期刊
MATERIALS CHEMISTRY AND PHYSICS
卷 259, 期 -, 页码 -出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.matchemphys.2020.124169
关键词
MWCNTs; Fe-Ni alloy; NiFe2O4; Polypyrrole; Polystyrene sulfonate; Microwave absorption
The MWCNTs/Fe-Ni alloy/NiFe2O4 (M/F/N) nanocomposite was prepared through a hydrothermal method and then coated with poly(pyrrole-co-styrene sulfonate) (PP@M/F/N) via in-situ polymerization. The nanocomposite exhibited excellent microwave absorption properties in the X band frequency range, with a minimum reflection loss of -85 dB at 12 GHz for 2 mm thickness. Coating with the copolymers improved electron transport, impedance matching, interfacial polarization, and attenuation ability of the composite. This study provides a facile and efficient method for preparing magneto-electric nanocomposites as promising candidates for microwave absorption applications.
In this work, MWCNTs/Fe-Ni alloy/NiFe2O4 (M/F/N) nanocomposite was prepared via hydrothermal method and then coated with poly(pyrrole-co-styrene sulfonate) (PP@M/F/N) via using in-situ polymerization method. The molar ratios of pyrrole and 3,4-ethylenedioxythiophene co-polymers were adjusted 1:1. The morphological observations confirmed that magnetic nanoparticles were decorated with MWCNTs and finally coated by co-polymers. The microwave absorption results demonstrate that the minimum reflection loss of PP@M/F/N achieved to-85 dB at 12 GHz with effective bandwidth (less than -10 dB) in the range of X band frequency for 2 mm thickness. It was clearly observed that the minimum RL resonance peaks matched at lower frequencies with the increase of thicknesses for PP@M/F/N nanocomposite. According to the results, the formation of conductive network facilitated the electron transport and improved the impedance matching, interfacial polarization, and attenuation ability of the composite. This work illustrated a facile and efficient way to prepared magneto electric nanocomposite as a promising candidate for microwave absorption with a versatile design concept for other types of absorber.
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