Review
Green & Sustainable Science & Technology
Rishabh Sharma, Miroslav Almasi, Satya Pal Nehra, Vikrant Singh Rao, Priyanka Panchal, Devina Rattan Paul, Indra Prabh Jain, Anshu Sharma
Summary: The exponentially increasing population leads to high energy demands and resource utilization, making the earth an unsustainable habitat. Utilizing renewable energy for water splitting and hydrogen generation can reduce carbon footprint and satisfy energy demands. However, existing photocatalysts still face challenges in terms of activity and stability.
RENEWABLE & SUSTAINABLE ENERGY REVIEWS
(2022)
Article
Environmental Sciences
Tae-Gyu Lee, Hui-Ju Kang, Gazi A. K. M. Rafiqul Bari, Jae-Woo Park, Hye-Won Seo, Byeong-Hyeon An, Hyun Jin Hwang, Young-Si Jun
Summary: This study develops monodisperse organic single-crystal monoliths with controllable dimensions, which are transformed into g-CN by thermal polycondensation, showcasing the potential to efficiently produce hydrogen via photoreforming. The dimensional tunability of the photocatalysts enables tailored catalytic activity for practical use and the formation of value-added products without compromising photocatalytic effectiveness in wastewater treatment.
Article
Chemistry, Physical
Yuepeng Liu, Shuo Zhao, Chao Zhang, Jiasheng Fang, Liying Xie, Yuming Zhou, Shuping Zhuo
Summary: The study demonstrates the enhancement of photocatalytic performance of carbon nitride through carbon doping and hollow tubular structure, leading to a significant increase in hydrogen evolution rate. The carbon content has a significant impact on the structure and photocatalytic activity of carbon nitride, while the hollow tubular structure can increase the specific surface area and visible light absorption capacity.
Article
Energy & Fuels
Amir Al-Ahmed
Summary: Global warming and environmental issues are driving the adoption of clean energy sources, with hydrogen being considered one of the most promising options. Photocatalytic water splitting using graphitic carbon nitride has been shown to be a cost-effective approach with potential for high performance.
Article
Chemistry, Multidisciplinary
Arindam Indra, Rodrigo Beltran-Suito, Marco Mueller, Ramesh P. Sivasankaran, Michael Schwarze, Amitava Acharjya, Bapi Pradhan, Johan Hofkens, Angelika Brueckner, Arne Thomas, Prashanth W. Menezes, Matthias Driess
Summary: The study investigated the dynamics of hole transfer from Pt-loaded sol-gel-prepared graphitic carbon nitride photocatalyst, using different adsorbed hole acceptors and a sacrificial agent. A significant increase in H-2 production was achieved by employing phenothiazine as the hole acceptor, with continuous H-2 production for 3 days. The charge-transfer dynamics of the photocatalytic process in the presence of hole acceptors were examined through time-resolved photoluminescence and in situ electron paramagnetic resonance studies.
Article
Chemistry, Multidisciplinary
Jinghua Li, Lunqiao Xiong, Bing Luo, Dengwei Jing, Jiamei Cao, Junwang Tang
Summary: A novel hybrid photocatalyst composed of NCS and CN has been prepared, showing efficient photocatalytic performance by promoting photoelectron transfer through a special coupling interface, which significantly improves the photocatalytic efficiency.
CHEMISTRY-A EUROPEAN JOURNAL
(2021)
Article
Chemistry, Physical
Lu Chen, Shangbo Ning, Ruowen Liang, Yuzhou Xia, Renkun Huang, Guiyang Yan, Xuxu Wang
Summary: Controlling the structure of semiconductors is crucial for tailoring their physicochemical and photoelectronic properties. Graphitic carbon nitride has shown potential in photocatalysis, but its photocatalytic activity is limited by the rapid recombination of charge carriers. In this study, we demonstrate that introducing potassium doping and nitrogen defects into graphitic carbon nitride can enhance visible light absorption, improve charge separation, and significantly enhance the photocatalytic behavior for water splitting.
