4.8 Article

Photonic Rashba effect from quantum emitters mediated by a Berry-phase defective photonic crystal

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NATURE NANOTECHNOLOGY
卷 15, 期 11, 页码 927-+

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NATURE RESEARCH
DOI: 10.1038/s41565-020-0758-6

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资金

  1. Israel Science Foundation (ISF)
  2. US Air Force Office of Scientific Research through their programme on Photonic Metamaterials [FA9550-18-1-0208]
  3. Israel Ministry of Science, Technology and Space
  4. United States-Israel Binational Science Foundation (BSF)
  5. Technion via an Aly Kaufman Fellowship

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Planar metasurfaces are a valuable tool to achieve custom-tailored photoluminescence from quantum emitters. The incorporation of a WSe(2)monolayer into a photonic crystal slab with geometric phase defects enables spin-dependent manipulation of the emission from valley excitons of the WSe2, as well as from randomly placed quantum emitters. Heterostructures combining a thin layer of quantum emitters and planar nanostructures enable custom-tailored photoluminescence in an integrated fashion. Here, we demonstrate a photonic Rashba effect from valley excitons in a WSe(2)monolayer, which is incorporated into a photonic crystal slab with geometric phase defects, that is, into a Berry-phase defective photonic crystal. This phenomenon of spin-split dispersion in momentum space arises from a coherent geometric phase pickup assisted by the Berry-phase defect mode. The valley excitons effectively interact with the defects for site-controlled excitation, photoluminescence enhancement and spin-dependent manipulation. Specifically, the spin-dependent branches of photoluminescence in momentum space originate from valley excitons with opposite helicities and evidence the valley separation at room temperature. To further demonstrate the versatility of the Berry-phase defective photonic crystals, we use this concept to separate opposite spin states of quantum dot emission. This spin-enabled manipulation of quantum emitters may enable highly efficient metasurfaces for customized planar sources with spin-polarized directional emission.

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