期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 22, 期 18, 页码 6234-6238出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201600570
关键词
carbonylation; cross-coupling; cyclization; lactones; palladium
资金
- National Research Foundation of Korea (NRF) [2011-0016830]
- National Research Foundation of Korea [2011-0016830] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
A carbonylative esterification reaction between aryl bromides and alcohols, promoted by Pd/C and NaF in the presence of oxiranes, has been developed. In this process, oxiranes serve as sources of carbon monoxide by their conversion to aldehydes through a palladium-promoted Meinwald rearrangement pathway. Intramolecular versions of this process serve as methods for the synthesis of lactones and phthalimides.
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