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2022)
Article
Chemistry, Physical
Songcan Wang, Xin Wang, Boyan Liu, Xiong Xiao, Lianzhou Wang, Wei Huang
Summary: The electronic structure of graphitic carbon nitride (g-C3N4) was tailored through a KOH-assisted sealed heating process, resulting in a significantly enhanced and stable photocatalytic hydrogen production rate and high apparent quantum efficiency. The introduction of more cyano groups during the heating process promoted charge separation and transfer, improving the photocatalytic performance.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2022)
Review
Materials Science, Multidisciplinary
Ping Niu, Junjing Dai, Xiaojuan Zhi, Zhonghui Xia, Shulan Wang, Li Li
Summary: Graphitic carbon nitride (GCN) has shown great potential as a photocatalyst for overall water splitting, with breakthrough progress being made in this dynamic research field. Modulating the activity of GCN can lead to more efficient photocatalytic water splitting, offering new ideas and methods for the design of advanced photocatalysts in the future.
Article
Chemistry, Physical
Yanping Liu, Wen Yin, Qingyun Lin, Zhigang Li, Wenwu Zhong, Baizeng Fang
Summary: Defect engineering has been proven to be a powerful strategy for enhancing the photocatalytic performance of materials. In this study, tri-coordinated nitrogen vacancies-modified graphitic carbon nitride (Nv-GCN) was successfully synthesized through a simple sintering process. The optimized Nv-GCN showed significantly improved photocatalytic hydrogen production under visible light irradiation compared to the pristine GCN. The nitrogen vacancies in Nv-GCN provided more active sites, modulated the electronic structure, and accelerated the separation and transfer of photogenerated charges. This study provides an effective route for designing high-performance photocatalysts for efficient conversion of solar energy.
APPLIED SURFACE SCIENCE
(2023)
Article
Chemistry, Physical
Lei Luo, Keran Wang, Zhuyu Gong, Haixing Zhu, Jiani Ma, Lunqiao Xiong, Junwang Tang
Summary: Introducing bridging nitrogen defects significantly enhances the photocatalytic hydrogen production performance of graphitic carbon nitride nanosheets, with an increase in hydrogen evolution rate of approximately 10-41 times compared to pristine nanosheets and bulk carbon nitride.
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2021)
Article
Chemistry, Physical
Jingzhen Zhang, Junyu Lang, Yan Wei, Qian Zheng, Liyan Liu, Yun-Hang Hu, Baoxue Zhou, Congli Yuan, Mingce Long
Summary: Efficient photocatalytic production of H2O2 in pure water was achieved by decorating graphitic carbon nitride with oxidative red phosphorus, leading to significant enhancement of H2O2 generation compared to pristine GCN. The strategy of utilizing red phosphorus for promoting charge separation while suppressing H2O2 decomposition opens up a new pathway for designing highly active metal-free photocatalysts for solar-to-H2O2 conversion in pure water.
APPLIED CATALYSIS B-ENVIRONMENTAL
(2021)
Article
Engineering, Chemical
M. Alejandra Quintana, Rafael R. Solis, M. Angeles Martin-Lara, Gabriel Blazquez, F. Monica Calero, Mario J. Munoz-Batisa
Summary: This study proposes the use of boron to modify the structure of graphitic carbon nitride, enhancing its photocatalytic activity. The choice of boron precursor affects the positions at which boron atoms replace carbon and nitrogen in the structure, leading to significant effects on photocatalytic activity. Specifically, the sample modified with NaBH4 shows the highest oxidation rate and selectivity.
SEPARATION AND PURIFICATION TECHNOLOGY
(2022)
Article
Chemistry, Physical
Miao Ren, Xueyan Zhang, Yunqing Liu, Guang Yang, Lang Qin, Jiaqi Meng, Yihang Guo, Yuxin Yang
Summary: In this study, a palladium-single-atom-coordinated cyano-group-rich g-C3N4 (Pd/D-N-UCN) was synthesized to improve the photocatalytic hydrogen evolution activity. The formation mechanism of Pd single atoms on g-C3N4 nanosheets and the coordination bonding of cyano groups with Pd atoms were proposed. The synthesized 0.16%Pd/D-N-UCN exhibited enhanced photocatalytic hydrogen production activity compared to electrostatically stabilized Pd single atoms.
