4.8 Article

Investigation of the thermal responses under gas channel and land inside proton exchange membrane fuel cell with assembly pressure

期刊

APPLIED ENERGY
卷 308, 期 -, 页码 -

出版社

ELSEVIER SCI LTD
DOI: 10.1016/j.apenergy.2021.118377

关键词

Proton exchange membrane fuel cell; Thermal response; Electrical and thermal contact resistances; Assembly pressure; Transient simulation

资金

  1. National Key Research and Development Program of China [2018YFB1502500]
  2. Nanchang Automotive Innovation Institute, Tongji University [QZKT2020-16]

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In this study, a new fuel cell model was established to investigate the thermal response of the proton exchange membrane fuel cell. The impacts of interface resistance, working conditions, and assembly pressure on thermal responses were systematically studied. It was found that the thermal contact resistance significantly increased the temperature in both regions, while the electrical contact resistance only slightly raised it. Additionally, uneven distribution and rapid overshoot/undershoot of temperature were observed during overload and change load operations. Choosing the appropriate assembly pressure was crucial for balancing performance and heat transfer.
The improper thermal response is one of the main causes of proton exchange membrane fuel cell degradation. In this study, a two-dimensional, non-isothermal, two-phase transient fuel cell model has been established com-bined with newly measured experimental data. This model fully incorporates the land and gas channel (GC) of the bipolar plate, comprehensively accounting for the electrical contact resistance (ECR) and the thermal contact resistance (TCR) at the carbon paper/land interface, as well as the changes of carbon paper structure and electrical/thermal resistance induced by assembly pressure. By simulation, the impacts of interface resistance, working conditions, and assembly pressure on the thermal responses under land and GC are systematically investigated. The existence of TCR is found to increase the two regions' temperature significantly, while ECR only slightly raises it by generating a surface heat source. Furthermore, uneven distribution, ununiform fluc-tuation, and rapid overshoot/undershoot of temperature are observed in the two areas during overload and change load operations. It is mainly caused by the different distributions and responses of reaction and phase change at various locations. In the end, the average temperature is found to fall significantly and reach a new steady fastly with the increase of assembly pressure due to the reduction of bulk and interface thermal resistances of carbon paper. However, performance degradation and hot spot temperature rise are further observed if the pressure is too high. To balance performance and heat transfer, we should choose an optimal assembly pressure.

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