期刊
SCIENCE CHINA-CHEMISTRY
卷 64, 期 9, 页码 1547-1553出版社
SCIENCE PRESS
DOI: 10.1007/s11426-021-1033-6
关键词
carbon dots; near-infrared; high quantum yields; self-oxidation; white LEDs
资金
- National Natural Science Foundation of China [21905253, 51973200]
- China Postdoctoral Science Foundation [2018M640681, 2019T120632]
- Natural Science Foundation of Henan [202300410372]
The study successfully prepared CDs with a maximum emission of 714 nm and a quantum yield as high as 22.64%, which can self-oxidize and emit white light, making them suitable for preparing WLEDs.
Carbon dots (CDs), as a kind of carbon nanomaterials, have attracted widespread attention due to their unique structure and excellent optical properties, and they are low-cost, environmentally friendly and biocompatible. However, the development of near-infrared (NIR) emission CDs remains a challenge. In this study, we successfully prepared CDs with a maximum emission of 714 nm using citric acid as the carbon source, thiourea and ammonium fluoride as the dopant source, and N,N-dimethylformamide as the solvent. The quantum yield (QY) is as high as 22.64%. Interestingly, the prepared CDs self-oxidize in the presence of oxygen, resulting in a blue shift of their emission. Therefore, they can be used to prepare white light-emitting diodes (WLEDs) without adding other fluorescent substances. Notably, the work presented herein constitutes the first report of WLEDs preparation from single CDs.
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