☆ 4.8 Article

Ultra-Stable Zn Anode Enabled by Fiber-Directed Ion Migration Using Mass-Producible Separator

ADVANCED FUNCTIONAL MATERIALS (2023)

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ADVANCED FUNCTIONAL MATERIALS
卷 33, 期 5, 页码 -

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WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.202209301

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aqueous zinc-ion batteries; separators; zincophilicity functional groups; Zn anodes; Zn dendrite growths

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Chemistry, Multidisciplinary Chemistry, Physical Nanoscience & Nanotechnology Materials Science, Multidisciplinary Physics, Applied Physics, Condensed Matter

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Aqueous zinc-ion battery (AZB) is a promising candidate for next-generation energy storage due to its inherent safety and low cost. However, current AZBs face challenges such as Zn dendrite growth and undesirable side-reactions, resulting in poor cycling stability. To address this issue, researchers have developed a unique separator based on polyacrylonitrile/graphene oxide (PG) composite nanofibers, which effectively regulate the migration and distribution of Zn2+ ions in the separator. The PG separator demonstrates high ionic conductivity and stable performance, providing a potential solution to overcome the limitations of Zn metal anode in AZBs.
Aqueous zinc-ion battery (AZB) is a promising candidate for next-generation energy storage owing to inherent safety and low cost. However, AZBs are currently plagued by Zn dendrite growth and undesirable side-reactions, leading to poor cycling stability and premature failure. To restrain the uncontrollable Zn growth, a unique separator is developed based on polyacrylonitrile/graphene oxide (abbreviated as PG) composite nanofibers, which contain abundance of zincophilicity functional groups to regulate the migration and distribution of Zn2+ ions in the separator. It is demonstrated that the cyano ligands on PG not only facilitate the dehydration of solvated Zn2+ ions prior to deposition, but also form fast lanes to enable homogenous scattering of deposition spots. Benefiting from these features, the PG separator offers a high ionic conductivity of 7.69 mS cm(-1) and a transference number of 0.74 for Zn2+. The Zn||Zn symmetrical cells with PG separators achieve an ultra-stable cycle life over 13 000 h. Zn||Zn0.27V2O5 full batteries with PG separators retain 71.5% of the original capacity after 2800 cycles at a high current density of 2 A g(-1). This work offers future research directions toward the design of multifunctional separators to overcome the limits of Zn metal anode in AZBs.

