期刊
MOLECULES
卷 21, 期 11, 页码 -出版社
MDPI
DOI: 10.3390/molecules21111467
关键词
nanoparticles; HKUST-1; oxidation; catechol
资金
- National Research Foundation of Korea (NRF) - Ministry of Science, ICT & Future Planning [NRF-2015R1D1A1A02060684, NRF-2013R1A1A2012960]
- GCRC-SOP [2011-0030013]
HKUST-1, a copper-based metal organic framework (MOF), has been investigated as a catalyst in various reactions. However, the HKUST-1 shows low catalytic activity in the oxidation of catechol. Therefore, we synthesized Fe3O4@HKUST-1 by layer-by layer assembly strategy and Cu@Cu2O by reduction of HKUST-1 for enhancement of catalytic activity. Cu@Cu2O nanoparticles exhibited highly effective catalytic activity in oxidation of 3,5-di-tert-butylcatechol. Through this method, MOF can maintain the original core-shell structure and be used in various other reactions with enhanced catalytic activity.
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