4.7 Article

Enhancing the corrosion resistance of Q235 mild steel by incorporating poly (dopamine) modified h-BN nanosheets on zinc phosphate-silane coating

期刊

SURFACE & COATINGS TECHNOLOGY
卷 390, 期 -, 页码 -

出版社

ELSEVIER SCIENCE SA
DOI: 10.1016/j.surfcoat.2020.125682

关键词

Zinc phosphating; Corrosion resistance; Boron nitride; Mild steel; Dopamine; Silane treatment

资金

  1. National Natural Science Foundation of China [51501055, 51601056]
  2. Hebei province Science and Technology Support Program [19274009D]

向作者/读者索取更多资源

Phosphate-silane coatings were developed on the Q235 mild steel by incorporating poly(dopamine) modified h-BNs into the zinc phosphating bath to enhance the corrosion resistance. The effects of PDA modified h-BNs with varying concentrations (0.10-0.90 g/L) on the surface modification, and corrosion resistance of the composite coatings were investigated. Results show that denser and uniform coatings were achieved for samples containing poly(dopamine) modified h-BN. Sample 0.60 g/L attained outstanding corrosion resistance, which is in one order of magnitude lower than the pure coatings with a current density of 1.95 x 10(-5) A/cm(2). Modified h-BN effectively accelerates and enhances the corrosion resistance of the phosphate-silane coatings.

作者

我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。

评论

主要评分

4.7
评分不足

次要评分

新颖性
-
重要性
-
科学严谨性
-
评价这篇论文

推荐

Article Chemistry, Multidisciplinary

Competitive Coordination-Oriented Monodispersed Ruthenium Sites in Conductive MOF/LDH Hetero-Nanotree Catalysts for Efficient Overall Water Splitting in Alkaline Media

Ying Wang, Shuo Wang, Ze-Lin Ma, Li-Ting Yan, Xue-Bo Zhao, Ying-Ying Xue, Jia-Min Huo, Xiao Yuan, Shu-Ni Li, Quan-Guo Zhai

Summary: This study reports a highly efficient electrocatalyst for water splitting, which is fabricated using a controllable grafted-growth strategy to form a cMOF/LDH hetero-nanotree array catalyst coupled with monodispersed ruthenium (Ru) sites. The optimized catalyst shows excellent electrochemical water-splitting properties in alkaline media, outperforming most reported MOF-based catalysts.

ADVANCED MATERIALS (2022)

Correction Chemistry, Multidisciplinary

Lattice Matching Growth of Conductive Hierarchical Porous MOF/LDH Heteronanotube Arrays for Highly Efficient Water Oxidation (vol 33, 2006351, 2021)

Ying Wang, Liting Yan, Kamran Dastafkan, Chuan Zhao, Xuebo Zhao, Yingying Xue, Jiamin Huo, Shuni Li, Quanguo Zhai

ADVANCED MATERIALS (2022)

Article Energy & Fuels

A weather-resistant daytime radiative cooler based on fluorocarbon resin

Ruifeng Dong, Tiantian Du, Shuhan Dong, Xue Zhao, Ruina Ma, An Du, Yongzhe Fan, Xiaoming Cao

Summary: Daytime radiative cooling technology allows for cooling without energy consumption or pollution, and the double-layer DRC structure using FEVE and silver as materials shows excellent cooling performance due to high reflectivity and emissivity. The application of this material in Tianjin, China demonstrates significant temperature drop, indicating its potential for practical use.