Article
Engineering, Environmental
Yanlin Zhu, Yanyan Sun, Javid Khan, Heng Liu, Guangling He, Xuetao Liu, Jiamin Xiao, Haijiao Xie, Lei Han
Summary: Graphitic carbon nitride (g-C3N4) has promising potential in photocatalytic production of hydrogen peroxide (H2O2) due to its suitable band structure and facile preparation. In this study, sodium doping and cyano groups with nitrogen vacancies were introduced into g-C3N4 by NaClO-assisted ammonia pyrolysis, leading to improved light absorption and separation efficiency of photo-generated electrons and holes, resulting in high H2O2 yield and excellent cyclic stability.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Materials Science, Multidisciplinary
Wei Tang, Liuping Xie, Zhixin Liu, Jie Zeng, Xuan Zhou, Pengqing Bi, Wencheng Tang, Lei Yan, Wai-Kwok Wong, Xunjin Zhu, Xiaotao Hao, Weiguo Zhu, Xingzhu Wang
Summary: The development of intermediate-sized acceptor-pi-porphyrin-pi-acceptor-type molecules MPor1 and MPor2 with panchromatic absorption profiles aims to enhance photovoltaic performance. These molecules successfully bridge the absorption gap between conventional porphyrin molecules, resulting in narrow optical bandgaps and demonstrating excellent light-harvesting properties and efficient charge separation. Solar cells utilizing MPor1/PC71BM active layer exhibit optimal performance with a power conversion efficiency of 8.59% and a short circuit current of 14.91 mA cm(-2).
JOURNAL OF MATERIALS CHEMISTRY C
(2022)
Article
Energy & Fuels
Venkatesh Piradi, Xiaopeng Xu, Hang Yin, Johnny Ka Wai Ho, Feng Yan, Qiang Peng, Shu Kong So, Xunjin Zhu
Summary: Two acceptor-donor-acceptor-based porphyrin dimers, C8TEBDT-2P and C8TBDT-2P, are presented as donors for high-performance semitransparent indoor organic photovoltaics. C8TEBDT-2P exhibits a more red-shifted absorption profile and higher power conversion efficiency, enriching the pool of porphyrin donors for such applications.
Article
Chemistry, Physical
Yang Li, Lingling Li, Suyang She, Shi Chen, Yanliang Liu, Baomin Xu, Fu-Wa Lee, Xunjin Zhu
Summary: A simple and efficient method was applied to prepare multidimensional perovskite with enhanced performance, demonstrating higher charge transfer ability and improved photocatalytic efficiency compared to traditional 3D and 2D perovskite materials.
ACS APPLIED ENERGY MATERIALS
(2022)
Review
Chemistry, Inorganic & Nuclear
Daniel Nnaemaka Tritton, Fung-Kit Tang, Govardhana Babu Bodedla, Fu-Wa Lee, Chak-Shing Kwan, Ken Cham-Fai Leung, Xunjin Zhu, Wai-Yeung Wong
Summary: This review surveys the design and evaluation of organometallic compounds based on iridium(III) and relevant metal complexes as photocatalysts/photosensitizers in systems for photocatalytic hydrogen evolution reactions. The photo-redox mechanisms and structure-catalytic activity relationships are discussed to guide future design of more efficient and robust photocatalytic systems.
COORDINATION CHEMISTRY REVIEWS
(2022)
Article
Engineering, Environmental
Jiamin Xu, Jiabang Chen, Shi Chen, Han Gao, Yaru Li, Zhengyan Jiang, Yong Zhang, Xingzhu Wang, Xunjin Zhu, Baomin Xu
Summary: Organic spacers can enhance the stability of RPP materials, but limit their performance. Binary spacer-based RPP devices show great potential. By introducing guanidinium, the film properties and device performance can be improved, resulting in higher efficiency and long-term stability of solar cells.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Chemistry, Physical
Govardhana Babu Bodedla, Venkatesh Piradi, Muhammad Imran, Jianzhang Zhao, Xunjin Zhu, Wai-Yeung Wong
Summary: In this study, two new A-pi-D-pi-A porphyrins, ZnP-CPDT and ZnP-BT, were synthesized and characterized as visible-to-near-infrared light-harvesting photosensitizers. The porphyrins exhibited absorption in the range of 370 to 800 nm in solution and 300 to 1100 nm in the solid state. The Soret- and Q-band absorption peaks of ZnP-CPDT were more red-shifted than those of ZnP-BT due to enhanced intramolecular charge transfer. Additionally, ZnP-CPDT showed better photoinduced charge separation and well-defined nanosphere morphology, resulting in a higher photocatalytic hydrogen evolution rate compared to ZnP-BT and a typical zinc(ii)-tetraphenylporphyrin.
