4.8 Article

Scaling of the strange-metal scattering in unconventional superconductors

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NATURE
卷 602, 期 7897, 页码 431-+

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NATURE PORTFOLIO
DOI: 10.1038/s41586-021-04305-5

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资金

  1. National Key Basic Research Program of China [2017YFA0302900, 2017YFA0303003, 2018YFB0704102]
  2. National Natural Science Foundation of China [11888101, 11927808, 11834016, 11961141008]
  3. Beijing Natural Science Foundation [Z190008]
  4. Chinese Academy of Sciences [XDB25000000, XDB33000000]
  5. CAS Interdisciplinary Innovation Team
  6. Key-Area Research and Development Program of Guangdong Province [2020B0101340002]
  7. NIST grant [60NANB19D027]
  8. US Department of Energy Office of Science User Facility [DE-AC02-05CH11231]
  9. [AFOSR FA9550-14-10332]
  10. [AFOSR FA9550-22-10023]
  11. [ONR N00014-13-1-0635]
  12. [ONR N00014-15-2-222]

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The research uncovers the precise quantitative scaling laws among the superconducting transition temperature, the linear-in-T scattering coefficient, and the doping level in electron-doped copper oxide La2-xCexCuO4, suggesting a common mechanism of the strange-metal behavior and unconventional superconductivity in these systems.
Marked evolution of properties with minute changes in the doping level is a hallmark of the complex chemistry that governs copper oxide superconductivity as manifested in the celebrated superconducting domes and quantum criticality taking place at precise compositions(1-4). The strange-metal state, in which the resistivity varies linearly with temperature, has emerged as a central feature in the normal state of copper oxide superconductors(5-9). The ubiquity of this behaviour signals an intimate link between the scattering mechanism and superconductivity(10-12). However, a clear quantitative picture of the correlation has been lacking. Here we report the observation of precise quantitative scaling laws among the superconducting transition temperature (T-c), the linear-in-T scattering coefficient (A(1)) and the doping level (x) in electron-doped copper oxide La2-xCexCuO4 (LCCO). High-resolution characterization of epitaxial composition-spread films, which encompass the entire overdoped range of LCCO, has enabled us to systematically map its structural and transport properties with unprecedented accuracy and with increments of Delta x = 0.0015. We have uncovered the relations T-c similar to (x(c) - x)(0.5) similar to (A(1)(rectangle))(0.5), where x(c) is the critical doping in which superconductivity disappears and A(1)(rectangle) is the coefficient of the linear resistivity per CuO2 plane. The striking similarity of the T-c versus A(1)(rectangle) relation among copper oxides, iron-based and organic superconductors may be an indication of a common mechanism of the strange-metal behaviour and unconventional superconductivity in these systems.

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