期刊
JOURNAL OF PHYSICAL CHEMISTRY C
卷 124, 期 28, 页码 15468-15473出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.jpcc.0c02715
关键词
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资金
- Austrian Science Fund (FWF) [P25377-N20]
- Major scientific research instrument development project of NSFC [61927808]
- China Scholarship Council (CSC)
- Eurasia Pacific Uninet
- Consejo Nacional de Cienciay Tecnologa, through the Becas Mixtas program
In-plane optical anisotropy has been detected from monolayer MoS2 grown on a-plane (11 (2) over bar0) sapphire substrate in the ultraviolet-visible wavelength range. Based on the measured optical anisotropy, the energy differences between the optical transitions polarized along the ordinary and extraordinary directions of the underlying sapphire substrate have been determined. The results corroborate comprehensively with the dielectric environment induced modification on the electronic band structure and exciton binding energy of monolayer MoS2 predicted recently by first-principle calculations. The output of this study proposes the symmetry as a new degree of freedom for dielectric engineering of the two-dimensional materials.
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