4.6 Article

Construction of Carbon Dot-Modified g-C3N4/BiOIO3 Z-Scheme Heterojunction for Boosting Photocatalytic CO2 Reduction under Full Spectrum Light

期刊

ACS SUSTAINABLE CHEMISTRY & ENGINEERING
卷 10, 期 34, 页码 11143-11153

出版社

AMER CHEMICAL SOC
DOI: 10.1021/acssuschemeng.2c02042

关键词

g-C3N4; CQDs; BiOIO3; photocatalytic performance

资金

  1. National Key R&D Program of China [2018YFB0605002]
  2. National Natural Science Foundation of China [21546014]

向作者/读者索取更多资源

In this study, a Z-scheme BiOIO3/CQDs/g-C3N4 composite modified with carbon quantum dots (CQDs) was successfully constructed for photocatalytic CO2 reduction. The experimental results demonstrated that the composite exhibited efficient photocatalytic activity.
In this study, we successfully constructed a Z-scheme BiOIO3/CQDs/g-C3N4 (BCCN) composite modified with carbon quantum dots (CQDs) for photocatalytic CO2 reduction. A series of characterization approaches and testing technologies were carried out to investigate the components, morphologies, and optical properties of the fabricated photo-catalysts. The 0.015B0.01CCN displayed an efficient photo-catalytic CO2 reduction activity within 7 h full spectrum light irradiation, producing CO with a rate of 117.88 smol gcat-1. The enhanced photocatalytic (2)(CO) reduction of the BCCN composite can be attributed to the synergistic effects of CQDs and the Z-scheme heterojunction. This work presents a new insight into integrating CQDs with g-C3N4 and BiOIO3 for the positive synergetic effect to obtain a high-efficient photocatalyst.

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