JOURNAL OF MATERIALS CHEMISTRY A
(2023)
Article
Chemistry, Multidisciplinary
Chao Wang, Yuzhuo Chen, Daijian Su, Wai-Lun Man, Kai-Chung Lau, Lianhuan Han, Liubin Zhao, Dongping Zhan, Xunjin Zhu
Summary: A new molecular electrocatalyst with highly dispersed CoN4 sites was synthesized for CO2 reduction reaction. The catalyst shortens the electron transfer pathway, accelerates the redox kinetics, and improves durability. Experimental results showed that it achieved high current density and CO conversion rate in commercial flow cells.
ADVANCED MATERIALS
(2023)
Article
Chemistry, Physical
Venkatesh Piradi, Guitao Feng, Muhammad Imran, Jianzhang Zhao, Feng Yan, Xunjin Zhu
Summary: Porphyrins are highly adaptable materials for organic photovoltaics due to their adjustable functional groups. In this study, two porphyrin-based small molecule donors, IDT-2TPE and TPE, were synthesized. The device based on the IDT-2TPE donor and IDTCR nonfullerene acceptor showed a broad photoelectron response up to 1000 nm and a power conversion efficiency of 10.41%, while the device based on the TPE donor and IDTCR acceptor had a much lower efficiency of 4.22%. The improved performance of the IDT-2TPE/IDTCR device was attributed to its higher photocurrent generation and more favorable surface morphology with elevated charge carrier mobilities.
ACS APPLIED ENERGY MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Govardhana Babu Bodedla, Muhammad Imran, Jianzhang Zhao, Xunjin Zhu, Wai-Yeung Wong
Summary: In this study, TPE-ZnPF was successfully synthesized and characterized by single-crystal X-ray diffraction. TPE-ZnPF aggregates exhibit long-lived photoexcited states, and enhance emission intensity through suppression of non-radiative decay channels. Moreover, TPE-ZnPF aggregates show more efficient light-harvesting ability, well-defined nanosphere morphology, and more efficient photoinduced charge separation compared to Ph-ZnPF aggregates. As a result, TPE-ZnPF aggregates demonstrate an excellent photocatalytic hydrogen evolution rate of 56.20 mmol g(-1) h(-1), which is 94-fold higher than that of Ph-ZnPF aggregates without TPE groups.
Article
Materials Science, Multidisciplinary
He Jiang, Hanlin Li, Jibiao Jin, Govardhana Babu Bodedla, Peng Tao, Dongge Ma, Wai-Yeung Wong
Summary: We designed and synthesized two novel deep-blue emitters based on anthracene and pyrene moieties for highly efficient TTA-based OLEDs. The twisted conformation of the molecules effectively interrupted p-conjugation, resulting in intense deep-blue emission with high photoluminescence quantum yields. The deep-blue OLEDs using these emitters achieved maximum external quantum efficiencies of 4.78% and 5.48% with excellent color purity.
JOURNAL OF MATERIALS CHEMISTRY C
(2023)
Review
Chemistry, Multidisciplinary
Govardhana Babu Bodedla, Xunjin Zhu, Wai-Yeung Wong
Summary: One major obstacle in porphyrins is aggregation-caused quenching (ACQ), which leads to nonradiative deactivation of photoexcited states and low photoluminescence and singlet quantum yields. This limits the use of porphyrins in various applications. However, by introducing aggregation-induced emission (AIE) features into porphyrins, their ACQ properties can be transformed and their performance in these applications can be enhanced.
