Insights into the source-specific health risk of ambient particle-bound metals in the Pearl River Delta region, China

Quantification of source-specific health risks of PM2.5 plays an essential role in health-oriented air pollution control. However, there is limited evidence supporting the source-based risk apportionment of particle-bound metals. In this study, source-specific cancer and non-cancer risk characterization of 12 particle-bound metals was performed in the Pearl River Delta (PRD) region, China. A combination of health risk assessment model and receptor-based source apportionment modeling with positive matrix factorization (PMF) was applied for characterizing the spatial-temporal patterns for inhalation health risks of particle-bound metals in three main city clusters, inland area and coastal area in the region from December 2014 through July 2016. Results showed that the carcinogenic risk of particle-bound metals for adults (4.13 x 10(-5)) was higher than that for children (9.53 x 10(-6)) in the PRD region. The highest and significant non-carcinogenic risk was found in the northwest city cluster. Industrial emission (63.3%) were the dominant contributors to the cancer risk, while the main contributors to the non-cancer risk were the vehicle emission source (33.2%) in the dry season and industrial emission (30.8%) in the wet season. Our results provide important evidence for spatial source-specific health risks with temporal characteristics of particle-bound metals in most densely populated areas in the southern China, and suggest that reduction of industrial and vehicle emissions could facilitate more cost-effective PM2.5 control measures to improve human health.

Automated summary

This study quantified source-specific cancer and non-cancer risk of 12 particle-bound metals in the Pearl River Delta region, China, using health risk assessment models and receptor-based source apportionment modeling. Results showed higher carcinogenic risk for adults compared to children, with industrial emissions being the dominant contributor to cancer risk and vehicle emissions being significant contributors to non-cancer risk. The findings provide important evidence for spatial source-specific health risks of particle-bound metals in densely populated areas in southern China.