SOLAR ENERGY MATERIALS AND SOLAR CELLS (2022)

Article Energy & Fuels

Defect-engineered MOF-808 with highly exposed Zr sites as highly efficient catalysts for catalytic transfer hydrogenation of furfural

Qiuju Fu, Dandan Liu, Weijing Niu, Shuo Zhang, Ruihua Chen, Yujia Wang, Pengze Zhao, Huimin Jiang, Yanchao Zhao, Lingzhi Yang, Liting Yan, Haiyan Wang, Xuebo Zhao

Summary: Defective MOF-808 prepared through a competitive coordination-removal strategy using benzoic acid (HBC) as a modulator showed excellent performance in the conversion of biomass-derived furfural to furfuryl alcohol.
Article Computer Science, Information Systems

Entrepreneurship, Digital Capabilities, and Sustainable Business Model Innovation: A Case Study

Suying Gao, Xiaohui Ma, Xue Zhao

Summary: This article aims to illustrate how entrepreneurship leads to and influences sustainable business model innovation. Through an exploratory single-case study, it is found that innovation spirit, adventure spirit, and co-benefit entrepreneurship have emerged in the digital economy, achieving sustainable business model innovation and multidimensional value creation through the role of digital capabilities.

MOBILE INFORMATION SYSTEMS (2022)

Article Chemistry, Multidisciplinary

Self-Terminating Surface Reconstruction Induced by High-Index Facets of Delafossite for Accelerating Ammonia Oxidation Reaction Involving Lattice Oxygen

Shuo Zhang, Huimin Jiang, Liting Yan, Yanchao Zhao, Lingzhi Yang, Qiuju Fu, Dawei Li, Jun Zhang, Xuebo Zhao

Summary: In this study, ultrasmall delafossite polyhedrons with high-index facets were prepared as pre-catalysts for ammonia electro-oxidation reaction. The high-index CuFeO2 facet facilitated surface reconstruction, resulting in the activation of dehydrogenation steps and an improved electrocatalytic performance. The involvement of lattice oxygen atoms in the dehydrogenation steps as a proton acceptor offers new opportunities for rational designs of ammonia electro-oxidation catalysts.
Article Chemistry, Multidisciplinary

Reticular Coordination Induced Interfacial Interstitial Carbon Atoms on Ni Nanocatalysts for Highly Selective Hydrogenation of Bio-Based Furfural under Facile Conditions

Dandan Liu, Qiuju Fu, Chao Feng, Taisan Xiang, Han Ye, Yuting Shi, Liangjun Li, Pengcheng Dai, Xin Gu, Xuebo Zhao

Summary: A series of Ni catalysts were synthesized by controlled thermal treatment of Ni-based metal-organic frameworks (MOFs) to achieve selective hydrogenation of furfural to tetrahydrofurfuryl alcohol under facile conditions. The catalytic performance of Ni/C catalyst obtained at 400 degrees C showed high conversion of furfural (>99%) and selectivity to tetrahydrofurfuryl alcohol (96.1%), under facile conditions (80 degrees C, 3 MPa H-2, 4.0 h). The decomposition of MOF at low temperatures resulted in highly dispersed Ni-0 particles and interfacial charge transfer, enabling the facile hydrogenation process.

NANOMATERIALS (2023)

Review Chemistry, Multidisciplinary

Recent advances in metal-organic framework based heterogeneous catalysts for furfural hydrogenation reactions

Qiuju Fu, Huimin Jiang, Yujia Wang, Haiyan Wang, Xuebo Zhao

Summary: Metal-organic framework (MOF) based heterogeneous catalysts are widely used in furfural (FFR) hydrogenation reactions. This review summarizes recent advances in upgrading FFR over MOF-based heterogeneous catalysts, ranging from MOFs and MOF derivatives to MOF composites. It also highlights critical issues and perspectives in the hydrogenation of FFR to high-value-added chemicals. This review provides valuable guidance for the preparation and rational design of MOF-based heterogeneous catalysts for upgrading FFR to high value-added chemicals.

MATERIALS CHEMISTRY FRONTIERS (2023)

Article Chemistry, Applied

Highly Selective Separation of C2H2/CO2 and C2H2/C2H4 in an N-Rich Cage-Based Microporous Metal-Organic Framework

Lingzhi Yang, Wenpeng Xie, Qiuju Fu, Liting Yan, Shuo Zhang, Huimin Jiang, Liangjun Li, Xin Gu, Dandan Liu, Pengcheng Dai, Qingbin Zheng, Xuebo Zhao

Summary: In this study, a new material Cd-TZ based on a nitrogen-rich cage-based microporous metal-organic framework (MOF) is reported, which can efficiently separate acetylene from carbon dioxide and ethylene. The gas adsorption experiments and molecular simulation studies reveal that Cd-TZ has a high adsorption capacity and adsorption heat for acetylene, enabling effective separation and purification.

