Article
Chemistry, Physical
Shouchun Ma, Yang Yang, Jiaqi Li, Yuqing Mei, Yufeng Zhu, Jie Wu, Li Liu, Tongjie Yao, Qingfeng Yang
Summary: By constructing a Z-scheme Fe-2(MoO4)(3)/Ag/Ag3PO4 heterojunction, the issues of photocorrosion and quenching effect by in-situ generated H2O2 in Ag3PO4-based photocatalysts have been addressed, leading to improved degradation rate and stability.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2022)
Article
Chemistry, Physical
Shufan Feng, Yan-Ping Zhang, Huihui Xu, Xue-qing Gong, Jianli Hua
Summary: Developing PDI-based photocatalysts with different substitutes, the Se-HPDI/g-C3N4 heterojunction showed the highest H2O2 production rate of 224.27 μM h-1 under visible light, which is 10.1 times higher than bare g-C3N4. The enhancement is attributed to the disparity of electron distribution between different constituent layers in heterojunctions, facilitated by the introduction of substitutes at the bay position. Additionally, the load of PDIs broadens the optical absorption range of g-C3N4 and suppresses H2O2 decomposition. This work provides inspiration for the further design of PDI-based photocatalysts.
JOURNAL OF ALLOYS AND COMPOUNDS
(2023)
Article
Engineering, Environmental
Rujin Li, Ming Zheng, Xin Zhou, Dan Zhang, Yan Shi, Chunxiang Li, Min Yang
Summary: In this paper, porous g-C3N4 nanosheets with carbon vacancies (Cv-PCNNS) were developed for efficient metronidazole degradation via the photocatalysis-self-Fenton system. The carbon vacancies in the Cv-PCNNS accelerated photo-induced charge separation and improved O2 activation. The Cv-PCNNS also provided H for photocatalytic O2 reduction to H2O2 and captured H from the surroundings to restore their original appearance. The introduction of carbon vacancies increased the H2O2 production rate and enhanced the metronidazole degradation efficiency.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Chemistry, Physical
Chuan Wang, Kai Wang, Xinxia He, Yang Liao, Hui Mao, Shilin Zhao, Jun Ma
Summary: This study explores the enhancement of H2O2 photocatalytic yield by constructing an internal electronic field (IEF) in P doped g-C3N4 framework, with the intensity of IEF adjustable through different doping amounts. The optimal photocatalyst PDCN-10 exhibits significantly higher IEF intensity and H2O2 yield.
Article
Chemistry, Physical
Yufeng Zhu, Shouchun Ma, Yang Yang, Jiaqi Li, Yuqing Mei, Li Liu, Tongjie Yao, Jie Wu
Summary: The study established a Z-scheme electron transfer pathway by preparing Fe2(MoO4)3/MoO3 heterojunction, and achieved a synergistic effect between heterogeneous Fenton reaction and photocatalytic reaction by utilizing H2O2 as a medium, leading to enhanced degradation efficiency.
JOURNAL OF ALLOYS AND COMPOUNDS
(2021)
Article
Engineering, Environmental
Xin Zhang, Fenyang Tian, Xiao Lan, Yequn Liu, Weiwei Yang, Jie Zhang, Yongsheng Yu
Summary: The research presents a novel method of synthesizing phosphorus-doped MoS2/g-C3N4 layered composite for enhanced photocatalytic efficiency. The composite shows high photocatalytic sterilization efficiency and offers a promising material for effective photocatalytic sterilization.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Chemistry, Physical
Yina Guan, Siwei Zhao, Jiaqi Li, Xianhe Deng, Shouchun Ma, Yanqiu Zhang, Baojiang Jiang, Tongjie Yao, Baifu Xin, Jiaxu Zhang, Jie Wu
Summary: The Photo-Fenton reaction combining the photocatalytic reaction and Fenton reaction showed excellent degradation performance. Fe-C3N4/Ti3C2/C-TiO2 catalyst exhibited high photothermal effect, enhanced H2O2 activation, and at least 4.2 times higher degradation rate compared to reference catalysts.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2022)
Article
Chemistry, Inorganic & Nuclear
Zhang Hui, Cheng Li-Qing, Hu Ming-Yue, Li Ming-Yu, Zheng Jian-Fei, Xin Si-Tian, Fang Cai-Hong, Chen Heng, Yang Yi-Qiong, Nie Long-Hui
Summary: The fabrication of BiOBr/g-C3N4 S-scheme heterojunction is an effective way to improve photocatalytic activity. This study investigated the photo-self-Fenton catalytic activity of the BiOBr/g-C3N4 S-scheme heterojunction without H2O2 for the first time. The results showed that Fe3+ addition greatly enhanced the photocatalytic and photo-self-Fenton catalytic degradation of rhodamine B (RhB) over the BiOBr/g-C3N4 S-scheme heterojunction.
