期刊
CHEMSUSCHEM
卷 9, 期 8, 页码 800-805出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.201600088
关键词
cadmium/aluminum; carbon dioxide; layered double hydroxide; photoreduction; reaction diffusion framework
资金
- American University of Beirut Research Board
- Lebanese National Council for Scientific Research (LCNSR)
- Masri institute at AUB [102882]
We report the synthesis of cadmium-aluminum layered double hydroxide (CdAl LDH) using the reaction-diffusion framework. As the hydroxide anions diffuse into an agar gel matrix containing the mixture of aluminum and cadmium salts at a given ratio, they react to give the LDH. The LDH self-assembles inside the pores of the gel matrix into a unique spherical-porous shaped microstructure. The internal and external morphologies of the particles are studied by electron microscopy and tomography revealing interconnected channels and a high surface area. This material is shown to exhibit a promising performance in the photoreduction of carbon dioxide using solar light. Moreover, the palladium-decorated version shows a significant improvement in its reduction potential at room temperature.
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