ADSORPTION SCIENCE & TECHNOLOGY (2023)

Review Chemistry, Multidisciplinary

The Adsorptive Separation of Ethylene from C2 Hydrocarbons by Metal-Organic Frameworks

Wenpeng Xie, Lingzhi Yang, Jun Zhang, Xuebo Zhao

Summary: This review summarizes the recent advances in metal-organic frameworks (MOFs) for the separation and purification of C2H4 from the C-2 hydrocarbons, and highlights the mechanisms underlying the separation of C2H4 from the C-2 hydrocarbons using MOFs. The major challenges and developments of MOFs for separating C2H4 from the C-2 hydrocarbons are discussed.

CHEMISTRY-A EUROPEAN JOURNAL (2023)

Article Chemistry, Multidisciplinary

Growth Process of Two-Dimensional Metal-Organic Framework Cu- BDC: A Particle Attachment Crystallization Mechanism Revealed by Microdroplet Flow Reaction

Huimin Jiang, Qiuju Fu, Huimin Liang, Liting Yan, Lingzhi Yang, Ying Wang, Jun Zhang, Xuebo Zhao

Summary: Two-dimensional metal-organic frameworks have been widely studied due to their unique properties. However, the process of crystallization in these frameworks is not well understood. Using the microdroplet flow reaction technique, researchers were able to capture different states of Cu-BDC during crystal growth and uncover a nonclassical crystallization mechanism. The intermediate state product of Cu-BDC nanosheets showed enhanced catalytic performance due to its accessible active sites. This finding can guide the rational design of various 2D MOFs with special structures.

CRYSTAL GROWTH & DESIGN (2023)

Article Biochemistry & Molecular Biology

Metal-Organic Framework Derived Ni2P/FeP@NPC Heterojunction as Stability Bifunctional Electrocatalysts for Large Current Density Water Splitting

Huimin Jiang, Shuo Zhang, Qiuju Fu, Liting Yan, Jun Zhang, Xuebo Zhao

Summary: The construction of heterojunction is a promising approach for developing high-performance non-precious metal-based catalysts for electrochemical water splitting. In this study, a metal-organic framework derived N, P-doped-carbon-encapsulated Ni2P/FeP nanorod with heterojunction was designed and prepared. The results showed that the Ni2P/FeP@NPC catalyst exhibited efficient hydrogen and oxygen evolution reactions, and achieved overall water splitting at industrially relevant high current densities.

MOLECULES (2023)

Article Chemistry, Multidisciplinary

Controllable Exfoliation of MOF-Derived Van Der Waals Superstructure into Ultrathin 2D B/N Co-Doped Porous Carbon Nanosheets: A Superior Catalyst for Ambient Ammonia Electrosynthesis

Liting Yan, Yanchao Zhao, Shuo Zhang, Enyan Guo, Cong Han, Huimin Jiang, Qiuju Fu, Lingzhi Yang, Weijing Niu, Yanlong Xing, Qiuju Zheng, Xuebo Zhao

Summary: A facile and efficient exfoliation strategy was reported to synthesize ultrathin 2D boron and nitrogen co-doped porous carbon nanosheets (B/N-C NS) via a metal-organic framework (MOF)-derived van der Waals superstructure for electrocatalytic nitrogen reduction reaction (NRR) to synthesize NH3. The doping of boron and nitrogen can modulate the electronic structure of the adjacent carbon atoms, promoting the competitive adsorption of nitrogen and reducing the energy required for ammonia synthesis. The B/N-C NS exhibited excellent catalytic performance and stability, with a yield rate of 153.4 μg·h(-1)·mg(-1)cat and a Faraday efficiency of 33.1%, surpassing most reported NRR electrocatalysts.
Article Chemistry, Multidisciplinary