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Goldouzian, M. Hildreth, K. Hurtado Anampa, C. Jessop, K. Lannon, J. Lawrence, N. Loukas, L. Lutton, J. Mariano, N. Marinelli, I. Mcalister, T. McCauley, C. Mcgrady, K. Mohrman, C. Moore, Y. Musienko, R. Ruchti, A. Townsend, M. Wayne, M. Zarucki, L. Zygala, B. Bylsma, L. S. Durkin, B. Francis, C. Hill, M. Nunez Ornelas, K. Wei, B. L. Winer, B. R. Yates, F. M. Addesa, B. Bonham, P. Das, G. Dezoort, P. Elmer, A. Frankenthal, B. Greenberg, N. Haubrich, S. Higginbotham, A. Kalogeropoulos, G. Kopp, S. Kwan, D. Lange, D. Marlow, K. Mei, I. Ojalvo, J. Olsen, D. Stickland, C. Tully, S. Malik, S. Norberg, A. S. Bakshi, V. E. Barnes, R. Chawla, S. Das, L. Gutay, M. Jones, A. W. Jung, D. Kondratyev, A. M. Koshy, M. Liu, G. Negro, N. Neumeister, G. Paspalaki, S. Piperov, A. Purohit, J. F. Schulte, M. Stojanovic, J. Thieman, F. Wang, R. Xiao, W. Xie, J. Dolen, N. Parashar, D. Acosta, A. Baty, T. Carnahan, M. Decaro, S. Dildick, K. M. Ecklund, S. Freed, P. Gardner, F. J. M. Geurts, A. Kumar, W. Li, B. P. Padley, R. Redjimi, J. Rotter, W. Shi, A. G. Stahl Leiton, S. Yang, L. Zhang, Y. Zhang, A. Bodek, P. de Barbaro, R. Demina, J. L. Dulemba, C. Fallon, T. Ferbel, M. Galanti, A. Garcia-Bellido, O. Hindrichs, A. Khukhunaishvili, E. Ranken, R. Taus, G. P. Van Onsem, K. Goulianos, B. Chiarito, J. P. Chou, Y. Gershtein, E. Halkiadakis, A. Hart, M. Heindl, O. Karacheban, I. Laflotte, A. Lath, R. Montalvo, K. Nash, M. Osherson, S. Salur, S. Schnetzer, S. Somalwar, R. Stone, S. A. Thayil, S. Thomas, H. Wang, H. Acharya, A. G. Delannoy, S. Fiorendi, T. Holmes, S. Spanier, O. Bouhali, M. Dalchenko, A. Delgado, R. Eusebi, J. Gilmore, T. Huang, T. Kamon, H. Kim, S. Luo, S. Malhotra, R. Mueller, D. Overton, D. Rathjens, A. Safonov, N. Akchurin, J. Damgov, V. Hegde, K. Lamichhane, S. W. Lee, T. Mengke, S. Muthumuni, T. Peltola, I. Volobouev, Z. Wang, A. Whitbeck, E. Appelt, S. Greene, A. Gurrola, W. Johns, A. Melo, K. Padeken, F. Romeo, P. Sheldon, S. Tuo, J. Velkovska, M. W. Arenton, B. Cardwell, B. Cox, G. Cummings, J. Hakala, R. Hirosky, M. Joyce, A. Ledovskoy, A. Li, C. Neu, C. E. Perez Lara, B. Tannenwald, S. White, N. Poudyal, S. Banerjee, K. Black, T. Bose, S. Dasu, I. De Bruyn, P. Everaerts, C. Galloni, H. He, M. Herndon, A. Herve, U. Hussain, A. Lanaro, A. Loeliger, R. Loveless, J. Madhusudanan Sreekala, A. Mallampalli, A. Mohammadi, D. Pinna, A. Savin, V. Shang, V. Sharma, W. H. Smith, D. Teague, S. Trembath-Reichert, W. Vetens, S. Afanasiev, V. Andreev, Yu. Andreev, T. Aushev, M. Azarkin, A. Babaev, A. Belyaev, V. Blinov, E. Boos, V. Borshch, D. Budkouski, O. Bychkova, V. Chekhovsky, R. Chistov, M. Danilov, A. Dermenev, T. Dimova, I. Dremin, M. Dubinin, L. Dudko, V. Epshteyn, G. Gavrilov, V. Gavrilov, S. Gninenko, V. Golovtcov, N. Golubev, I. Golutvin, I. Gorbunov, A. Gribushin, V. Ivanchenko, Y. Ivanov, V. Kachanov, L. Kardapoltsev, V. Karjavine, A. Karneyeu, V. Kim, M. Kirakosyan, D. Kirpichnikov, M. Kirsanov, V. Klyukhin, O. Kodolova, D. Konstantinov, V. Korenkov, A. Kozyrev, N. Krasnikov, E. Kuznetsova, A. Lanev, A. Litomin, O. Lukina, N. Lychkovskaya, V. Makarenko, A. Malakhov, V. Matveev, V. Murzin, A. Nikitenko, S. Obraztsov, V. Okhotnikov, V. Oreshkin, A. Oskin, I. Ovtin, V. Palichik, P. Parygin, A. Pashenkov, V. Perelygin, S. Petrushanko, G. Pivovarov, S. Polikarpov, V. Popov, O. Radchenko, M. Savina, V. Savrin, V. Shalaev, S. Shmatov, S. Shulha, Y. Skovpen, S. Slabospitskii, I. Smirnov, V. Smirnov, A. Snigirev, D. Sosnov, A. Stepennov, V. Sulimov, E. Tcherniaev, A. Terkulov, O. Teryaev, M. Toms, A. Toropin, L. Uvarov, A. Uzunian, E. Vlasov, S. Volkov, A. Vorobyev, N. Voytishin, B. S. Yuldashev, A. Zarubin, I. Zhizhin, A. Zhokin

Summary: Measurements of Higgs boson production and decay, using different analyses, are presented based on data collected by the CMS experiment. The results provide information about the signal strengths relative to the standard model predictions and the cross sections and branching fractions of the Higgs boson to tau leptons, in multiple kinematic regions.