CHINESE JOURNAL OF INORGANIC CHEMISTRY
(2023)
Article
Green & Sustainable Science & Technology
Xidong Zhang, Jiaguo Yu, Wojciech Macyk, S. Wageh, Ahmed A. Al-Ghamdi, Linxi Wang
Summary: In this study, a step-scheme heterojunction photocatalyst C3N4/PDA (CNP) was constructed, which showed improved H2O2 production rate compared to most reported photocatalysts.
ADVANCED SUSTAINABLE SYSTEMS
(2023)
Article
Engineering, Environmental
Jiaoni Li, Jinhui Huang, Guangming Zeng, Chenyu Zhang, Hanbo Yu, Qiongfang Wan, Kaixin Yi, Wei Zhang, Haoliang Pang, Si Liu, Suzhou Li, Wenjuan He
Summary: Efficient visible-light-driven H2O2 production and antibiotic degradation are achieved using nitrogen-deficient modified polymeric carbon nitride (g-C3N4) as a catalyst. The N defects in the framework construct a giant internal electric field (IEF), inhibiting carrier recombination and promoting selective 2-oxygen reduction reaction (ORR). This study reveals the synergistic effects of the terminal cyano group and nitrogen vacancies over g-C3N4 for efficient H2O2 photogeneration photosynthesis.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Environmental Sciences
Yufei Du, Rui Ma, Lingzhen Wang, Jin Qian, Qilin Wang
Summary: The performance of the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) were enhanced by synthesizing the BiOI/graphitic carbon nitride nanotubes (g-C3N4 nanotubes) heterojunction. The stable heterojunction prevented rapid recombination between photoexcited electrons and holes, resulting in optimized electronic transmission pathway and faster surface reaction rates. Additionally, the composite exhibited outstanding OER and HER activities under illuminated conditions.
SCIENCE OF THE TOTAL ENVIRONMENT
(2022)
Article
Nanoscience & Nanotechnology
Lijun Yang, Ao Zhang, Lei Zhang
Summary: Researchers have designed a novel two-dimensional/three-dimensional hierarchical CuS@MnS photocatalyst for the synthesis of H2O2 through regulating crystal structure, morphology, and photocharge transfer mechanism. By coupling with Sn3O4/Ni foam, the prepared two-compartment cell exhibited boosted activity and stability for the dual production of H2O2. Additionally, a direct hydrazine/O2 fuel cell was used to construct an energy-saving H2O2 generation system, significantly reducing electricity consumption.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Chemistry, Physical
Lan Ding, Yaoyao Tang, Siyang Wang, Yuqi Zhang, Xinyi Chen, Hongjun Zhou
Summary: A novel 0D/2D heterojunction consisting of bimetallic Mo2Ti2C3 MXene Quantum Dots (Mo2Ti2C3 QDs) immobilized on g-C3N4 nanosheets was successfully constructed. The resulting Mo2Ti2C3 QDs/g-C3N4 exhibited highly efficient and stable photocatalytic hydrogen production, with a performance 7.96 times higher than pure g-C3N4 nanosheets. The significant improvement was attributed to the formation of a giant interfacial electric field, facilitating the separation and transfer of photo-generated carriers.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Xianhe Deng, Yang Yang, Yuqing Mei, Jiaqi Li, Changliang Guo, Tongjie Yao, Yongmei Guo, Baifu Xin, Jie Wu
Summary: The sandwich-like Fe3O4@FeS2@C@MoS2 composite was prepared by coating MoS2 shell on the surface of core/shell Fe3O4@C composite. It exhibited a higher degradation efficiency in photo-Fenton reaction and maintained good cycling stability. The study revealed the contribution order of radicals and the impact of the built-in electric field on charge transfer.
JOURNAL OF ALLOYS AND COMPOUNDS
(2022)
Article
Chemistry, Physical
Junpeng Yue, Hanpei Yang, Chen Liu, Qiang Zhang, Yanhui Ao
Summary: A new strategy for efficiently removing organics from water through photo-self-Fenton was investigated. It was found that a novel twin carbon nitride with abundant surficial N defects and compressed n-n layer stacking could be created by thermal polymerization of urea under suitable basicity. The twins exhibited a high in-situ H2O2 production rate at 420 nm and significantly higher mineralization rates for various organic compounds compared to pristine C3N4.
