期刊
EUROPEAN POLYMER JOURNAL
卷 134, 期 -, 页码 -出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.eurpolymj.2020.109803
关键词
Microfibrillated lignocellulose; Surface modification; Acetylation; Biocomposites; Polylactic acid
资金
- Republic of Turkey - Ministry of National Education
- Turkish Forestry Service
High hemicellulose and lignin content MFC (MFLC) was isolated from chemi-thermomechanical pulp (CTMP), and surface acetylation used to significantly decrease its polarity. This modification of MFLC provided good dispersibility in PLA when used for biocomposites fabrication via a solvent casting method. MFLC exhibited higher modification efficiency compared to lignin-free MFC. Base-catalysed surface acetylation unchanged the crystalline structure of MFLC. Detection of the hydrogen bond between acetylated MFLC (Ac-MFLC) and PLA confirmed its role in improvement of the mechanical performance, thermal properties and crystallinity of the biocomposite with Ac-MFLC acting as an effective reinforcing and nucleating agent. The approach confirms the suitability of surface functionalization of MFLC for fabrication of biocomposites for a wide range of applications such as packaging and biomedical products.
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