EUROPEAN PHYSICAL JOURNAL C (2023)

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Article Computer Science, Interdisciplinary Applications

A novel methodology for evaluation of S2 wide split via estimated parameters

Shuping Sun, Wei Song, Yaonan Tong, Xu Li, Man Zhao, Qi Deng, Guangyu Liu, Zhi Liu, Chao Liu

Summary: This study proposes a novel methodology to detect the wide splitting of the second heart sound using an estimated split coefficient of S-2 combined with an adaptive number of S-2. The overall accuracy of this method is 100%, indicating its high precision in diagnosing the wide split of S-2.

COMPUTER METHODS AND PROGRAMS IN BIOMEDICINE (2023)

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Article Chemistry, Physical

Construction of amorphous V2O5@Ti3C2Tx synergistic heterostructure on 3D carbon cloth substrate by a self-assembled strategy towards high-performance aqueous Zn-ion batteries

Weiwei Wang, Rui Huang, Peng He, Ruiting Hu, Ling Ran, Yu Tao, Yani Li, Jun Yan

Summary: This study reports a high capacity and stable cathode material for aqueous Zn-ion batteries, which is synthesized by a synergistic combination of amorphous V2O5@Ti3C2Tx heterostructure and three-dimensional carbon cloth substrate, providing isotropic ion migration channels and rapid electron transfer kinetics.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2024)

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Article Fisheries

Methionine deficiency affects myogenesis and muscle macronutrient metabolism in juvenile turbot Scophthalmus maximus

Zhongmin Sui, Xuan Wang, Yongkai Sun, Huihui Zhou, Chengdong Liu, Kangsen Mai, Gen He

Summary: This study aimed to investigate the effects of dietary methionine availability on muscle growth and macronutrient metabolism in turbot. The results showed that methionine deprivation inhibited fish growth, reduced protein content, and affected the expression of genes related to muscle development. It also impacted the mTOR pathway, autophagy-lysosomal system, and ubiquitin-proteasome system. Furthermore, methionine deficiency influenced amino acid metabolism and energy utilization in muscle. Excess methionine intake did not further modulate metabolism in muscle.

AQUACULTURE (2024)

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Article Geriatrics & Gerontology

The relationship between lifestyles and sarcopenia-related traits: A two-sample Mendelian randomization study

Xiaoting Xia, Shate Xiang, Lijiangshan Hua, Qiuhua Sun, Rongyun Wang

Summary: This study found that smoking may be causally related to a lower risk of low hand grip strength, while alcohol consumption may increase the risk of low hand grip strength. There was no causal relationship between physical activity and sarcopenia-related traits.

ARCHIVES OF GERONTOLOGY AND GERIATRICS (2024)

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Article Radiology, Nuclear Medicine & Medical Imaging

Combined ultrasonography and CT for prognosis and predicting clinical outcomes of patients with pseudomyxoma peritonei

Xuedi Han, Qian Zhang, Nan Zhou, Ruiqing Ma, Jiajun Wang, Xichao Zhai, Bin Cui, Yiyan Lu, Lei Liang

Summary: This study aimed to evaluate the diagnostic accuracy of combined ultrasonography and computed tomography in assessing tumor burden and predicting complete resection in patients with pseudomyxoma peritonei (PMP). The results showed that US-CT PCI had a high accuracy in evaluating moderate tumor burden and could predict incomplete resection. Mesenteric involvement was identified as an independent predictor of incomplete resection.

EUROPEAN RADIOLOGY (2023)

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