期刊
MATERIALS CHEMISTRY AND PHYSICS
卷 258, 期 -, 页码 -出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.matchemphys.2020.123830
关键词
Reduction of nitrogen; Modifying Fe(III); Carbon nitride; Nitrogen vacancies
资金
- National Natural Science Foundation of China [51872116, 51571100]
- National Key R&D Program of China [2016YFA0200400]
- Program for JLU. Science and Technology Innovative Research Team (JLUSTIRT) [2017TD-09]
- Jilin province science and the Technology development program [20190201233JC]
The modification of Fe(III) onto carbon nitride has been shown to enhance the photocatalytic nitrogen fixation, making it a promising strategy for high-efficiency artificial photosynthesis ammonia. This new approach involves narrowing down the carbon nitride intrinsic bandgap and suppressing radiative electron-hole recombination.
Solar-driven reduction of nitrogen to ammonia is a promising strategy for energy storage and conversion. Herein, a new strategy of modifying Fe(III) onto carbon nitride is reported showing enhanced photocatalytic nitrogen fixation. The Fe(III) and nitrogen vacancies narrow down the carbon nitride intrinsic bandgap and suppress the radiative electron-hole recombination. Fe(III)-C3N4 therefore shows potential as a new high-efficiency artificial photosynthesis ammonia.
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