Stress-Dispersed Superstructure of Sn3(PO4)2@PC Derived from Programmable Assembly of Metal-Organic Framework as Long-Life Potassium/Sodium-Ion Batteries Anodes

Huimin Jiang, Shuo Zhang, Liting Yan, Yanlong Xing, Zhichao Zhang, Qiuju Zheng, Jianxing Shen, Xuebo Zhao, Lianzhou Wang

Summary: The structures of anode materials are crucial for their performance in rechargeable batteries. A programmable assembly strategy of metal-organic frameworks (MOFs) is used to construct a Sn-based MOF superstructure precursor, which is then calcinated to obtain Sn-3(PO4)(2)@phosphorus doped carbon (Sn-3(PO4)(2)@PC-48) with improved reversible capacity and low capacity degradation. The optimized electronic structure and stress-dispersed superstructure morphology of Sn-3(PO4)(2)@PC contribute to enhanced electronic conductivity, K+/ Na+ binding ability, and improved structure stabilization.

ADVANCED SCIENCE (2023)

Article Materials Science, Multidisciplinary

A versatile microfluidic strategy using air-liquid segmented flow for continuous and efficient synthesis of metal-organic frameworks

Qiuju Fu, Weijing Niu, Liting Yan, Wenpeng Xie, Huimin Jiang, Shuo Zhang, Lingzhi Yang, Ying Wang, Yanlong Xing, Xuebo Zhao

Summary: Microfluidic synthesis is an advanced method for preparing metal-organic frameworks (MOFs) due to its efficiency in mass/heat transfer and controllable reaction process. However, the post-processing in most liquid-liquid methods is complicated and environmentally burdensome. This study introduces a simple and efficient air-liquid segmented flow method for synthesizing MOFs, resulting in six different MOFs with high crystallinity, yield, and homogeneous morphology compared to traditional solvothermal methods. These prepared MOFs can be applied in various fields such as gas adsorption and catalysis.

MATERIALS LETTERS (2023)

Article Materials Science, Coatings & Films

Effect of micro-arc oxidation on antimicrobial properties and biocompatibility of biomedical Ti-xFe alloys

Yanchun Xie, Xiaodong Wang, Shenshen Cui, Jiali Hu, Yongcun Wei, Yi Lian, Anwu Xuan, Bin Yu, Erlin Zhang

Summary: In this study, Ti-xFe (x = 3,5,9 wt%) alloys were surface modified by micro-arc oxidation (MAO) to improve their antimicrobial properties and biocompatibility. The results showed that increasing the oxidation voltage greatly enhanced the roughness and hydrophilicity of Ti-xFe-MAO alloys. The Ti-xFe alloys micro-arc oxidized at 250 V and 300 V exhibited improved corrosion resistance and excellent antimicrobial and cytocompatibility properties, making them suitable for orthopedic implant materials.

SURFACE & COATINGS TECHNOLOGY (2024)

Article Materials Science, Coatings & Films

Fabrication of ultra-low porosity plasma electrolytic oxidation coating on Ta-12W alloys and its formation mechanism

Yuting Hao, Zuoyan Ye, Lili Wang, Minheng Ye, Hui Dong, Chao Wang, Yunchen Du

Summary: This study focuses on the modification of PEO coatings on Ta-12W alloy using NH4F additive. The results show that ultra-low porosity coatings can be prepared by optimizing the NH4F content. The formation process of specific structures on the coating surface is discussed, and the effects of NH4F concentration and treatment duration on coating characteristics are investigated.

SURFACE & COATINGS TECHNOLOGY (2024)

Article Materials Science, Coatings & Films

Pulsed laser cladding on IN718 alloy using pre-coated CrCoNi-TiC/SiC powders for enhancing wear resistance

Yuanzhuo Liu, Linjiang Chai, Tao Yang, Chaodan Hu, Chuanmei Wang, Guoqiang Xi

Summary: By employing a pulsed laser, laser cladding was performed on IN718 alloy pre-coated with CrCoNi-TiC/SiC powders and three defect-free coatings were successfully prepared. The addition of TiC and SiC powders generated fine carbides dispersed in the coatings and led to changes in grain and substructure morphologies, resulting in increased hardness and wear resistance.