APPLIED CATALYSIS B-ENVIRONMENTAL
(2023)
Article
Chemistry, Multidisciplinary
Hongli Wang, Jianan Liu, Xudong Xiao, Huiyuan Meng, Jie Wu, Chuanyu Guo, Mang Zheng, Xiaolei Wang, Shien Guo, Baojiang Jiang
Summary: In this work, a compact and stable photocatalyst (SnO2/TiO2 heterostructure) with abundant oxygen vacancies was prepared. The heterojunction system provides active sites for catalytic reactions and promotes the separation and migration of photogenerated carriers. The hydrogen production rate of SnO2/TiO2 is significantly higher than that of TiO2 due to its good dynamical properties.
CHINESE CHEMICAL LETTERS
(2023)
Article
Materials Science, Multidisciplinary
Mang Zheng, Qi Li, Mingyang Liu, Jianan Liu, Chen Zhao, Xudong Xiao, Hongli Wang, Jing Zhou, Liping Zhang, Baojiang Jiang
Summary: In this study, Mo-doped In2O3 was synthesized with a porous rod-shaped structure, achieving high conversion rate and selectivity under visible-light irradiation. Mo doping introduced defect states and enhanced the separation of photogenerated electron-hole pairs, while Mo atoms on the surface enhanced reaction rate by forming extra adsorption and reaction centers. This work provides insights into transition metal-doped semiconductor photocatalysts for amino acid production.
SCIENCE CHINA-MATERIALS
(2022)
Article
Nanoscience & Nanotechnology
Jianan Liu, Xuemeng Sun, Baojiang Jiang, Mingyang Liu, Qi Li, Xudong Xiao, Hongli Wang, Mang Zheng, Shien Guo, Jie Wu, Yanhong Zhang, Keying Shi, Wei Zhou
Summary: In this study, ZnFe2O4/UiO-66-NH2 composites were fabricated via an electrostatic self-assembly process for photocatalytic selective oxidation of alcohols. The optimized composite exhibited excellent photocatalytic activity and stability, providing a strategy for optimizing nanoscale catalysts under mild conditions.
ACS APPLIED NANO MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Xudong Xiao, Zhoushilin Ruan, Qi Li, Liping Zhang, Huiyuan Meng, Qun Zhang, Hongliang Bao, Baojiang Jiang, Jing Zhou, Chuanyu Guo, Xiaolei Wang, Honggang Fu
Summary: This study demonstrates a new method utilizing individual iron atoms on polymeric carbon nitride to activate superoxide anions for promoting the oxidation reaction of ethylbenzene, resulting in high conversion rate and selectivity.
ADVANCED MATERIALS
(2022)
Article
Chemistry, Physical
Yuqing Mei, Yanqiu Zhang, Jiaqi Li, Xianhe Deng, Yang Yang, Qingfeng Yang, Baojiang Jiang, Baifu Xin, Tongjie Yao, Jie Wu
Summary: In this study, a Co-doped CeO2 nanoflower catalyst with high adsorption capacity and degradation efficiency was prepared for Fenton-like reaction. The nanoflower structure had a hierarchical porous structure, and Co doping increased the number of Ce(III) sites and defects, resulting in an enhanced maximum adsorption capacity. The high activity of Co towards the activation of PMS significantly improved the degradation rate. Additionally, the catalyst exhibited high efficiency in the degradation of various organic pollutants and demonstrated excellent reusability after multiple cycles.
JOURNAL OF ALLOYS AND COMPOUNDS
(2022)
Article
Chemistry, Physical
Shuai Wang, Changhao Yao, Yifeng Cai, Yang Yang, Huiyuan Ma, Baojiang Jiang, Jun Ma
Summary: In this study, alpha-Fe2O3/rGO was synthesized using a one-step method and used to activate persulfate for the degradation of Bisphenol A under sunlight. The results showed that the introduction of alpha-Fe2O3/rGO and persulfate significantly enhanced the photocatalytic efficiency, resulting in a degradation rate of 99.1%. Electron spin resonance spectroscopy and trapping experiments identified ·OH and ·SO42- as the principal oxidative species in the reaction system.
