期刊
ACS APPLIED MATERIALS & INTERFACES
卷 14, 期 27, 页码 31343-31353出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.2c08434
关键词
quartz crystal microbalance; humidity sensor; guar gum; ethyl cellulose; electrospinning; emotional breathing
资金
- National Natural Science Foundation of China [51777215]
In this study, a quartz crystal microbalance (QCM) sensor was fabricated using guar gum (GG) and electro-spun ethyl cellulose-polyvinyl pyrrolidone (EC-PVP) nanofibers as humidity-sensitive materials. The GG/EC-PVP-coated QCM sensor exhibited high sensitivity, low hysteresis, excellent selectivity, good repeatability, and stability in a wide range of relative humidity. The sensor's hydrophilic groups and porous structure contributed to its enhanced humidity sensitivity. The GG/EC-PVP sensor could capture and measure typical breathing patterns in different human emotions, and could also be used for lie detection.
In this work, the guar gum (GG) and the electro-spinned ethyl cellulose-polyvinyl pyrrolidone (EC-PVP) nanofibers were used as humidity-sensitive materials for fabricating a quartz crystal microbalance (QCM) sensor. Fourier transform infrared spectroscopy, scanning electron microscopy, water contact angle test, and X-ray photoelectron spectra were used to characterize the synthesized GG/EC-PVP composite material, confirming its successful preparation and good hydrophilicity. The humidity sensitivity experiments were performed at room temperature. The GG/EC-PVP-coated QCM sensor has high sensitivity (55.72 Hz/% RH) and low hysteresis (2.8% RH) in a wide relative humidity range (0-97% RH), short response/recovery time (26/2 s), excellent selectivity, good repeatability, and stability. The combined action of hydrophilic groups and porous structure enhances the humidity sensitivity. The GG/EC-PVP sensor can be used to capture and measure typical breathing patterns in different human basic emotions due to its good performance. Furthermore, a lie-detector system was also designed for judging the lying through detecting the emotional breathing pattern of the subjects.
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