4.7 Article

Experimental study on the treatment of oil-based drill cutting by pulsed dielectric barrier discharge plasma at atmospheric pressure

期刊

JOURNAL OF CLEANER PRODUCTION
卷 339, 期 -, 页码 -

出版社

ELSEVIER SCI LTD
DOI: 10.1016/j.jclepro.2022.130757

关键词

Dielectric barrier discharge; Oil-based drilling cutting; Low temperature plasma; Plasma treatment; Active Al2O3 ball

资金

  1. National Natural Science Foundation of China [52022096]
  2. Royal Society -Newton Advanced Fellowship, UK
  3. NAF [\R2\192117]

向作者/读者索取更多资源

In this study, low-temperature plasma technology was used to treat oil-based drilling cuttings, and the effect of adding active Al2O3 balls on the degradation rate of mineral oil was evaluated. The results demonstrated that the addition of active Al2O3 balls significantly increased the degradation rate of mineral oil. This study provides important insights into the treatment of oil-based drilling cuttings.
Oil-based drilling cuttings produced in the process of oil exploration and shale gas development are harmful to the ecological environment. The emerging low-temperature plasma technology has shown potential for environmental protection. In this paper, pulsed dielectric barrier discharge (DBD) plasma was used to treat contaminated drilling cuttings at atmospheric pressure. The effect of adding active aluminium oxide (Al2O3) balls to the oil-based cuttings on the degradation rate of mineral oil was evaluated. Results showed that when the oilbased drilling cuttings were mixed with active Al2O3 balls, the highest degradation rate of mineral oil (68.1%) was achieved when the treatment time was 30 min. This rate was 41.8% higher than that obtained by DBD treatment alone. The Fourier transform infrared spectroscopy showed that the content of alkanes in the treated samples decreased significantly. The gas chromatography-mass spectrometry and ion chromatography analysis showed that formic acid, acetic acid, and other by-products were formed. The contents of C and H in the samples treated by DBD decreased. Overall, this study provides much-needed insights into the reaction mechanism and pollutant degradation process of the synergistic treatment system of pulsed DBD and active Al2O3 balls in the field of oil-based drilling cuttings treatment.

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