4.7 Article

A novel visible light controllable adsorption-desorption system with a magnetic recyclable adsorbent

期刊

SCIENCE OF THE TOTAL ENVIRONMENT
卷 707, 期 -, 页码 -

出版社

ELSEVIER
DOI: 10.1016/j.scitotenv.2019.136025

关键词

Adsorbent; Photo-induced desorption; Magnetism; Recyclability

资金

  1. National Natural Science Foundation of China [21677040, 21377031]
  2. Natural Science Foundation of Henan Province [182300410121]
  3. Technology Department of the Henan Science and Technology Fund Project [172102310465]

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Convenient and energy-efficient desorption or regeneration processes are prerequisites for the development of an ideal adsorbent. For this work, a novelmagnetic adsorbent (citric acid/Bi2O2CO3/Fe3O4) was controllably synthesized via a facile hydrothermalmethod. The as-prepared materials demonstrated the excellent adsorption of methylene blue (MB), where similar to 70% of the MB was absorbed within 10 min. Interestingly, the desorption process could be triggered by visible light irradiation, and 99% of the absorbed MB was released into solution within 4 h. Further, the magnetic materials could be conveniently recovered using a magnet and regenerated via a model hydrothermal process. Even after two regeneration cycles, approximately 60% adsorption and 63% desorption abilities were retained, which suggested strong potential for the recyclability of these materials. (C) 2019 Elsevier B.V. All rights reserved.

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