JOURNAL OF ALLOYS AND COMPOUNDS
(2022)
Article
Chemistry, Physical
Changliang Guo, Baogang Wu, Sheng Ye, Jianan Liu, Xianhe Deng, Laiyu Luo, Qi Li, Xudong Xiao, Junxia Wang, Jian Liu, Tian Xia, Baojiang Jiang
Summary: In this study, a high-efficiency photoreduction catalyst was successfully synthesized by in-situ growing a layer of flaky nickel chromium layered double hydroxides nanosheets on carbon nitride hexagonal tube. The resulting tube-flakes heterostructure showed significantly enhanced hydrogen evolution efficiency.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2022)
Article
Chemistry, Physical
Chen Zhao, Chunjing Shi, Qi Li, Xinyao Wang, Guang Zeng, Sheng Ye, Baojiang Jiang, Jian Liu
Summary: By utilizing supramolecular self-assembly, connection, and calcination treatment, we successfully prepared porous carbon nitride nanosheets with nitrogen vacancies, which exhibited excellent activity and selectivity in photocatalytic H2O2 generation.
MATERIALS TODAY ENERGY
(2022)
Article
Engineering, Environmental
Yanqiu Zhang, Yuqing Mei, Shouchun Ma, Yang Yang, Xianhe Deng, Yina Guan, Tingting Zhao, Baojiang Jiang, Tongjie Yao, Qingfeng Yang, Jie Wu
Summary: This study presents the preparation of a non-typical yolk/shell nanoreactor (ZIF-67 @Co2SiO4/SiO2) with outstanding catalytic activity and recyclability. The nanoreactor exposes more active sites and provides better protection, and the inner shell structure extends the travel path and retention time of pollutants.
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Article
Engineering, Environmental
Bingke Zhang, Dongbo Wang, Shujie Jiao, Zhikun Xu, Yaxin Liu, Chenchen Zhao, Jingwen Pan, Donghao Liu, Gang Liu, Baojiang Jiang, Yongfeng Li, Liancheng Zhao, Jinzhong Wang
Summary: In this study, a hierarchical S-scheme photocatalyst composite was prepared, which achieved efficient hydrogen production through an optimized heterostructure.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Chemistry, Physical
Shuai Wang, Xin Du, Changhao Yao, Yifeng Cai, Huiyuan Ma, Baojiang Jiang, Jun Ma
Summary: Designing photocatalysts with high light utilization and efficient photogenerated carrier separation is crucial for pollutant degradation. In this study, a hierarchical core shell material alpha-Fe2O3@ZnIn2S4 with a tandem heterojunction mechanism and MXene Ti3C2 quantum dots (QDs) was synthesized. The alpha-Fe2O3@ZnIn2S4/Ti3C2 QDs exhibited significantly higher photodegradation efficiency compared to pure alpha-Fe2O3. The enhanced photocatalytic activity was attributed to the S-scheme heterojunction and Schottky junction tandem, which facilitated charge separation. This study provides a new approach for the construction of tandem double heterojunctions for pollutant degradation.
Article
Materials Science, Multidisciplinary
Junxia Wang, Changliang Guo, Yong Jiang, Jiafeng Wan, Bing Zheng, Yuxin Li, Baojiang Jiang
Summary: This study has developed an efficient and environmentally friendly strategy for H2O2 production and improved photocatalytic activity through the formation of a heterojunction. This method has scientific and practical value for environmental remediation.
SCIENCE CHINA-MATERIALS
(2023)
Article
Chemistry, Physical
Changhao Yao, Zihui Wang, Zhi Xu, Baojiang Jiang, Yang Yang, Shuai Wang
Summary: The coupling of photocatalytic process with persulfate activation can release active groups synergistically, showing great potential in environmental remediation. This study designs a 2D/2D alpha-Fe2O3/single-layer MXene Ti3C2/Peroxymonosulfate (PMS) Schottky-scheme photocatalytic-PMS activation coupled system with bidirectional strengthening properties. This system exhibits excellent pollutant degradation activity with ultra-high apparent rate constant, and it is proven that the active group with the highest contribution is 1O2 originated from the preferential reaction between photogenerated holes and PMS. This work provides a suitable direction for designing coupled systems for environmental remediation using sustainable energy sources.
JOURNAL OF ALLOYS AND COMPOUNDS
(2023)
Article
Chemistry, Multidisciplinary
Longjiang Sun, Dongxu Wang, Yuxin Li, Baogang Wu, Qi Li, Cheng Wang, Shuao Wang, Baojiang Jiang
Summary: Developing efficient photocatalysts for selective oxidation of benzene to phenol is challenging. In this study, a CuO@CN photocatalyst was fabricated by loading tubular carbon nitride with CuO nanoparticles thermally polymerized from Cu-based MOFs. The fabricated nanocomposite demonstrated 99.9% benzene photoconversion and 99.1% phenol selectivity under AM 1.5 illumination for 12 h. The excellent stability and sluggish photocharge carrier recombination rate indicate that this nanocomposite is an ideal photocatalyst for benzene oxidation.
