4.8 Article

Tunable Chiral Optics in All-Solid-Phase Reconfigurable Dielectric Nanostructures

期刊

NANO LETTERS
卷 21, 期 2, 页码 973-979

出版社

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.0c03957

关键词

reconfigurable chiral metamaterials; dielectric materials; optical coupling; optical nanofabrication; biosensing

资金

  1. National Aeronautics and Space Administration Early Career Faculty Award [80NSSC17K0520]
  2. National Science Foundation [NSF-CMMI-1761743, NSF-CBET-1704634]
  3. National Institute of General Medical Sciences of the National Institutes of Health [DP2GM128446]
  4. University Graduate Continuing Fellowship of the University of Texas at Austin
  5. Simons Foundation
  6. Air Force Office of Scientific Research
  7. Robert A. Welch Foundation [F-1464]
  8. National Science Foundation through the Center for Dynamics and Control of Materials (CDCM) Materials Research Science and Engineering Center (MRSEC) [DMR-1720595]
  9. Welch Foundation [F-1734-20190330]

向作者/读者索取更多资源

A study has reported reconfigurable chiral nanostructures with silicon nanoparticles and nanowires, allowing for tailored configurations and chiroptical responses. The optical chirality arises from the coupling between optical resonances of the silicon nanoparticle and nanowire, enabling label-free enantiodiscrimination of biomolecules in single structures. This research provides insights into high-index material design and new strategies for adaptive devices in photonic and electronic applications.
Subwavelength nanostructures with tunable compositions and geometries show favorable optical functionalities for the implementation of nanophotonic systems. Precise and versatile control of structural configurations on solid substrates is essential for their applications in on-chip devices. Here, we report all-solid-phase reconfigurable chiral nanostructures with silicon nanoparticles and nanowires as the building blocks in which the configuration and chiroptical response can be tailored on-demand by dynamic manipulation of the silicon nanoparticle. We reveal that the optical chirality originates from the handedness-dependent coupling between optical resonances of the silicon nanoparticle and the silicon nanowire via numerical simulations and coupled-mode theory analysis. Furthermore, the coexisting electric and magnetic resonances support strong enhancement of optical near-field chirality, which enables label-free enantiodiscrimination of biomolecules in single nanostructures. Our results not only provide insight into the design of functional high-index materials but also bring new strategies to develop adaptive devices for photonic and electronic applications.

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