期刊
ORGANIC LETTERS
卷 21, 期 22, 页码 9076-9079出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.9b03468
关键词
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资金
- National Natural Science Foundation of China [21572024]
- Jiangsu Key Laboratory of Advanced Catalytic Materials Technology [BM2012110]
- Green Manufacturing Collaborative Innovation Center
A copper-catalyzed 1,2-difiinctionalization of ynamides has been developed by using readily available N,O-acetals as the bifunctional reagents. Importantly, contrary to the initially expected 1,2-oxy-aminomethylation reaction, an unprecedented 1,2-amino-oxymethylation has been observed. This reaction is atom-economical and tolerates a broad substrate scope, affording the difunctionalization products in good yield with unique Z configuration.
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