4.8 Review

Recent progress of cathode materials for aqueous zinc-ion capacitors: Carbon-based materials and beyond

期刊

CARBON
卷 185, 期 -, 页码 126-151

出版社

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.carbon.2021.08.084

关键词

Zinc-ion capacitor; Supercapacitor; Cathode material; Nano carbon; Hybrid capacitor

资金

  1. Ministry of Science and Technology of China (MoST) [2016YFA0200200]
  2. National Natural Science Foundation of China (NSFC) [21421001, 51633002, 21902071]
  3. Henan Provincial Key Research and Development Program [192102310202]
  4. Sun Tat-Sen University
  5. Adlerbertska Forskningsstiftelsen [C 2020-1230]
  6. Goteborg Energi
  7. Swedish Research Council [2020-04903]
  8. Stiftelsen Chalmers Tekniska Hogskola
  9. Swedish Research Council [2020-04903] Funding Source: Swedish Research Council

向作者/读者索取更多资源

Aqueous zinc-ion capacitors (AZICs) combine the advantages of zinc-ion batteries and supercapacitors, making them a promising electrochemical energy storage system. However, their energy density needs to be improved for practical applications, requiring high-capacity cathode materials.
As an emerging multivalent-ion-based energy storage device, aqueous zinc-ion capacitors (AZICs) combine the merits of zinc-ion batteries with high energy density, excellent safety, low cost and environmental friendliness, and the advantages of supercapacitors with high power density and superior cycling performance. Therefore, AZICs have been considered as a new promising electrochemical energy storage system. Though great progress of AZICs has been made recently, they are still in the infant stage and face many challenges. Specially, the unsatisfactory energy density needs to be improved to realize their practical applications, which calls for high-capacity cathode materials. In this review, after a brief introduction of progress and mechanism for AZICs, we provide a systematical overview of the latest advances in the state-of-art cathode materials. The synthesis route, structure and morphology, electrochemical performance, energy storage mechanism as well as the merits and drawbacks of various cathode materials are comprehensively compared and discussed. Finally, a summary and outlook of the challenges and future perspectives of AZICs were presented. With these, this review might offer some guidance for the future design of dedicated novel cathode materials to realize the great potential of AZICs. (c) 2021 Elsevier Ltd. All rights reserved.

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