期刊
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
卷 11, 期 11, 页码 4524-4529出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.jpclett.0c00748
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资金
- National Natural Science Foundation of China [61875002]
- National Key R&D Program of China [2018YFA0306302]
- Beijing Natural Science Foundation [Z190005]
Distribution of the transition dipole moments (TDMs) of light emitters can intrinsically affect the light out-coupling efficiency of planar light-emitting diodes (LEDs). Lacking the control of TDM distribution has limited the efficiency of nanocrystal-based LEDs to 20%. Her; we present a method that deposits uniform nanocrystal films with unity in-plane TDM distribution. Combining an inkjet printing technique and colloidal nanocrystal self-assembly, we achieved direct printing and in situ assembly of colloidal CdSe/CdS nanoplatelets to all orient face-down on various substrates. With motorized translation stages, pattern printing is realized, which demonstrates the potential for integration in industrial-scale fabrication. The method is applied to achieve uniform nanoplatelet films with unity in-plane TDM distribution on zinc-oxide films, a commonly used electron-transport layer. Thus, our work paves the way to break the light out-coupling efficiency limitation of 20% in state-of-the-art nanocrystal-based LEDs, which exclusively possess an isotropic TDM distribution.
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