期刊
ADVANCED MATERIALS INTERFACES
卷 9, 期 8, 页码 -出版社
WILEY
DOI: 10.1002/admi.202101773
关键词
advanced electrolytes; interface models; liquid electrolytes; Na-ion batteries; solid electrolyte interphase; transport properties; X-ray photoelectron spectroscopy
资金
- Ministerio de Ciencia, Innovacion y Universidades [PID2019-107468RB-C21]
- Gobierno Vasco/Eusko Jaurlaritza [IT1226-19]
- Helmholtz Association
This article presents the research progress on the electrode-electrolyte interphase in rechargeable lithium-ion battery technology and sodium-ion technology, emphasizing the importance of establishing a stable interface and the factors that affect it.
Rechargeable Li-ion battery technology has progressed due to the development of a suitable combination of electroactive materials, binders, electrolytes, additives, and electrochemical cycling protocols that resulted in the formation of a stable electrode-electrolyte interphase. It is expected that Na-ion technology will attain a position comparable to Li-ion batteries dependent on advancements in establishing a stable electrode-electrolyte interphase. However, Li and Na are both alkali metals with similar characteristics, yet the physicochemical properties of these systems differ. For this reason, a detailed study on the electrode-electrolyte interphase properties, composition, and structure is required to understand the factors that influence the battery's behavior. Herein, the research that has been performed on the electrode-electrolyte interphase for both anode and cathode in the most important families of electrode materials, including carbonate ester-based and advanced electrolytes such as ether-based carbonates and ionic liquids is presented.
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