CHINESE CHEMICAL LETTERS
(2023)
Article
Chemistry, Physical
Shuai Wang, Xin Du, Changhao Yao, Yifeng Cai, Huiyuan Ma, Baojiang Jiang, Jun Ma
Summary: This study presents a new approach for designing photocatalysts with high efficiency in pollutant degradation. A hierarchical core shell material and MXene Ti3C2 quantum dots were used to construct a double-heterojunction tandem mechanism, leading to enhanced charge separation and improved degradation performance.
Article
Chemistry, Physical
Panpan Zhang, Xu Wang, Yangyang Yang, Haifeng Yang, Chunsheng Lu, Mingru Su, Yu Zhou, Aichun Dou, Xiaowei Li, Xiaochuan Hou, Yunjian Liu
Summary: In this study, the influence of transition metal doping on the electronic and mechanical properties and electrochemical performance of 2HMoS2/NC was investigated using Cobalt (Co) as an example. Co doping was found to effectively improve the electronic conductivity and active site areas of 2H-MoS2/NC at different positions, optimizing the adsorption and diffusion capability of potassium ions. Furthermore, the study revealed the optimal roles of different types of nitrogen atoms in kinetic adsorption, diffusion, and interfacial stability of potassium ions. These findings provide guidance for the experimental design of high rate 2H-MoS2/NC electrode materials and the optimal design of other functional composite materials.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Zeeshan Ajmal, Mahmood Ul Haq, Shahid Zaman, M. K. Al-Muhanna, Anuj Kumar, Mohammed M. Fadhali, Siwar Ben Hadj Hassine, Muhammas Qasim, K. F. Alshammari, Ghulam Abbas Ashraf, Abdul Qadeer, Adil Murtaza, Sulaiman Al-Sulaimi, Huaqiang Zeng
Summary: This study presents a novel heterojunction structure (SrTiO3/CN-TAL10.0) for enhanced photocatalytic water splitting (PWS). The incorporation of thiophenedicarboxaldehyde (TAL) through copolymerization significantly improves the photocatalytic activity of carbon nitride (CN) while maintaining its photostability performance. The optimized composition allows efficient isolation of photoinduced charge carriers and enhanced charge transport, resulting in a remarkable increase in overall photocatalytic efficiency.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Angela Arnosa-Prieto, Patricia Diaz-Rodriguez, Manuel A. Gonzalez-Gomez, Pelayo Garcia-Acevedo, Lisandra de Castro-Alves, Yolanda Pineiro, Jose Rivas
Summary: Macrophages can exhibit different phenotypes depending on the microenvironment and the characteristics of magnetic iron oxide nanoparticles (MNPs). This study demonstrates that the concentration and morphology of MNPs can influence the polarization of macrophages. The findings have implications for therapeutics targeting tissue regeneration and tumor progression.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Yu Fang, Cheng-Ye Zhu, Hao-Cheng Yang, Chao Zhang, Zhi-Kang Xu
Summary: This study demonstrates the advantages of vacuum-assisted interfacial polymerization (VAIP) in fabricating polyimide nanofiltration membranes. By using vacuum filtration, aqueous solutions of PIP can be evenly distributed on different microfiltration substrates, leading to the fabrication of uniform and ultra-thin polyamide layers with excellent performance. The membranes exhibit high rejection rates and water permeance, as well as satisfactory long-term stability.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Isaac J. Gresham, Edwin C. Johnson, Hayden Robertson, Joshua D. Willott, Grant B. Webber, Erica J. Wanless, Andrew R. J. Nelson, Stuart W. Prescott
Summary: Understanding the interactions between polymers and surfactants is crucial for optimizing commercial systems. This study tested the behavior of polymer-surfactant systems, revealing that they do not behave like polyelectrolytes in the presence of salt. Additionally, the structure of polymer-surfactant complexes under confinement differs from that of polyelectrolytes.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Yunxiao Xie, Cui Liu, Jie Zhang, Yan Li, Bin Li, Shilin Liu
Summary: This study aimed to improve the microstructure and rheological properties of W/W Pickering emulsions by crosslinking sodium alginate at the water-water interface, thereby enhancing the activity of encapsulated probiotics in simulated gastrointestinal digestion.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Sang Ho Lee, Yige Sun, Patrick S. Grant
