期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 81, 期 24, 页码 12401-12407出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.6b02529
关键词
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资金
- SRF for ROCS, SEM [20141685]
- Shandong Natural Science Foundation [ZR2014BQ024, ZR2013BM007]
- Higher Educational Science and Technology Program [J15LA02]
- Qufu Normal University for Research Start-up Foundation [bsqd20130115]
A silver-catalyzed domino reaction of orthocarbonylated alkynyl-substituted arylaldehydes with conjugated dienes is described here. Through this reaction, the synthesis of a variety of indanone-fused cyclohexene derivatives can be achieved efficiently. The formation of these tricyclic products could involve a key Diels Alder reaction of in situ generated indanenone dienophiles with conjugated dienes. Particularly, the products can be accomplished in a high endo/exo selective way.
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