4.8 Article

Self-Resonant Microlasers of Colloidal Quantum Wells Constructed by Direct Deep Patterning

期刊

NANO LETTERS
卷 21, 期 11, 页码 4598-4605

出版社

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.1c00464

关键词

semiconductor nanocrystals; direct nanopatterning; UV-induced ligand exchange; electron beam lithography; microlaser; optical nanocircuit; colloidal quantum wells

资金

  1. National Research Foundation, Prime Minister's Office, Singapore [NRF-NRFI2016-08]
  2. Singapore Agency for Science, Technology and Research (A*STAR) SERC Pharos Program [152 73 00025]
  3. TUBITAK [115E679, 115F297, 117E713]
  4. TUBITAK through the BIDEB-2211 program

向作者/读者索取更多资源

The study presents the first account of self-resonant fully colloidal mu-lasers made from colloidal quantum well (CQW) solution. A deep patterning technique is developed to fabricate well-defined high aspect-ratio on-chip CQW resonators, allowing for in-plane lasing with tight optical confinement. The method is also successfully applied to various nanoparticles without affecting their physical and chemical properties.
Here, the first account of self-resonant fully colloidal mu-lasers made from colloidal quantum well (CQW) solution is reported. A deep patterning technique is developed to fabricate well-defined high aspect-ratio on-chip CQW resonators made of grating waveguides and in-plane reflectors. The fabricated waveguide-coupled laser, enabling tight optical confinement, assures in-plane lasing. CQWs of the patterned layers are closed-packed with sharp edges and residual-free lifted-off surfaces. Additionally, the method is successfully applied to various nanoparticles including colloidal quantum dots and metal nanoparticles. It is observed that the patterning process does not affect the nanocrystals (NCs) immobilized in the attained patterns and the different physical and chemical properties of the NCs remain pristine. Thanks to the deep patterning capability of the proposed method, patterns of NCs with subwavelength lateral feature sizes and micron-scale heights can possibly be fabricated in high aspect ratios.

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