Article
Multidisciplinary Sciences
Matthew Grasinger, Kosar Mozaffari, Pradeep Sharma
Summary: Soft robotics require materials that can undergo large deformations and respond to external stimuli like electric fields. Electroactive soft materials enable applications such as energy harvesting, biomedical devices, flexible electronics, and sensors. Flexoelectricity is an attractive phenomenon where dielectrics develop electric polarization under strain gradients, offering a linear coupling between flexure and electric stimulus. Although the flexoelectric effect is generally weak, combining stretching and bending in elastomers may lead to giant flexoelectricity, as observed in some specific conditions.
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
(2021)
Article
Chemistry, Multidisciplinary
Christopher A. Mizzi, Laurence D. Marks
Summary: This article presents a new flexoelectric model for triboelectricity, where contact deformation at the nanoscale drives charge transfer through band bending. The authors use first-principles and finite element calculations to investigate the implications of charge transfer for different contact geometry and materials combinations. They demonstrate that their ab initio based formulation is compatible with existing empirical models and experimental observations.
Article
Chemistry, Multidisciplinary
Karl P. Olson, Christopher A. Mizzi, Laurence D. Marks
Summary: Triboelectric charge transfer is a complex and important phenomenon whose fundamental mechanism is still not fully understood. Recent research has proposed a model suggesting that flexoelectric band bending due to local asperity contacts is the main driving force for triboelectric charge transfer in non-metals. Experimental analysis of a doped semiconductor sample using a conductive atomic force microscope probe confirms the theoretical model, providing strong evidence for the significant role of flexoelectric band bending in triboelectric contacts.
Article
Biology
Ciara Felix, Davide Folloni, Haoyu Chen, Jerome Sallet, Antoine Jerusalem
Summary: A numerical model was used to investigate the effects of transcranial ultrasound stimulation on white matter electrical activity, revealing a relationship between the degree of alteration in white matter tracts and the connectivity fingerprint of different cortical regions. The results highlight the importance of minimizing spillage on neighboring tracts to maintain functional connectivity with other regions when modulating the target area.
COMPUTERS IN BIOLOGY AND MEDICINE
(2022)
Article
Multidisciplinary Sciences
Gokul Krishna Unnikrishnan, Saurav Sharma, Himanshu Pathak, Vishal Singh Chauhan, Satish Chandra Jain
Summary: To accurately analyze the fracture behavior of piezoceramics at small length scales, flexoelectricity, which is dependent on size, must be considered along with piezoelectricity. The extended isogeometric analysis (XIGA) method, using non-uniform rational B-splines (NURBS) basis functions, is proven to be an accurate and efficient approach for modeling cracks computationally. The implemented XIGA-based computational model in this study investigates the fracture behavior under different flexoelectric coefficients and electrical and mechanical loading combinations, showing a significant reduction in J-integral with an increase in the flexoelectric coefficient.
ADVANCED THEORY AND SIMULATIONS
(2023)
Article
Materials Science, Multidisciplinary
D. Codony, P. Gupta, O. Marco, I. Arias
Summary: This paper develops equilibrium equations describing the flexoelectric effect in soft dielectrics under large deformations. It formulates the model using a flexoelectric tensor defined in the material frame, leading to objective flexoelectric polarization fields. The study also includes a theory of geometrically nonlinear extensible flexoelectric rods and examines cantilever bending and buckling under mechanical and electrical actuation. The numerical implementation of the model proves to be robust in handling electromechanical instabilities in soft flexoelectric materials.
JOURNAL OF THE MECHANICS AND PHYSICS OF SOLIDS
(2021)
Article
Multidisciplinary Sciences
Vishal P. Patil, Harry Tuazon, Emily Kaufman, Tuhin Chakrabortty, David Qin, Jorn Dunkel, M. Saad Bhamla
Summary: Tangled active filaments are common in nature and understanding their collective topological transformations is important. By studying California blackworms, researchers developed a mechanistic model that explains their tangle formation and ultrafast untangling. These findings can provide guidance for designing topologically tunable active materials.
Article
Chemistry, Multidisciplinary
Chullhee Cho, Zhichao Zhang, Jin Myung Kim, Peiwen J. Ma, Md Farhadul Haque, Peter Snapp, SungWoo Nam
Summary: This study reports the formation of a micrometer-scale freestanding wrinkled structure of 2D materials without encapsulation layers, showing enhanced light-matter interactions and spatial modulation. Compared to supported wrinkled structures, the freestanding wrinkled structures exhibit significant enhancement.
Article
Chemistry, Physical
Karl P. Olson, Laurence D. Marks
Summary: This paper investigates the role of contacting shapes in triboelectricity and provides scaling rules for designing energy harvesting devices.