SURFACE & COATINGS TECHNOLOGY (2024)

Article Materials Science, Coatings & Films

Growth of Nb films on Cu for superconducting radio frequency cavities by direct current and high power impulse magnetron sputtering: A molecular dynamics and experimental study

M. Ghaemi, A. Lopez-Cazalilla, K. Sarakinos, G. J. Rosaz, C. P. A. Carlos, S. Leith, S. Calatroni, M. Himmerlich, F. Djurabekova

Summary: The use of high-power impulse magnetron sputtering can result in dense and uniform niobium films on all surfaces of superconducting rf cavities, as simulated and investigated in this study.

SURFACE & COATINGS TECHNOLOGY (2024)

Article Materials Science, Coatings & Films

Electrophoretic coating of magnesium oxide on microarc-oxidized titanium and characterization of in vitro antibacterial activity and biocompatibility

Jiaheng Du, Xinli Fan, Dongqin Xiao, Wuxiang Wang, Yiran Yin, Zhong Li, Kui He, Yanfei Tan, Jiyuan Yan, Gangli Liu, Ke Duan

Summary: This study investigated the electrophoretic deposition (EPD) of magnesium oxide (MgO) coatings on micro-arc oxidized titanium (MAO-Ti) and evaluated their in vitro antibacterial properties and biocompatibility. The results showed that MgO coatings significantly reduced bacterial numbers and biofilm formation, while also demonstrating good cytocompatibility and induction of osteoblast mineralization.

SURFACE & COATINGS TECHNOLOGY (2024)

Article Materials Science, Coatings & Films

Enhancing the fretting damage resistance of suspension plasma sprayed hydroxyapatite coating with Titania addition

Samiksha Moharana, Yuichi Otsuka, R. Gnanamoorthy

Summary: The addition of titania to HAp coatings improves their wear resistance and reduces damage to titanium implants caused by debris generation. This study evaluates the fretting wear resistance of titania-added HAp suspension plasma spray coating and finds that it exhibits reduced friction coefficient and increased wear resistance.

SURFACE & COATINGS TECHNOLOGY (2024)

Article Materials Science, Coatings & Films

Potentiostatic preparation and in vitro characterization of functional hazenite conversion coatings on AZ31 magnesium alloy

Li-Ping Wu

Summary: The functional hazenite coating deposited on AZ31 Mg alloy showed improved roughness and hydrophilicity, enhanced biocompatibility, reduced degradation rate, and decreased susceptibility to stress corrosion cracking.

SURFACE & COATINGS TECHNOLOGY (2024)

Article Materials Science, Coatings & Films

Long-lasting anti-bacterial face masks enabled by combining anti-bacterial materials and superhydrophobic coating

Ning Tian, Delei Xu, Jinfei Wei, Bucheng Li, Junping Zhang

Summary: This study reports the preparation of a superhydrophobic and anti-bacterial fabric for face masks. The fabric exhibits high superhydrophobicity and excellent moisture resistance, enabling functionality effectiveness in cold weather conditions. The fabric also demonstrates remarkable anti-bacterial activity against E. coli, attributed to the synergistic effect of superhydrophobicity and embedded ZnO nanoparticles. This superhydrophobic anti-bacterial fabric holds great potential for various practical applications in personal protective equipment, healthcare, and disease prevention.

SURFACE & COATINGS TECHNOLOGY (2024)

Article Materials Science, Coatings & Films

Aluminide diffusion coatings for improving the pesting behavior of refractory metals

Katharina Beck, Anke S. Ulrich, Andreas K. Czerny, Emma M. H. White, Martin Heilmaier, Mathias C. Galetz

Summary: Refractory metal based alloys have great potential as structural materials for high-temperature applications due to their high melting points. However, they are prone to catastrophic oxidation at around 700 degrees C. This study investigated the effect of aluminium diffusion coatings on the oxidation resistance of pure molybdenum, niobium, tantalum, and tungsten. The results showed that the aluminization improved the oxidation behavior and decreased the oxide growth rate for molybdenum and tantalum.

