期刊
FUEL
卷 300, 期 -, 页码 -出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.fuel.2021.120979
关键词
Ammonia; Oxidation; Nitrogen oxides; Kinetic modeling; Carbon-free fuels
资金
- Aragon Government [T22_17R]
- FEDER 2014-2020 Construyendo Europa desde Aragon
- FEDER [RTI2018-098856-B-I00]
- MCIU [RTI2018-098856-B-I00]
This study focused on the analysis of the ammonia oxidation process and the formation of main nitrogen oxides over a wide range of temperatures and O2 reaction environments. Experimental results were simulated and interpreted using a detailed chemical-kinetic mechanism, with reaction path and sensitivity analyses used to delineate the NH3 oxidation scheme.
The present work is focused on the analysis of the ammonia oxidation process and the formation of main nitrogen oxides (NO, NO2 and N2O) over a wide range of temperatures and O2 reaction environments. Experiments are performed at atmospheric pressure in a laboratory quartz tubular flow reactor, covering the temperature range of 875 to 1450 K and for different air excess ratios (from pyrolysis to very oxidizing conditions). The experimental results are simulated and interpreted in terms of a detailed chemical-kinetic mechanism. Reaction path and sensitivity analyses are used to delineate the NH3 oxidation scheme.
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