期刊
CHEMICAL COMMUNICATIONS
卷 52, 期 50, 页码 7826-7829出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cc03787a
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资金
- Royal Society of Chemistry
- University of Bath
- H2FC SUPERGEN Hub [EP/E040071/1]
- Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]
- EPSRC [EP/E040071/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/E040071/1] Funding Source: researchfish
Three highly porous Zr(IV)-based metal-organic frameworks, UBMOF-8, UBMOF-9, and UBMOF-31, were synthesized by using 2,2'-diamino-4,4'- stilbenedicarboxylic acid, 4,4'-stilbenedicarboxylic acid, and combination of both linkers, respectively. The mixed-linker UBMOF-31 showed excellent hydrogen uptake of 4.9 wt% and high selectivity for adsorption of CO2 over N-2 with high thermal stability and moderate water stability with permanent porosity and surface area of 2552 m(2) g(-1).
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