期刊
JOURNAL OF ENVIRONMENTAL SCIENCES
卷 42, 期 -, 页码 227-235出版社
SCIENCE PRESS
DOI: 10.1016/j.jes.2015.07.007
关键词
Elemental sulfur; Flocculation; Optimization; Response surfacemethodology (RSM)
资金
- National High-Tech Research and Development Program (863) of China [2011AA060904]
- National Science Foundation for Distinguished Young Scholars [51225802]
- Science Fund for Creative Research Groups of the National Natural Science Foundation of China [51121062]
- National Key Technology Research and Development Program of the Ministry of Science and Technology of China [2010BAC67B02]
- Fundamental Research Funds for Central Universities [AUGA5710055514]
- National Natural Science Foundation of China [51176037, 51308147, 51408591]
The colloidal properties of biogenic elemental sulfur (S-0) cause solid-liquid separation problems, such as poor settling and membrane fouling. In this study, the separation of S0 from bulk liquids was performed using flocculation. Polyaluminum chloride (PAC), polyacrylamide (PAM) and microbial flocculant (MBF) were compared to investigate their abilities to flocculate S-0 produced during the treatment of sulfate-containing wastewater. A novel approach with response surface methodology (RSM) was employed to evaluate the effects and interactions of flocculant dose, pH and stirring intensity, on the treatment efficiency in terms of the S-0 flocculation and the supernatant turbidity removal. The dose optimization results indicated that the S-0 flocculation efficiency decreased in the following order PAC > MBF > PAM. Optimum S-0 flocculation conditions were observed at pH 4.73, a stirring speed of 129 r/min and a flocculant dose of 2.42 mg PAC/mg S. During optimum flocculation conditions, the S-0 flocculation rate reached 97.53%. Confirmation experiments demonstrated that employing PAC for S-0 flocculation is feasible and RSM is an efficient approach for optimizing the process of S-0 flocculation. The results provide basic parameters and conditions for recovering sulfur during the treatment of sulfate-laden wastewaters. (C) 2015 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.
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