期刊
ACS APPLIED ENERGY MATERIALS
卷 4, 期 11, 页码 12007-12031出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsaem.1c02548
关键词
PEC water splitting; electrocatalysts; energy conversion; surface passivation; defect engineering; heterojunction constructions
资金
- Ministry of Science and Technology of China [2018YFA0702100]
- National Natural Science Foundation of China [11874169, 51972129]
- National Key R&D Program of China [2017YFE0120500]
- Key Research and Development Program of Hubei [2020BAB079]
- South Xinjiang Innovation and Development Program of Key Industries of Xinjiang Production and Construction Corps [2020DB002]
- Saudi Aramco Chair Program [ORCP2390]
This review provides a detailed explanation of the basic mechanism of PEC water splitting using electrocatalysts, and highlights recent advancements in the design, fabrication, and modification of high-efficiency electrocatalysts for energy conversion.
Photoelectrochemical (PEC) water splitting offers a sparkling and sustainable strategy for hydrogen generation, and significant research for enhancing the conversion efficiency of electrocatalysts is underway, since a huge number of publications have been reported in this field. Hence, it is urgent to write a comprehensive and updated review in order to highlight the latest progress in the design, fabrication, and modification of electrocatalysts for high-efficiency PEC water splitting. In this review, we describe the basic mechanism of PEC water splitting utilizing electrocatalysts in detail. Further, we highlighted the recent advancements in the design, fabrication, and modification of high-efficiency electrocatalysts for energy conversion. In addition, the catalysts' surface passivation, heterojunction constructions, defect engineering, and photovoltage and photocurrent enhancements are also highlighted.
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