期刊
JOURNAL OF PHYSICAL CHEMISTRY B
卷 125, 期 32, 页码 9037-9051出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.jpcb.1c03756
关键词
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资金
- CPIMS program by Office of Science, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy [DEAC02-05CH11231]
- Chemical Sciences Geosciences and Biosciences Division of the Office of Basic Energy Sciences of the DOE [DE-AC02-05CH11231]
- DOE Office of Science User Facility [DE-AC0205CH11231]
- Office of Science of the U.S. Department of Energy [DE-AC0205CH11231]
This passage discusses how the properties of bulk water and aqueous solutions change near an interface or in a confined environment, and how air, liquid, and solid interfaces can alter molecular properties and chemical reactivity compared to bulk water and multicomponent solutions. It also highlights advancements in interfacial chemistry through new theory, molecular simulation, and experiments.
The properties of bulk water and aqueous solutions are known to change in the vicinity of an interface and/or in a confined environment, including the thermodynamics of ion selectivity at interfaces, transition states and pathways of chemical reactions, and nucleation events and phase growth. Here we describe joint progress in identifying unifying concepts about how air, liquid, and solid interfaces can alter molecular properties and chemical reactivity compared to bulk water and multicomponent solutions. We also discuss progress made in interfacial chemistry through advancements in new theory, molecular simulation, and experiments.
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