期刊
APPLIED SURFACE SCIENCE
卷 512, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.apsusc.2020.145602
关键词
Mixed Metal Oxides; Soot oxidation; Oxygen vacancy; Durability; Mechanism
类别
资金
- China Science and Technology Exchange Center [2016YFE0126600]
- National Key R&D Program of China [2017YFC0211102]
- National Engineering Laboratory for Mobile Source Emission Control Technology [NELMS2017A13]
A series of flower-like CuxMnyCez mixed oxides catalysts for soot removal were prepared via a facile co-precipitation approach followed by calcination. The structural and surface properties of these catalysts were investigated by powder X-ray diffraction, N-2 physisorption, transmission electron microscopy, scanning electron microscopy, X-ray photoelectron spectroscopy, hydrogen temperature-programmed reduction, oxygen temperature-programmed desorption and NO temperature-programmed oxidation. Superior soot oxidation performance was obtained over these ternary mixed oxides catalysts and the corresponding mechanism was explored. In particular, the Cu1Mn1Ce1 catalyst showed a remarkable improvement in soot oxidation activity in both NO + O-2 and O-2 atmospheres. The reusability and durability of these catalysts were assessed, and these materials showed high soot oxidation activity after the hydrothermal stability test.
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