Article
Chemistry, Multidisciplinary
Chao Wang, Yuzhuo Chen, Daijian Su, Wai-Lun Man, Kai-Chung Lau, Lianhuan Han, Liubin Zhao, Dongping Zhan, Xunjin Zhu
Summary: The new electrocatalyst EP-CoP shows improved efficiency and durability in CO2 reduction reactions by enhancing the dispersion of CoN4 sites and optimizing redox kinetics. In commercial flow cells, EP-CoP demonstrates excellent catalytic performance under various overpotential conditions.
ADVANCED MATERIALS
(2023)
Article
Chemistry, Physical
Qi-Wen Chen, Ze-Qing Guo, Jian-Ping Zhou
Summary: Multifunctional continuous solid solutions NFMTO-x were successfully synthesized via a one-step hydrothermal method by controlling the ratio of Mg and Fe. The NFMTO-x materials exhibited enhanced visible light response, effective adsorption and photocatalytic degradation of organic pollutants, CO2 methanation capability, and easy recyclability due to their magnetic properties. This research provides a significant multifunctional material for water purification.
APPLIED SURFACE SCIENCE
(2024)
Review
Chemistry, Physical
George E. Stan, Maziar Montazerian, Adam Shearer, Bryan W. Stuart, Francesco Baino, John C. Mauro, Jose M. F. Ferreira
Summary: Bioactive glasses have the ability to form strong bonds with tissues and release therapeutic ions. However, their biomechanical compatibility limits their use in load-bearing applications. The use of magnetron sputtering technology to fabricate BG coatings shows promise in improving their efficacy and potential for application.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Zhaoxuan Wang, Zhicheng Yan, Zhigang Qi, Yu Feng, Qi Chen, Ziqi Song, Meng Huang, Peng Jia, Ki Buem Kim, Weimin Wang
Summary: The corrosion behavior of Fe-60 and Fe-83 ribbons in 0.6 M NaCl was studied. Fe-60 exhibited a local corrosion mode and formed a stable passivation film with higher corrosion resistance, while Fe-83 showed a combination of local and global corrosion modes and had lower corrosion resistance. Controlling the precipitation of nanocrystalline phases and increasing the POx content in the passivation film significantly improved the corrosion resistance of Fe-based glassy alloys.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Hao-Kai Peng, Sheng-Yen Zheng, Wei-Ning Kao, Ting-Chieh Lai, Kai-Sheun Lee, Yung- Hsien Wu
Summary: This study investigates the effects of high energy/fluence proton radiation on the performance of HfZrOx-based FeFETs memory with different Zr content. The results show that the characteristics of FeFETs are influenced by proton radiation, and the extent of the influence depends on the Zr content. FeFETs with 50% Zr content exhibit minimal changes in memory window and demonstrate good endurance and retention performance.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Zongyi Yue, Guangyi Wang, Zengguang Huang, Sihua Zhong
Summary: In this study, AZO and ITO films were successfully tuned as excellent passivation layers for c-Si surfaces, achieving effective minority carrier lifetime and outstanding optical properties through the optimization of annealing temperature and interfacial silicon oxide.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Martin Hruska, Jan Kejzlar, Jaroslav Otta, Premysl Fitl, Michal Novotny, Jakub Cizek, Oksana Melikhova, Matej Micusik, Peter Machata, Martin Vrnata
Summary: This paper presents a detailed study on the hydrogen sensing capabilities of highly nanoporous black gold films. The films exhibit fast response and recovery times at low temperatures. Different levels of nanoporosity were prepared and tested to investigate the sensing properties, and it was found that nanoporous black gold is suitable for hydrogen sensing. The sensitivity of the film depends on its nanoporosity.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Yupu Wang, Gaofeng Teng, Chun To Yiu, Junyi Zhu
Summary: In the study of BM-SCO and HSCO thin films, it was found that H vacancies tend to prefer sites near the external surface or oxygen vacancy channels (OVCs), while H interstitials prefer sites of oxygen on a layer that contains six-fold coordinated Co. These findings not only enrich the understanding of complex surface phenomena of defect formation but also provide an explanation for the reversibility during phase transformation.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Jiafeng Lu, Linping Teng, Qinxiao Zhai, Chunhua Wang, Matthieu Lancry, Ye Dai, Xianglong Zeng
