期刊
ORGANIC LETTERS
卷 22, 期 11, 页码 4222-4227出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.0c01270
关键词
-
资金
- King Abdullah University of Science and Technology (KAUST), Saudi Arabia, Office of Sponsored Research [FCC/1/1974]
The first base metal-catalyzed regioselective dehydrogenative alkylation of indolines using readily available alcohols as the alkylating reagent is reported. A single air- and moisturestable manganese catalyst provides access to either C-3- or N-alkylated indoles depending on the solvent used. Mechanistic studies indicate that the reaction takes place through a combined acceptorless dehydrogenation and hydrogen autotransfer strategy.
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