Summary: This research developed an effective approach to enhance the charging rates of lithium ion batteries (LIBs) by strategically incorporating carbon nanotube (CNT) conductivity boosters into Li4Ti5O12 (LTO) electrodes. Multi-layer architectures comprising CNT-rich and CNT-free LTO electrode layers were manufactured using a layer-by-layer spray coating method to promote charge transfer kinetics of high mass loading electrodes. The best performing multi-layer was paired with a spray-coated LiFePO4 (LFP) positive electrode, resulting in attractive power performance that outperformed conventional LTO || LFP combinations.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Jingwei Liang, Shaobin Li, Fengbo Li, Li Zhang, Yufeng Jiang, Huiyuan Ma, Kun Cheng, Liang Qing
Summary: A molybdenum-regulated self-supporting electrode material with rich vacancy defects has been successfully synthesized and shows exceptional catalytic activities and stability for electrocatalytic overall water splitting. This study provides a new perspective for the design and synthesis of non-precious metal bifunctional electrocatalysts.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Jonas Blahnik, Jennifer Schuster, Rainer Mueller, Eva Mueller, Werner Kunz
Summary: This study investigates the relationship between the morphology of PMMA monopolymers and PMMA-PHEMA copolymers with the expected nature of surfactant-free microemulsions (SFMEs) before polymerization. It is found that previously mesostructured, surfactant-free mixtures can produce porous polymers of different morphologies, while unstructured, oil-rich regions lead to solid, transparent polymers without nanostructured morphologies. Additionally, a surfactant-based reference system shows similar phase behavior and polymer morphologies as the comparable surfactant-free system, indicating the importance of the hydrotropic behavior of HEMA in this system.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Zheng-Fen Pu, Wen-Zhi She, Rong Sheng Li, Qiu-Lin Wen, Bi-Chao Wu, Chun-Hua Li, Jian Ling, Qiue Cao
Summary: This study synthesized two framework-isomeric covalent organic frameworks (COFs) and discovered that the light scattering signal of COFs can be used for the analytical detection of lead ions. By controlling synthesis conditions and introducing regulators, the morphology of COFs could be controlled and framework-isomeric COFs could be precisely synthesized.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Yuchen Weng, Ying Hong, Jingyu Deng, Sicheng Cao, Li-Juan Fan
Summary: This paper reports the preparation of dynamic color-changing fluorescent polymer nanoparticles (PNPs) by constructing a fluorescence resonance energy transfer (FRET) pair. The PNPs show excellent anti-counterfeiting effects and reproducibility. The study demonstrates a promising encryption strategy that can achieve multiple outputs with simple operation.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Guodong Liu, Zijian Wang, Jianing Wang, Hanbin Liu, Zhijian Li
Summary: This study investigates the combination of multicolor switchable polyaniline (PANI) electrode and 1-methyl-4,4'-bipyridyl iodide (MBI), which demonstrates superior optical properties in visible and near-infrared light modulation, as well as excellent electrochemical performances. This combination can be used to develop novel electrochromic devices for applications in smart packaging, smart labels, and flexible smart windows.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Huying Yan, Yang Guo, Xingzhi Bai, Jiawei Qi, Haipeng Lu
Summary: By modifying Ti3C2Tx through heterogeneous interface engineering, optimized impedance matching is achieved, leading to enhanced electromagnetic wave absorption performance.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Kehu Zhang, Yang Zhou, Silvia Moreno, Simona Schwarz, Susanne Boye, Brigitte Voit, Dietmar Appelhans
Summary: This article presents an advanced crosslinking strategy to fabricate clustered polymersomes using host-guest interactions. By controlling the input of crosslinker and environmental conditions, reversible aggregation and disassembly of these polymersomes can be achieved. The size and structure of these clustered polymersomes can be regulated and visualized through a fluorescent enzymatic cascade reaction.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Junjie Xu, Weixiong Huang, Ruiling Li, Li Li, Jinjin Ma, Jiaou Qi, Haiyan Ma, Min Ruan, Lilin Lu
Summary: In this study, a potassium doped palladium catalyst was developed for acetylene hydrogenation, showing excellent catalytic performance and durability. The doping of potassium effectively weakened the adsorption of ethylene, improved ethylene selectivity, and lowered the barriers of hydrogen activation and transfer reactions.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)