期刊
OPTIK
卷 204, 期 -, 页码 -出版社
ELSEVIER GMBH
DOI: 10.1016/j.ijleo.2019.164131
关键词
Semiconductor photocatalysts; ZnO; Ce doping; ZnO-Graphene; Flower-like; Organic dyes; Photocatalytic activity
类别
资金
- Key scientific research project of the university scientific research plan in Xinjiang Uygur Autonomous Region [XJEDU2016I018]
- National Natural Science Foundation of China [11764040]
- Natural Science Foundation of Xinjiang Uygur Autonomous Region [2017D01C022]
Semiconductor photocatalysts have played an important role in degrading water pollution in recent years. In this paper, the effects of graphene on the structure, morphology, optical properties and photocatalytic activity of ZnO and Ce-doped ZnO were studied. The photocatalysts of ZnO, Ce doped ZnO (ZnCeO), ZnO-Graphene (ZG), Ce doped ZnO-Graphene (ZGCeO) were synthesized via one-step hydrothermal method and were characterized by X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), scanning electron microscopy (SEM), ultraviolet visible absorption (UV-vis). The results of XRD show the synthesized samples were all ZnO phases without impurity peaks. The prepared ZnO was hexagonal wurtzite crystal structure. A flower-like ZG and an approximate flower-like ZGCeO were characterized via SEM. The UV-vis spectra shows that the absorption edges have red-shifts and the absorption band broaden in all doped or composite samples, meanwhile, the band gap energy decreased from 3.26 eV to 3.06 eV. In addition, compared with pure ZnO, the photocatalytic activity of ZnCeO, ZG and ZGCeO are improved. Among them, ZGCeO shows superior photocatalytic activity: the degradation rate of organic dye MB was 99.17 % in 90 min under simulated solar irradiation.
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