期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 142, 期 22, 页码 9890-9895出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.0c02121
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资金
- National Research Foundation of Korea (NRF) - Korean government [2011-0018355]
- National Research Foundation of Korea [2011-0018355] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
Described herein is the first iridium-catalyzed cyclative indenylation through sequential B(4)-C and intramolecular C-C bond formation from o-carboranes and propargyl alcohols, leading to the formation of B(4)-indenylated o-carboranes with excellent regioselectivity via direct B-H activation. Moreover, the iridium-catalyzed regioselective 1,3-dienylation has been accessed through sequential B-H activation, dehydration, and decarboxylation, producing B(4)-dienylated o-carboranes.
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