4.7 Article

Modeling hydrogen-rock-brine interactions for the Jurassic reservoir and cap rocks from Polish Lowlands

期刊

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
卷 47, 期 20, 页码 10947-10962

出版社

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ijhydene.2022.01.134

关键词

Underground hydrogen storage; Reservoir rocks; Cap rocks; Geochemical modeling; Hydrogen-Rock-Fluid; interactions; Aquifer storage

资金

  1. Mineral and Energy Economy Research Institute of the Polish Academy of Sciences
  2. Fuel Cells and Hydrogen 2 Joint Undertaking [101007176]
  3. European Union
  4. Hydrogen Europe
  5. Hydrogen Europe Research

向作者/读者索取更多资源

This study presents the geochemical modeling results of hydrogen-rock-brine interactions for different types of rocks from the Polish Lowland. Goethite is identified as the main component responsible for the consumption of stored hydrogen. The changes in rock porosity are found to be smaller in sandstones compared to mudstones and claystones. The findings provide insights into the behavior of hydrogen in underground storage conditions.
Hydrogen offers an opportunity to move away from fossil fuels, it may help to alleviate major drawbacks of intermittent renewable energy generation. The results of geochemical modeling of hydrogen-rock-brine interactions for sandstones, mudstones and claystones from the geological structures from Polish Lowland are presented. The pH of the pore water is a critical parameter that controls the extent of the reaction. Several dominant reaction schemes were distinguished, and goethite was indicated as responsible for the consumption of stored hydrogen. It was found that the changes in rock porosity in sandstones were much smaller than in mudstones and claystones. The Zaosie sandstones are more favorable for UHS than those from Chabowo. The degradation of cap rock integrity, requires each time further experimental research. The findings of this study can help for better understanding of the behavior of hydrogen, in terms of gas-rock-brine interactions, in conditions of its underground storage.(c) 2022 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

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