4.8 Article

Understanding global changes in fine-mode aerosols during 2008-2017 using statistical methods and deep learning approach

期刊

ENVIRONMENT INTERNATIONAL
卷 149, 期 -, 页码 -

出版社

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.envint.2021.106392

关键词

Satellite; Aerosol; fAOD; FMF

资金

  1. National Natural Science Foundation of China [41801329, 91837204]
  2. National Key Research and Development Plan of China [2017YFC1501702]
  3. Open Fund of State Key Laboratory of Remote Sensing Science [OFSLRSS201915]
  4. Fundamental Research Funds for the Central Universities

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The study found that from 2008 to 2017, there was a significant increasing trend in global fine-mode aerosols on land, while no significant trends were observed in aerosol fine-mode fraction over the ocean and fine-mode aerosol optical depth over both land and ocean. A significant decline in fine-mode aerosol optical depth was identified in China, indicating the effectiveness of government emission controls.
Despite their extremely small size, fine-mode aerosols have significant impacts on the environment, climate, and human health. However, current understandings of global changes in fine-mode aerosols are limited. In this study, we employed newly developed satellite retrieval data and an attentive interpretable deep learning model to explore the status, changes, and association factors of the global fine-mode aerosol optical depth (fAOD) and aerosol fine-mode fraction (FMF) from 2008 to 2017. At the global scale, the results show a significant increasing trend in land FMF (2.34 x 10(-3)/year); however, the FMF over the ocean and the fAOD over land and ocean did not reveal significant trends. Between 2008 and 2017, high levels of both fAOD (<0.65), while land fAOD was high in summer (>0.15) but low in winter (<0.13). Importantly, Australia and Mexico experienced significant increasing trends in FMF during all four seasons. At the regional scale, a significant decline in fAOD was identified in China, which indicates that government emission controls and reductions have been effective in recent decades. The deep learning model was used to interpret the result and showed that O-3 was significantly associated with changes in both the FMF and fAOD. This finding suggests the importance of synergizing the regulations for both O-3 and fine particles. Our work comprehensively examined global spatial and seasonal fAOD and FMF changes and provides a holistic understanding of global anthropogenic impacts.

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