期刊
MATERIALS TODAY ENERGY
卷 30, 期 -, 页码 -出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.mtener.2022.101153
关键词
Si; C anodes; Molecular design; Functional groups; Supramolecular structures; 3D cross-linking
资金
- Shenzhen Science and Technology Research Grant
- Soft Science Research Project of Guangdong Province
- [JCYJ20200109140416788]
- [2017B030301013]
This review summarizes recent advances in functional polymers for silicon/carbon composite anode, focusing on the relationship between structural units and binder performance.
Silicon/carbon composite anode that combines high capacity and cycling stability has been successfully commercialized in lithium-ion battery (LIB) industry. Compared with the massive efforts devoted to optimizing the anode material structure or the electrolyte, less attention has been paid to the devel-opment of functional binders and their interaction with silicon/carbon material. As an essential component in the electrode, binders are expected to accommodate the repeated volume change of Si/C anode and maintain the electrode integrity as well as construct efficient electron/ion conductive network. In this review, recent advances in the functional polymers for silicon/carbon composite anode have been summarized from the perspective of intermolecular chemistry. The relationships between representative structure units (i.e. functional groups and chain structures) and performance of binders in Si/C anodes are discussed and we hope provide a fundamental perspective on performance optimization of Si/C anodes.(c) 2022 Elsevier Ltd. All rights reserved.
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