期刊
TETRAHEDRON LETTERS
卷 81, 期 -, 页码 -出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tetlet.2021.153357
关键词
Visible-light photoredox catalysis; Homoallylic amines; Desilylative allylation; alpha-Amino alkyl radical
资金
- Foundation of Henan University of Technology [2018BS045]
- Colleges and Universities Key Research Program Foundation of Henan Province [20A150014]
- Innovative Funds Plan of Henan University of Technology [2020ZKCJ29]
- National Natural Science Foundation of China [21801063]
A facile and efficient synthesis of homoallylic amines was achieved by visible-light photoredox-promoted desilylative allylation of alpha-silylamines with allylic sulfones, providing good to high yields under mild reaction conditions.
A facile and efficient synthesis of homoallylic amines by visible-light photoredox-promoted desilylative allylation of alpha-silylamines with allylic sulfones is described. A variety of alpha-silylamines derived from anilines, cyclic and acyclic alkyl amines reacted with a serious of mono or disubstituted allylic sulfones well to provide homollylic amines in good to high yields under very mild reaction conditions. (C) 2021 Elsevier Ltd. All rights reserved.
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