期刊
SMALL
卷 18, 期 19, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/smll.202201039
关键词
air suction effect; elasticity; high-temperature resistance; silicon carbide aerogels; super thermal insulation
类别
资金
- Natural Science Foundation of Anhui Province [2108085J28]
- Major Science and Technology Projects of Anhui Province [202103a05020011]
- National Natural Science Foundation of China [52074253]
- Youth Innovation Promotion Association CAS [CX2320007001]
- University Synergy Innovation Program of Anhui Province [GXXT-2019-027]
In this study, an air suction effect induction strategy was proposed to fabricate a super thermally insulating SiC aerogel with a directional lamellar structure. The STISA showed significant improvements in compression and elasticity performance, as well as an ultralow thermal conductivity. This research paves the way for structural design of advanced ceramic aerogels for super thermal insulation.
Silicon carbide (SiC) aerogels are promising thermal insulators that are lightweight and possess high thermal stability. However, their application is hindered by their brittleness. Herein, an air suction effect induction (ASEI) strategy is proposed to fabricate a super thermally insulating SiC aerogel (STISA). The ASEI strategy exploits the air suction effect to subtly regulate the directional flow of the SiO gas, which can induce directional growth and assembly of SiC nanowires to form a directional lamellar structure. The sintering time is significantly reduced by >90%. Significant improvements in the compression and elasticity performance of the STISA are achieved upon the formation of a directional lamellar structure through the ASEI strategy. Moreover, the lamellar structure endows the STISA with an ultralow thermal conductivity of 0.019 W m(-1) K-1. The ASEI strategy paves the way for structural design of advanced ceramic aerogels for super thermal insulation.
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