Summary: In this study, we achieved full control of fiber nanograting orientation by manipulating laser polarization, and tailored space variant fiber nanogratings, which expanded the diversity in fiber nanograting engineering.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Yibo Liu, Yujie Tao, Yue Liu, Qi Sun, Qinrong Lin, Kexin Kang, Qinghua Zhang, Qingjie Sun
Summary: This study investigates the wettability of the Ti-Cu-Fe multi-metal system, specifically the wetting behaviors of CuSi3 droplets on TC4 and 304SS plates. The results show that the CO2 + Ar gas atmosphere significantly affects interfacial mass transfer, thus influencing the wettability of the systems.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Jimei Liu, Fei Wang, Rong Guo, Yuqi Liu, Mengyu Zhang, Jaka Sunarso, Dong Liu
Summary: This study developed Co/MXene composites with anti-corrosion properties by varying the cobalt content. These composites exhibited remarkable electromagnetic absorption performance and high resistance to corrosion under various corrosive conditions. The study also revealed the mechanism of electron transfer from cobalt to MXene and the electromagnetic dissipation behavior originated from polarization loss alone.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Moujie Huang, Yongsong Ma, Jingbo Yang, Lingyun Xu, Hangqi Yang, Miao Wang, Xin Ma, Xin Xia, Junhao Yang, Deli Wang, Chuang Peng
Summary: Strong metal-support interactions (SMSIs) are important for enhancing catalytic activities and stability in thermal catalysis. This study demonstrates a method to create SMSIs in electrocatalysis using carbon nanotubes and Ru nanoparticles, resulting in excellent catalytic activity and stability.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Ravi Trivedi, Brinti Mondal, Nandini Garg, Brahmananda Chakraborty
Summary: This study explores the potential of biphenylene as a nanocarrier for the delivery of the anticancer drug cisplatin. It is found that biphenylene offers physical stability, rapid release rate, solubility, and bio-compatibilities compared to other nanocarriers. The adsorption of cisplatin on the surface of biphenylene involves charge transfer from cisplatin to biphenylene. The drug is shown to be released at body temperature in an acidic environment. Biphenylene also exhibits excellent cytotoxicity activity and cellular uptake of the drug. Overall, biphenylene shows promise as a potential nanocarrier for cisplatin delivery.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Hyun Jeong, Hyeong Chan Suh, Ga Hyun Cho, Rafael Salas-Montiel, Hayoung Ko, Ki Kang Kim, Mun Seok Jeong
Summary: In this study, a potential platform to enhance Raman scattering and increase the number of observable Raman modes in monolayer transition metal dichalcogenides (TMDs) was proposed. The platform consisted of large-scale arrays of gold micropillars (MPs), which were able to enhance the Raman intensity of TMDs and make difficult-to-detect Raman modes observable. The platform showed great industrial advantages and wide applicability due to its low cost, simple process, large controllable area, and short process time.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Yasir Abbas, Shafqat Ali, Sajjad Ali, Waqar Azeem, Zareen Zuhra, Haoliang Wang, Mohamed Bououdina, Zhenzhong Sun
Summary: In this study, FeOx@SPNO-C core-shell nanospheres as a catalyst for degradation of sulfamethoxazole (SMX) were successfully synthesized. The synergistic interaction between FeOx and SPNO-C, high carbon charge density, and the presence of C = O groups and N/Fe-Nx sites were found to be key factors for the enhanced degradation of SMX.
APPLIED SURFACE SCIENCE
(2024)
Article
Chemistry, Physical
Qiaoting Yang, Yuxiao Gong, Yan Qian, Zhou-Qing Xiao, Serge Cosnier, Xue-Ji Zhang, Robert S. Marks, Dan Shan
Summary: This study proposes a hierarchical confinement strategy to design Prussian blue nanoparticles (PB NPs) with satisfactory electrocatalytic ability and stability. The catalytic synthesis of PB NPs is achieved through a hydrothermal process, and the as-prepared PB@NH2MIL exhibits efficient electronic transmission and enhanced electrocatalytic properties.
APPLIED SURFACE SCIENCE
(2024)