期刊
NATURE
卷 609, 期 7925, 页码 46-+出版社
NATURE PORTFOLIO
DOI: 10.1038/s41586-022-05031-2
关键词
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资金
- National Key R&D Program of China [2020YFA0308800, 2017YFA0206301]
- NSF of China [12074009, 11774009, 62174013, 12061131102, 11734003]
- BIT [2021CX11013]
- National Research Foundation, Singapore under its NRF-ISF joint research programme [NRF-CRP22-2019-0007, NRF-CRP22-2019-0004, NRF2020-NRF-ISF004-3520]
- Ministry of Education, Singapore [MOE2018-T3-1-002]
- National Key Basic Research Program of China [2017YFB0701603]
- NSFC [51971037]
- JSPS-KAKENHI [JP16H06333, JP22H05478, 18K14119]
- JST-CREST programme [JPMJCR20B1, JMJCR20B5, JPMJCR1993]
- JSPS A3 Foresight Program
- Kazato Research Encouragement Prize
- Innovation Program of Shanghai Municipal Education Commission [2019-01-07-00-09-E00020]
- Shanghai Municipal Science and Technology Commission [18JC1412800]
- High Magnetic Field Laboratory of Anhui Province
- Strategic Priority Research Program of Chinese Academy of Sciences [XDB30000000]
This study reports an intrinsic heterodimensional superlattice consisting of vanadium disulfide and a vanadium sulfide chain array. The superlattice exhibits unconventional stacking and an unexpected Hall effect due to out-of-plane Berry curvature induced by an in-plane magnetic field.
Superlattices-a periodic stacking of two-dimensional layers of two or more materials-provide a versatile scheme for engineering materials with tailored properties(1,2). Here we report an intrinsic heterodimensional superlattice consisting of alternating layers of two-dimensional vanadium disulfide (VS2) and a one-dimensional vanadium sulfide (VS) chain array, deposited directly by chemical vapour deposition. This unique superlattice features an unconventional 1T stacking with a monoclinic unit cell of VS2/VS layers identified by scanning transmission electron microscopy. An unexpected Hall effect, persisting up to 380 kelvin, is observed when the magnetic field is in-plane, a condition under which the Hall effect usually vanishes. The observation of this effect is supported bytheoretical calculations, and can be attributed to an unconventional anomalous Hall effect owing to an out-of-plane Berry curvature induced by an in-plane magnetic field, which is related to the one-dimensional VS chain. Our work expandsthe conventional understanding of superlattices and will stimulate the synthesis of more extraordinary superstructures.
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