4.8 Article

Wearable Porous Au Smartsensors for On-Site Detection of Multiple Metal Ions

期刊

ANALYTICAL CHEMISTRY
卷 93, 期 4, 页码 2603-2609

出版社

AMER CHEMICAL SOC
DOI: 10.1021/acs.analchem.0c04701

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资金

  1. National Natural Science Foundation of China [22074010, 21705014]
  2. Dalian Science and Technology Bureau, China [2019J12SN54]
  3. Zhang Dayu School of Chemistry, Dalian University of Technology, China

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A porous Au-based smartsensor was developed using screen printing technology and sacrificial template electrodeposition for on-site detection of multiple metal ions. It exhibited excellent detection performance, stability, and reliability in actual liquid cosmetic samples, showing potential for application in artificial intelligence in daily life.
Owing to advantages of miniaturization, convenient integration, flexibility, and real-time monitoring, wearable smartsensors have received numerous attention and greatly developed in various fields. However, there usually appears a contradiction between sensing behaviors and simple fabricated methods, seriously limiting on-site detection of actual samples. In this work, a porous Au-based smartsensor has been in situ prepared by combining screen printing technology and sacrificial template electrodeposition. Thanks to abundant active adsorption sites, multiple metal ions (Pb, Cu, and Hg) can be easily achieved on-site detection by this smart platform with a low limit of detection as well as high sensitivity, excellent selectivity, good stability, repeatability, and bending performance. Significantly, it also exhibits a reliable detective capability in actual liquid cosmetic samples with a portable cellphone, which identically corresponds to standard inductively coupled plasma-mass spectrometry (ICP--MS) evaluation. Therefore, this wearable smartsensor provides a promising platform for artificial intelligence application in future daily life.

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