4.5 Article

Visible-light induced photocatalytic removal of U(VI) from aqueous solution by MoS2/g-C3N4 nanocomposites

期刊

出版社

SPRINGER
DOI: 10.1007/s10967-020-07567-x

关键词

U(VI); Photocatalysis; MoS2; g-C3N4; Reduction

资金

  1. National Natural Science Foundation of China [21866004, 21866003]
  2. Defense Industrial Technology Development Program [JCKY2019401C004]
  3. Jiangxi Provincial Department of Science and Technology [2018ACB21007]
  4. Major Discipline Academic and Technical Leaders Training Program of Jiangxi Province [20182BCB22011]

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In this study, MoS2/g-C3N4 nanocomposites were prepared and showed efficient uranium ions removal. The optimal composites containing 3% MoS2 demonstrated superior photocatalytic performance in reducing U(VI) due to the pivotal role of MoS2 in light adsorption and charge separation.
In this study, MoS2/g-C3N4 nanocomposites was prepared via an ultrasonication and calcination method and used for uranium ions removal from uranium containing solution. The optimum MoS2/g-C3N4 composites photocatalyst with the molar content of 3% MoS2 had the highest photocatalytic performance (93% reduction efficiency within 60 min irradiation time), which was approximately five times faster than that of pure g-C3N4. MoS2 plays pivotal roles in light adsorption, transfer and charge separation in photoreduction of U(VI) process.

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