期刊
MATERIALS RESEARCH BULLETIN
卷 130, 期 -, 页码 -出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.materresbull.2020.110870
关键词
g-C3N4; rGO; Photocatalyst; Visible light; Degradation
资金
- Anna University through Anna Centenary Research Fellowship [CFR/ACRF-2019/AR1]
- CSIR [09/468/0532/2019 EMR-I]
- DST-TDP [DST/TDT/TDP-06/2017]
In this study, bare g-C3N4, g-C3N4/rGO and Br-modified g-C3N4/rGO catalysts were synthesized by a simple hydrothermal method. The synthesized catalysts were analyzed by XRD, FTIR, Raman, HR-SEM, TEM, BET, UV-DRS, PL and EIS techniques. The photocatalytic performance of synthesized catalysts was evaluated towards the decolourisation of Reactive Blue-19, Methyl Orange and Rhodamine-B dyes under visible light irradiation. In comparison with bare g-C3N4 and g-C3N4/rGO catalysts, the Br modified g-C3N4/rGO catalyst showed superior photocatalytic performance. The PL spectra of synthesized catalysts reveal that Br modified g-C3N4/rGO catalyst has a lower rate of electron hole-pair recombination when compared to bare g-C3N4 and g-C3N4/rGO catalysts, which leads to enhanced photocatalytic activity. The stability of the most active catalyst was analyzed by recyclability test. The major influences of photogenerated holes (h(+)) followed by O-center dot(2)- radicals and (OH)-O-center dot radicals were observed on the photocatalytic degradation of dyes by radical trapping experiment over Br modified g-C3N4/rGO.
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