SURFACE & COATINGS TECHNOLOGY (2024)

Article Materials Science, Coatings & Films

Preparation and characterization of La-doped Y3Al5O12 as a potential protective coating material against CMAS corrosion

Wenwen Shuai, Haijun Dou, Zhichen Guan, Wei Qian, Zhibao Li, Yinqun Hua, Jie Cai

Summary: This study synthesized (Y1-xLax)3Al5O12 (x = 0, 0.1, 0.2, 0.3) materials by doping lanthanum ions, and found that the doped materials exhibited improved mechanical properties and thermal expansion coefficient, as well as enhanced resistance to CMAS corrosion. These materials have potential applications.

SURFACE & COATINGS TECHNOLOGY (2024)

Article Materials Science, Coatings & Films

Microstructural, mechanical and corrosion characterization of (C-HA)SiCnws coating on AZ31 magnesium alloy surface

Xianglei Liu, Jiahui Ding, Wanbo Hou, Xinhao Shi, Tao Feng, Xiangyuan Meng, Shifeng Wen, Mingde Tong, Zhufeng Yue

Summary: A composite coating was developed to improve the adhesion, wear resistance, and corrosion resistance, which exhibited significant enhancements in these properties.

SURFACE & COATINGS TECHNOLOGY (2024)

Article Materials Science, Coatings & Films

Mechanism study of composite co-deposited Cu/Co-Mo corrosion-resistant coating on 6061 Al alloy

Hongxuan Xing, Jidong Li, Xianwei Hu, Liang Tian, Renyun Zhang, Yiyong Wang

Summary: By depositing a Cu/Co-Mo corrosion-resistant plating layer on the surface of 6061 Al alloy, the bonding strength between the alloy and the plating layer can be improved and the corrosion resistance can be enhanced. The composite coating forms an obvious three-layer structure with Co-Mo coating exhibiting amorphous characteristics and Co3Mo phase composition. The composite coating improves the corrosion resistance and hardness of the substrate, effectively protecting the 6061 Al alloy.

SURFACE & COATINGS TECHNOLOGY (2024)

Article Materials Science, Coatings & Films

The impact-corrosion behavior of HVAF-sprayed monolayer and hierarchical Fe-based amorphous coatings

Fan Yang, Debin Wang, Tianrun Li, Baijun Yang, Suode Zhang, Jianqiang Wang

Summary: The impact-corrosion behavior of monolayer and hierarchical Fe-based amorphous coatings fabricated by HVAF was investigated in 3.5 wt% NaCl solution. The monolayer coating exhibits corrosion failure with increased impact energy, while the hierarchical coating shows improved resistance. However, at high impact energies, both coatings experience corrosion degradation.

SURFACE & COATINGS TECHNOLOGY (2024)

Article Materials Science, Coatings & Films

Modified Ni-Al layer double hydroxides as nanoparticles for self-healing anti-corrosion composite coating

Shoaib Ahmad, Muddasir Nawaz, Solaiman Mohammad, R. A. Shakoor, Ramazan Kahraman, Talal Mohammed Al Tahtamouni

Summary: This research presents a novel self-healing anti-corrosion composite coating that demonstrates higher inhibition efficiency and self-healing effect, providing protection for metallic structures against corrosive environments.

SURFACE & COATINGS TECHNOLOGY (2024)

Article Materials Science, Coatings & Films

Effects of silicon and neodymium additions on microstructures and mechanical properties of CoCrNi medium entropy alloy films

Hui-Wen Peng, Chun-Hway Hsueh

Summary: A series of (CoCrNi)100-x-ySixNdy medium entropy alloy films with manipulated metalloid element, Si, and rare earth element, Nd, were synthesized using magnetron three-target co-sputtering. The films showed different structures and mechanical properties with varying Si and Nd contents. The optimized mechanical properties were observed in the film with Si0.61Nd5.14, attributed to precipitation strengthening and grain refinement.

SURFACE & COATINGS TECHNOLOGY (2024)