Editorial Material
Nanoscience & Nanotechnology
Charlotte Allard
Summary: An article in Nano Letters introduces a method for transferring metallic nanopatterns onto soft matter such as tissues or single cells.
NATURE REVIEWS MATERIALS
(2023)
Article
Chemistry, Physical
Artemii S. Ivanov, Konstantin G. Nikolaev, Alexander S. Novikov, Stanislav O. Yurchenko, Kostya S. Novoselov, Daria Andreeva, Ekaterina Skorb
Summary: The research focuses on using hydrogels of polyethylenimine and poly(acrylic acid) to form an interface on the surface of gallium-indium eutectic alloy, gradually increasing voltage to create various electronic components. A multilayer perceptron model with one hidden layer and 12 nodes is used to identify hydrogels' composition and automatically set the desired architecture of electronic components. This design allows for easy production of new electronic parts and programmable soft-matter electronics.
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
(2021)
Article
Chemistry, Physical
Elayne M. Thomas, Hongbo Fu, Ryan C. Hayward, Alfred J. Crosby
Summary: Soft materials interfaces can develop complex morphologies during separation due to mechanical instabilities, and a model has been expanded to account for geometry and material properties of two soft materials forming an interface. Experimental validation shows that geometric asymmetry can influence stress in each layer and provide means of controlling interface separations.
Article
Physics, Condensed Matter
Sushil Dubey, Sukh Veer, R. V. Seshagiri Rao, Chirag Kalelkar, Pramod A. Pullarkat
Summary: This article introduces a versatile device for conducting extensional deformation studies of samples at microscopic scales with simultaneous imaging. The operational features of this device are discussed, and several applications are presented.
JOURNAL OF PHYSICS-CONDENSED MATTER
(2021)
Article
Materials Science, Multidisciplinary
Yancheng Meng, Henggao Xiang, Jianqiang Zhang, Jun Yin, Liqiang Li, Zhuhua Zhang, Wanlin Guo
Summary: Compression of soft substrates with stiff membranes leads to wrinkling, and the evolution of wrinkle instability has been extensively studied. A scaling law is obtained, showing that the final instability order of the wrinkle evolution can be determined by a single parameter related to the thickness contrast and material constant. Contrary to common belief, the thickness of the soft substrate plays a dominant role even when the thickness contrast is large. This law is universal and can control the complex behavior of stiff/soft bilayer systems.
Article
Physics, Applied
Liwen Zhu, Renhong Liang, Mao Ye, Longlong Shu, Renkui Zheng, Shanming Ke
Summary: We investigated the thickness-dependent flexoresistance effect in SrTiO3 epitaxial thin films caused by the strain gradient. The strain gradient was induced by using an atomic force microscope diamond-coated tip. The depolarization field caused by the strain gradient changed the film's electrical state, resulting in a significant decrease in resistance. By testing the current-voltage curves of STO films with different thicknesses, we found that the force threshold to trigger the film to enter a highly conductive state increased with film thickness. Only when the film thickness was below 8 nm, the film could transition from an insulating state to a conductive state without damaging the surface. The strain gradient caused by tip loading played a crucial role in modifying the film barrier during the electrical state switching process.
APPLIED PHYSICS LETTERS
(2023)
Article
Materials Science, Multidisciplinary
Kosar Mozaffari, Fatemeh Ahmadpoor, Pradeep Sharma
Summary: At physiological temperatures, biological membranes undergo thermal fluctuations and exhibit entropic repulsive force when approaching each other, influenced by the flexoelectricity phenomenon. This leads to enhanced attraction at close separations and enhanced repulsion at further separations.
MATHEMATICS AND MECHANICS OF SOLIDS
(2021)
Article
Multidisciplinary Sciences
Matthew Grasinger, Kosar Mozaffari, Pradeep Sharma
Summary: Soft robotics require materials that can undergo large deformations and respond to external stimuli like electric fields. Electroactive soft materials enable applications such as energy harvesting, biomedical devices, flexible electronics, and sensors. Flexoelectricity is an attractive phenomenon where dielectrics develop electric polarization under strain gradients, offering a linear coupling between flexure and electric stimulus. Although the flexoelectric effect is generally weak, combining stretching and bending in elastomers may lead to giant flexoelectricity, as observed in some specific conditions.
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
(2021)
Article
Materials Science, Multidisciplinary
Kosar Mozaffari, Liping Liu, Pradeep Sharma
Summary: Solid electrolytes have great potential in rechargeable batteries but suffer from low ionic conductivity. This study proposes a microstructure design to enhance the effective ionic conductivity of composite polymer electrolytes, improving battery performance.
JOURNAL OF THE MECHANICS AND PHYSICS OF SOLIDS
(2022)