期刊
CHEMICAL ENGINEERING & TECHNOLOGY
卷 43, 期 10, 页码 2126-2133出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ceat.202000154
关键词
Alkali promoter; Ammonia production; Chemical looping; Manganese nitride; Renewable energy carrier
资金
- National Science Foundation [1856084Number DOE EPSCOR 0001572]
Affordable synthetic ammonia (NH3) enables the production of nearly half of the food we eat and is emerging as a renewable energy carrier. Sodium-promoted chemical looping NH(3)synthesis at atmospheric pressure using manganese (Mn) is here demonstrated. The looping process may be advantageous when inexpensive renewable hydrogen from electrolysis is available. Avoiding the high pressure of the Haber-Bosch process by chemical looping using earth-abundant materials may reduce capital cost, facilitate intermittent operation, and allow operation in geographic areas where infrastructure is less sophisticated. At this early stage, the data suggest that 0.28 m(3)of a 50 % porosity solid Mn bed may suffice to produce 100 kg NH(3)per day by chemical looping, with abundant opportunities for improvement.
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