4.8 Article

Power Management and Reaction Optimization for a Self-Powered Electrochemical System Driven by a Triboelectric Nanogenerator

期刊

NANO LETTERS
卷 21, 期 13, 页码 5633-5640

出版社

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.1c01152

关键词

triboelectric nanogenerators; electrochemistry; power management; reaction optimization; self-powered electrochemical system

资金

  1. National Key R&D Project from the Minister of Science and Technology [2016YFA0202704]
  2. National Natural Science Foundation of China [51432005, 51702018, 51561145021]
  3. Youth Innovation Promotion Association, CAS

向作者/读者索取更多资源

The research demonstrates an advanced self-powered electrochemical system that achieves significant results in hydrogen peroxide production and internal current efficiency through optimizing power management and electrochemical reaction regulation. The system not only saves electricity but also utilizes environmental mechanical vibrational energy for ecological improvement or recyclable chemical fuel generation, enabling the application of electrochemical reactions in remote areas.
Harvesting distributed and low-quality mechanical energies by triboelectric nanogenerators to power electrochemical reactions is beneficial to electric energy saving and certain applications. However, the conventional self-powered electrochemical process is awkward about the reaction rate, energy conversion efficiency, high-operation frequency, and mismatched impedance. Here we demonstrate an advanced self-powered electrochemical system. In comparison with the conventional system that is inert in activity, the superior power management and electrochemical reaction regulation in tandem make the novel system outstanding for hydrogen peroxide production. In addition to the visible product, an internal current efficiency of 24.6% in the system was achieved. The developed system provides an optimization strategy toward electric energy saving for electrochemical reactions as well as enabling their applications in remote areas by converting environmental mechanical vibrational energy for ecological improvement or recyclable chemical fuel generation.

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