jaewon Beom, Yoonyoung Yi, Do Kyung Kim, Eun-Hye Joe, Hee-Jung Song, Yonghyun Kim, Dong Woon Kim
Summary: This study investigates the role of SOX9 in reactive astrocytes following ischemic brain damage using a PLGA nanoparticle plasmid delivery system. The results demonstrate that PLGA nanoparticles can reduce ischemia-induced neurological deficits and infarct volume, providing a potential opportunity for stroke treatment.
Article
Chemistry, Multidisciplinary
Anurag Chaudhury, Koushik Debnath, Nikhil R. Jana, Jaydeep K. Basu
Summary: The study investigates the interaction between nanoparticles and cell membranes, and identifies key parameters, including charge, crowding, and membrane fluidity, that determine the adsorbed concentration and unbinding transition of nanoparticles.
Article
Chemistry, Multidisciplinary
Sina Sadeghi, Fazel Bateni, Taekhoon Kim, Dae Yong Son, Jeffrey A. Bennett, Negin Orouji, Venkat S. Punati, Christine Stark, Teagan D. Cerra, Rami Awad, Fernando Delgado-Licona, Jinge Xu, Nikolai Mukhin, Hannah Dickerson, Kristofer G. Reyes, Milad Abolhasani
Summary: In this study, an autonomous approach for the development of lead-free metal halide perovskite nanocrystals is presented, which integrates a modular microfluidic platform with machine learning-assisted synthesis modeling. This approach enables rapid and optimized synthesis of copper-based lead-free nanocrystals.
Article
Chemistry, Multidisciplinary
Zahir Abbas, Nissar Hussain, Surender Kumar, Shaikh M. Mobin
Summary: The rational construction of free-standing and flexible electrodes for electrochemical energy storage devices is an emerging research focus. In this study, a redox-active metal-organic framework (MOF) was prepared on carbon nanofibers using an in situ approach, resulting in a flexible electrode with high redox-active behavior and unique properties such as high flexibility and lightweight. The prepared electrode showed excellent cyclic retention and rate capability in supercapacitor applications. Additionally, it could be used as a freestanding electrode in flexible devices at different bending angles.
Article
Chemistry, Multidisciplinary
Lishan Zhang, Xiaoting Zhang, Hui Ran, Ze Chen, Yicheng Ye, Jiamiao Jiang, Ziwei Hu, Miral Azechi, Fei Peng, Hao Tian, Zhili Xu, Yingfeng Tu
Summary: Photodynamic therapy (PDT) is a promising local treatment modality in cancer therapy, but its therapeutic efficacy is restricted by ineffective delivery of photosensitizers and tumor hypoxia. In this study, a phototactic Chlorella-based near-infrared (NIR) driven green affording-oxygen microrobot system was developed for enhanced PDT. The system exhibited desirable phototaxis and continuous oxygen generation, leading to the inhibition of tumor growth in mice. This study demonstrates the potential of using a light-driven green affording-oxygen microrobot to enhance photodynamic therapy.
Article
Chemistry, Multidisciplinary
Yujin Li, Jing Xu, Xinqi Luo, Futing Wang, Zhong Dong, Ke-Jing Huang, Chengjie Hu, Mengyi Hou, Ren Cai
Summary: In this study, hollow heterostructured materials were constructed using an innovative template-engaged method as cathodes for zinc-ion batteries. The materials exhibited fast Zn2+ transport channels, improved electrical conductivity, and controlled volume expansion during cycling. The designed structure allowed for an admirable reversible capacity and high coulombic efficiency.
Article
Chemistry, Multidisciplinary
Paritosh Mahato, Shashi Shekhar, Rahul Yadav, Saptarshi Mukherjee
Summary: This study comprehensively elucidates the role of the core and electrostatic surface of metal nanoclusters in catalytic reduction reactions. The electrostatic surface dramatically modulates the reactivity of metal nanoclusters.
Article
Chemistry, Multidisciplinary
Pei Liu, Mengdi Liang, Zhengwei Liu, Haiyu Long, Han Cheng, Jiahe Su, Zhongbiao Tan, Xuewen He, Min Sun, Xiangqian Li, Shuai He
Summary: This study demonstrates a simple and environmentally-friendly method for the synthesis of zinc oxide nanozymes (ZnO NZs) using wasted hop extract (WHE). The WHE-ZnO NZs exhibit exceptional peroxidase-like activity and serve as effective catalysts for the oxidation of 3,3,5,5-tetramethylbenzidine (TMB) in the presence of hydrogen peroxide (H2O2). In addition, a straightforward colorimetric technique for detecting both H2O2 and glucose was developed using the WHE-ZnO NZs as peroxidase-like catalysts.
Article
Chemistry, Multidisciplinary
Hyunkyu Oh, Young Jun Lee, Eun Ji Kim, Jinseok Park, Hee-Eun Kim, Hyunsoo Lee, Hyunjoo Lee, Bumjoon J. Kim
Summary: Mesoporous carbon particles have unique structural properties that make them suitable as support materials for catalytic applications. This study investigates the impact of channel nanostructures on the catalytic activity of porous carbon particles (PCPs) by fabricating PCPs with controlled channel exposure on the carbon surface. The results show that PCPs with highly open channel nanostructures exhibit significantly higher catalytic activity compared to those with closed channel nanostructures.
Article
Chemistry, Multidisciplinary
Yunjie Lu, Zhaohui Li, Zewei Li, Shihao Zhou, Ning Zhang, Jianming Zhang, Lu Zong
Summary: A tough, long-lasting adhesive and highly conductive nanocomposite hydrogel (PACPH) was fabricated via the synergy of interfacial entanglement and adhesion group densification. PACPH possesses excellent mechanical properties, interfacial adhesion strength, and conductivity, making it a promising material for long-term monitoring of human activities and electrocardiogram signals.
Article
Chemistry, Multidisciplinary
Zichao Wei, Audrey Vandergriff, Chung-Hao Liu, Maham Liaqat, Mu-Ping Nieh, Yu Lei, Jie He
Summary: We have developed a simple method to prepare polymer-grafted plasmonic metal nanoparticles with pH-responsive surface-enhanced Raman scattering. By using pH-responsive polymers as ligands, the aggregation of nanoparticles can be controlled, leading to enhanced SERS. The pH-responsive polymer-grafted nanoparticles show high reproducibility and sensitivity in solution, providing a novel approach for SERS without the need for sample pre-concentration.
Article
Chemistry, Multidisciplinary
Melis Ozge Alas Colak, Ahmet Gungor, Merve Buldu Akturk, Emre Erdem, Rukan Genc
Summary: This research investigates the effect of functionalizing carbon dots with hydroxyl polymers on their performance as electrode materials in a supercapacitor. The results show that the functionalized carbon dots exhibit excellent electrochemical performance and improved stability.